Ultrafast Plasmonic Control of Second Harmonic Generation

Davidson, Roderick B.; Yanchenko, Anna; Ziegler, Jed I.; Avanesyan, Sergey M.; Lawrie, Benjamin J.; Haglund, Richard F.

doi:10.1021/acsphotonics.6b00034

Title: Ultrafast Plasmonic Control of Second Harmonic Generation

Journal Article · Wed Jun 01 00:00:00 EDT 2016 · ACS Photonics

DOI:https://doi.org/10.1021/acsphotonics.6b00034· OSTI ID:1364273

Davidson, Roderick B. ^[1]; Yanchenko, Anna ^[2]; Ziegler, Jed I. ^[3]; Avanesyan, Sergey M. ^[3]; Lawrie, Benjamin J. ^[4]; Haglund, Richard F. ^[3]

Vanderbilt Univ., Nashville, TN (United States). Dept. of Physics and Astronomy; Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Computational Sciences and Engineering Division
Vanderbilt Univ., Nashville, TN (United States). Dept. of Physics and Astronomy; Univ. of Virginia, Charlottesville, VA (United States). Dept. of Physics
Vanderbilt Univ., Nashville, TN (United States). Dept. of Physics and Astronomy
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Computational Sciences and Engineering Division

Efficient frequency conversion techniques are crucial to the development of plasmonic metasurfaces for information processing and signal modulation. In principle, nanoscale electric-field confinement in nonlinear materials enables higher harmonic conversion efficiencies per unit volume than those attainable in bulk materials. Here we demonstrate efficient second-harmonic generation (SHG) in a serrated nanogap plasmonic geometry that generates steep electric field gradients on a dielectric metasurface. An ultrafast control pulse is used to control plasmon-induced electric fields in a thin-film material with inversion symmetry that, without plasmonic enhancement, does not exhibit an even-order nonlinear optical response. The temporal evolution of the plasmonic near-field is characterized with ~100 as resolution using a novel nonlinear interferometric technique. The serrated nanogap is a unique platform in which to investigate optically controlled, plasmonically enhanced harmonic generation in dielectric materials on an ultrafast time scale. Lastly, this metamaterial geometry can also be readily extended to all-optical control of other nonlinear phenomena, such as four-wave mixing and sum- and difference-frequency generation, in a wide variety of dielectric materials.

View Accepted Manuscript (DOE)

Cite

Export

Save

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Oak Ridge Leadership Computing Facility (OLCF)

Sponsoring Organization:: USDOE Laboratory Directed Research and Development (LDRD) Program; National Science Foundation (NSF); USDOE Office of Science (SC)

Grant/Contract Number:: AC05-00OR22725; FG02-01ER45916

OSTI ID:: 1364273

Journal Information:: ACS Photonics, Vol. 3, Issue 8; ISSN 2330-4022

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 18 works

Citation information provided by
Web of Science

References (18)

Nonlinear plasmonics Kauranen, Martti; Zayats, Anatoly V. Nature Photonics, Vol. 6, Issue 11 https://doi.org/10.1038/nphoton.2012.244	journal	November 2012
Active nanoplasmonic metamaterials Hess, O.; Pendry, J. B.; Maier, S. A. Nature Materials, Vol. 11, Issue 7 https://doi.org/10.1038/nmat3356	journal	June 2012
High-speed plasmonic phase modulators Melikyan, A.; Alloatti, L.; Muslija, A. Nature Photonics, Vol. 8, Issue 3 https://doi.org/10.1038/nphoton.2014.9	journal	February 2014
Efficient forward second-harmonic generation from planar archimedean nanospirals Davidson II, Roderick B.; Ziegler, Jed I.; Vargas, Guillermo Nanophotonics, Vol. 4, Issue 1 https://doi.org/10.1515/nanoph-2015-0002	journal	January 2015
Multiresonant Broadband Optical Antennas As Efficient Tunable Nanosources of Second Harmonic Light Aouani, Heykel; Navarro-Cia, Miguel; Rahmani, Mohsen Nano Letters, Vol. 12, Issue 9 https://doi.org/10.1021/nl302665m	journal	January 2012
Three-Dimensional Nanostructures as Highly Efficient Generators of Second Harmonic Light Zhang, Yu; Grady, Nathaniel K.; Ayala-Orozco, Ciceron Nano Letters, Vol. 11, Issue 12 https://doi.org/10.1021/nl2033602	journal	December 2011
Multipolar second harmonic generation from planar arrays of Au nanoparticles Capretti, Antonio; Walsh, Gary F.; Minissale, Salvatore Optics Express, Vol. 20, Issue 14 https://doi.org/10.1364/OE.20.015797	journal	January 2012
Size-dependent second-harmonic generation from gold nanoparticles Capretti, Antonio; Pecora, Emanuele F.; Forestiere, Carlo Physical Review B, Vol. 89, Issue 12 https://doi.org/10.1103/PhysRevB.89.125414	journal	March 2014
Giant nonlinear response from plasmonic metasurfaces coupled to intersubband transitions Lee, Jongwon; Tymchenko, Mykhailo; Argyropoulos, Christos Nature, Vol. 511, Issue 7507 https://doi.org/10.1038/nature13455	journal	July 2014
Third-harmonic-upconversion enhancement from a single semiconductor nanoparticle coupled to a plasmonic antenna Aouani, Heykel; Rahmani, Mohsen; Navarro-Cía, Miguel Nature Nanotechnology, Vol. 9, Issue 4 https://doi.org/10.1038/nnano.2014.27	journal	March 2014
Spatiotemporal control of nanooptical excitations Aeschlimann, M.; Bauer, M.; Bayer, D. Proceedings of the National Academy of Sciences, Vol. 107, Issue 12 https://doi.org/10.1073/pnas.0913556107	journal	March 2010
Tailoring Spatiotemporal Light Confinement in Single Plasmonic Nanoantennas Hanke, Tobias; Cesar, Julijan; Knittel, Vanessa Nano Letters, Vol. 12, Issue 2 https://doi.org/10.1021/nl2041047	journal	January 2012
Electrically Controlled Nonlinear Generation of Light with Plasmonics Cai, W.; Vasudev, A. P.; Brongersma, M. L. Science, Vol. 333, Issue 6050 https://doi.org/10.1126/science.1207858	journal	September 2011
Electrifying photonic metamaterials for tunable nonlinear optics Kang, Lei; Cui, Yonghao; Lan, Shoufeng Nature Communications, Vol. 5, Issue 1 https://doi.org/10.1038/ncomms5680	journal	August 2014
Near-Field Two-Photon-Induced Photoluminescence from Single Gold Nanorods and Imaging of Plasmon Modes Imura, Kohei; Nagahara, Tetsuhiko; Okamoto, Hiromi The Journal of Physical Chemistry B, Vol. 109, Issue 27 https://doi.org/10.1021/jp051631o	journal	July 2005
Terahertz-field-induced second harmonic generation through Pockels effect in zinc telluride crystal Cornet, Marion; Degert, Jérôme; Abraham, Emmanuel Optics Letters, Vol. 39, Issue 20 https://doi.org/10.1364/OL.39.005921	journal	January 2014
Multiple Independent Comb Shaping (MICS): Phase-only generation of optical pulse sequences Pestov, Dmitry; Lozovoy, Vadim V.; Dantus, Marcos Optics Express, Vol. 17, Issue 16 https://doi.org/10.1364/OE.17.014351	journal	January 2009
Optical Constants of the Noble Metals Johnson, P. B.; Christy, R. W. Physical Review B, Vol. 6, Issue 12, p. 4370-4379 https://doi.org/10.1103/PhysRevB.6.4370	journal	December 1972

Cited By (3)

Nanofocusing in SOI-based hybrid plasmonic metal slot waveguides Güsken, Nicholas A.; Nielsen, Michael P.; Nguyen, Ngoc B. Optics Express, Vol. 26, Issue 23 https://doi.org/10.1364/oe.26.030634	journal	January 2018
Fano Resonance on Nanostructured Lithium Niobate for Highly Efficient and Tunable Second Harmonic Generation Huang, Zhijin; Lu, Huihui; Xiong, Hanqing Nanomaterials, Vol. 9, Issue 1 https://doi.org/10.3390/nano9010069	journal	January 2019
ALD assisted nanoplasmonic slot waveguide for on-chip enhanced Raman spectroscopy Raza, Ali; Clemmen, Stéphane; Wuytens, Pieter APL Photonics, Vol. 3, Issue 11 https://doi.org/10.1063/1.5048266	journal	November 2018

Similar Records

Efficient nonlinear metasurface based on nonplanar plasmonic nanocavities

Journal Article · Mon Apr 03 00:00:00 EDT 2017 · ACS Photonics · OSTI ID:1364273

Wang, Feng; Martinson, Alex B. F.; Harutyunyan, Hayk

Resonantly enhanced second-harmonic generation using III–V semiconductor all-dielectric metasurfaces

Journal Article · Mon Aug 08 00:00:00 EDT 2016 · Nano Letters · OSTI ID:1364273

Liu, Sheng; Sinclair, Michael B.; Saravi, Sina; +8 more

Dynamically tunable second-harmonic generation using hybrid nanostructures incorporating phase-change chalcogenides

Journal Article · Tue Apr 26 00:00:00 EDT 2022 · Nanophotonics (Online) · OSTI ID:1364273

Zhu, Muliang; Abdollahramezani, Sajjad; Li, Chentao; +3 more

Related Subjects

36 MATERIALS SCIENCE
interferometry
metasurfaces
nonlinear optics
optical control
plasmonic enhancement

Title: Ultrafast Plasmonic Control of Second Harmonic Generation

Citation Formats

References (18)

Cited By (3)

Similar Records

Related Subjects