Magnetic structure and dispersion relation of the S=12 quasi-one-dimensional Ising-like antiferromagnet BaCo2V2O8 in a transverse magnetic field

Matsuda, M.; Onishi, H.; Okutani, A.; Ma, J.; Agrawal, H.; Hong, Tao; Pajerowski, D. M.; Copley, J. R. D.; Okunishi, K.; Mori, M.; Kimura, S.; Hagiwara, M.

doi:10.1103/PhysRevB.96.024439

Title: Magnetic structure and dispersion relation of the $S = \frac{1}{2}$ quasi-one-dimensional Ising-like antiferromagnet ${BaCo}_{2} V_{2} O_{8}$ in a transverse magnetic field

Journal Article · Tue Jul 25 00:00:00 EDT 2017 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.96.024439· OSTI ID:1376477

Matsuda, M. ^[1]; Onishi, H. ^[2]; Okutani, A. ^[3]; Ma, J. ^[4]; Agrawal, H. ^[1];

^[1]; Pajerowski, D. M. ^[5]; Copley, J. R. D. ^[6]; Okunishi, K. ^[7]; Mori, M. ^[2]; Kimura, S. ^[8]; Hagiwara, M. ^[3]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Japan Atomic Energy Agency, Ibaraki (Japan)
Osaka Univ., Osaka (Japan)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Shanghai Jiao Tong Univ., Shanghai (People's Republic of China)
NIST Center for Neutron Research, Gaithersburg, MD (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
NIST Center for Neutron Research, Gaithersburg, MD (United States)
Niigata Univ., Niigata (Japan)
Tohoku Univ., Sendai (Japan)

Here, BaCo₂V₂O₈ consists of Co chains in which a Co²⁺ ion carries a fictitious spin 1/2 with Ising anisotropy. We performed elastic and inelastic neutron scattering experiments in BaCo₂V₂O₈ in a magnetic field perpendicular to the c axis which is the chain direction. With applying magnetic field along the a axis at 3.5 K, the antiferromagnetic order with the easy axis along the c axis, observed in zero magnetic field, is completely suppressed at 8 T, while the magnetic field gradually induces an antiferromagnetic order with the spin component along the b axis. We also studied magnetic excitations as a function of transverse magnetic field. The lower boundary of the spinon excitations splits gradually with increasing magnetic field. The overall feature of the magnetic excitation spectra in the magnetic field is reproduced by the theoretical calculation based on the spin 1/2 XXZ antiferromagnetic chain model, which predicts that the dynamic magnetic structure factor of the spin component along the chain direction is enhanced and that along the field direction has clear incommensurate correlations.

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Research Organization:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1376477

Alternate ID(s):: OSTI ID: 1372718

Journal Information:: Physical Review B, Vol. 96, Issue 2; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 10 works

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References (31)

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Spinon confinement and a sharp longitudinal mode in Yb2Pt2Pb in magnetic fields Gannon, W. J.; Zaliznyak, I. A.; Wu, L. S. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-08715-y	journal	March 2019
Intrinsic transverse field in frustrated quantum Ising magnets: Physical origin and quantum effects Chen, Gang Physical Review Research, Vol. 1, Issue 3 https://doi.org/10.1103/physrevresearch.1.033141	journal	December 2019
Spinon Confinement and a Sharp Longitudinal Mode in Yb$_2$Pt$_2$Pb in Magnetic Fields Gannon, W. J.; Zaliznyak, I. A.; Wu, L. S. arXiv https://doi.org/10.48550/arxiv.1907.01067	text	January 2019

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Title: Magnetic structure and dispersion relation of the $S = \frac{1}{2}$ quasi-one-dimensional Ising-like antiferromagnet ${BaCo}_{2} V_{2} O_{8}$ in a transverse magnetic field