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Title: Synthesis of Sn-Loaded Plastic Scintillators.

Abstract

Abstract not provided.

Authors:
;
Publication Date:
Research Org.:
Sandia National Lab. (SNL-CA), Livermore, CA (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1373468
Report Number(s):
SAND2016-7244D
646181
DOE Contract Number:
AC04-94AL85000
Resource Type:
Conference
Resource Relation:
Conference: Proposed for presentation at the Sandia Intern Symposium.
Country of Publication:
United States
Language:
English

Citation Formats

Feist, John, and Feng, Patrick L. Synthesis of Sn-Loaded Plastic Scintillators.. United States: N. p., 2016. Web.
Feist, John, & Feng, Patrick L. Synthesis of Sn-Loaded Plastic Scintillators.. United States.
Feist, John, and Feng, Patrick L. 2016. "Synthesis of Sn-Loaded Plastic Scintillators.". United States. doi:. https://www.osti.gov/servlets/purl/1373468.
@article{osti_1373468,
title = {Synthesis of Sn-Loaded Plastic Scintillators.},
author = {Feist, John and Feng, Patrick L},
abstractNote = {Abstract not provided.},
doi = {},
journal = {},
number = ,
volume = ,
place = {United States},
year = 2016,
month = 7
}

Conference:
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  • Abstract not provided.
  • We are developing new scintillator materials that offer potential for high resolution gamma ray spectroscopy at low cost. Single crystal SrI{sub 2}(Eu) offers {approx}3% resolution at 662 keV, in sizes of {approx}1 in{sup 3}. We have developed ceramics processing technology allowing us to achieve cubic inch scale transparent ceramic scintillators offering gamma spectroscopy performance superior to NaI(Tl). We fabricated a bismuth-loaded plastic scintillator that demonstrates energy resolution of {approx}8% at 662 keV in small sizes. Gamma ray spectroscopy can be used to identify the presence of weak radioactive sources within natural background. The ability to discriminate close-lying spectral lines ismore » strongly dependent upon the energy resolution of the detector. In addition to excellent energy resolution, large volume detectors are needed to acquire sufficient events, for example, to identify a radioactive anomaly moving past a detector. We have employed a 'directed search' methodology for identifying potential scintillator materials candidates, resulting in the discovery of Europium-doped Strontium Iodide, SrI{sub 2}(Eu), Cerium-doped Gadolinium Garnet, GYGAG(Ce), and Bismuth-loaded Polymers. These scintillators possess very low self-radioactivity, offer energy resolution of 3-8% at 662 keV, and have potential to be grown cost-effectively to sizes similar to the most widely deployed gamma spectroscopy scintillator, Thallium-doped Sodium Iodide, NaI(Tl). In this study, gamma ray spectra of a variety of sources, were obtained employing SrI{sub 2}(Eu), GYGAG(Ce), Bi-loaded polymers, LaBr{sub 3}(Ce), and NaI(Tl). The effects of detector size, energy resolution, and background radioactivity (including self-radioactivity) on the ability to distinguish weak sources is quantified, based on a simple model, and qualitatively compared to laboratory data.« less
  • The scope of this project intends to record spatially resolved images of core shape and size of a DT micro-balloon during Inertial Confinement Fusion (ICF) experiments at Laser Mega Joule facility (LMJ). We need to develop an X-ray imaging system which can operate in the radiative background generated by an ignition shot of ICF. The scintillator is a part of the imaging system and has to gather a compromise of scintillating properties (scintillating efficiency, decay time, emission wavelength) so as to both operate in the hard radiative environment and to allow the acquisition of spatially resolved images. Inorganic scintillators cannotmore » be used because no compromise can be found regarding the expected scintillating properties, most of them are not fast enough and emit blue light. Organic scintillators are generally fast, but present low X-ray absorption in the 10 to 40 keV range, that does not permit the acquisition of spatially resolved images. To this aim, we have developed highly lead-loaded and red-fluorescent fast plastic scintillators. Such a combination is not currently available via scintillator suppliers, since they propose only blue-fluorescent plastic scintillators doped with up to 12%w Pb. Thus, incorporation ratio up to 27%w Pb has been reached in our laboratory, which can afford a plastic scintillator with an outstanding Z{sub eff} close to 50. X-rays in the 10 to 40 keV range can thus be detected with a higher probability of photoelectric effect than for classic organic scintillators, such as NE102. The strong orange-red fluorescence can be filtered, so that we can eliminate residual Cerenkov light, generated by {gamma}-ray absorption in glass parts of the imaging system. Decay times of our scintillators evaluated under UV excitation were estimated to be in the range 10 to 13 ns. (authors)« less
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