A new electron-ion coincidence 3D momentum-imaging method and its application in probing strong field dynamics of 2-phenylethyl-N, N-dimethylamine

Fan, Lin; Lee, Suk Kyoung; Tu, Yi-Jung; Mignolet, Benoît; Couch, David; Dorney, Kevin; Nguyen, Quynh; Wooldridge, Laura; Murnane, Margaret; Remacle, Françoise; Schlegel, H. Bernhard; Li, Wen

doi:10.1063/1.4981526

Title: A new electron-ion coincidence 3D momentum-imaging method and its application in probing strong field dynamics of 2-phenylethyl-N, N-dimethylamine

Journal Article · Mon Apr 24 00:00:00 EDT 2017 · Journal of Chemical Physics

DOI:https://doi.org/10.1063/1.4981526· OSTI ID:1465981

Fan, Lin ^[1]; Lee, Suk Kyoung ^[1]; Tu, Yi-Jung ^[1];

^[2]; Couch, David ^[3]; Dorney, Kevin ^[3]; Nguyen, Quynh ^[3]; Wooldridge, Laura ^[3]; Murnane, Margaret ^[3]; Remacle, Françoise ^[2];

^[1]; Li, Wen ^[1]

Wayne State Univ., Detroit, MI (United States). Dept. of Chemistry
Univ. of Liège (Belgium). Dept. of Chemistry
Univ. of Colorado, Boulder, CO (United States). JILA

In this paper, we report the development of a new three-dimensional (3D) momentum-imaging setup based on conventional velocity map imaging to achieve the coincidence measurement of photoelectrons and photo-ions. This setup uses only one imaging detector (microchannel plates (MCP)/phosphor screen) but the voltages on electrodes are pulsed to push both electrons and ions toward the same detector. The ion-electron coincidence is achieved using two cameras to capture images of ions and electrons separately. The time-of-flight of ions and electrons are read out from MCP using a digitizer. We demonstrate this new system by studying the dissociative single and double ionization of PENNA (2-phenylethyl-N,N-dimethylamine). Finally, we further show that the camera-based 3D imaging system can operate at 10 kHz repetition rate.

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Research Organization:: Wayne State Univ., Detroit, MI (United States); Univ. of Liege, (Belgium)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Fund for Scientific Research (F.R.S.-FNRS) (Belgium)

Grant/Contract Number:: SC0012628; 2.5020.11

OSTI ID:: 1465981

Alternate ID(s):: OSTI ID: 1361835

Journal Information:: Journal of Chemical Physics, Vol. 147, Issue 1; ISSN 0021-9606

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

References (32)

Observation of Site-Specific Electron Emission in the Decay of Superexcited $O_{2}$ Golovin, A. V.; Heiser, F.; Quayle, C. J. K. Physical Review Letters, Vol. 79, Issue 23 https://doi.org/10.1103/physrevlett.79.4554	journal	December 1997
Control of Local Ionization and Charge Transfer in the Bifunctional Molecule 2-Phenylethyl- N , N -dimethylamine Using Rydberg Fingerprint Spectroscopy Cheng, Wei; Kuthirummal, Narayanan; Gosselin, Jaimie L. The Journal of Physical Chemistry A, Vol. 109, Issue 9 https://doi.org/10.1021/jp046400g	journal	March 2005
Ion dissociation dynamics and thermochemistry by photoelectron photoion coincidence (PEPICO) spectroscopy Baer, Tomas International Journal of Mass Spectrometry, Vol. 200, Issue 1-3 https://doi.org/10.1016/s1387-3806(00)00327-4	journal	December 2000
Communication: Time- and space-sliced velocity map electron imaging Lee, Suk Kyoung; Lin, Yun Fei; Lingenfelter, Steven The Journal of Chemical Physics, Vol. 141, Issue 22 https://doi.org/10.1063/1.4903744	journal	December 2014
A photoelectron-photoion coincidence imaging apparatus for femtosecond time-resolved molecular dynamics with electron time-of-flight resolution of σ=18ps and energy resolution ΔE∕E=3.5% Vredenborg, Arno; Roeterdink, Wim G.; Janssen, Maurice H. M. Review of Scientific Instruments, Vol. 79, Issue 6 https://doi.org/10.1063/1.2949142	journal	June 2008
State-resolved three-dimensional electron-momentum correlation in nonsequential double ionization of benzene Winney, Alexander H.; Lin, Yun Fei; Lee, Suk Kyoung Physical Review A, Vol. 93, Issue 3 https://doi.org/10.1103/physreva.93.031402	journal	March 2016
Femtosecond Coincidence Imaging of Multichannel Multiphoton Dynamics Rijs, Anouk M.; Janssen, Maurice H. M.; Chrysostom, Engelene t. H. Physical Review Letters, Vol. 92, Issue 12 https://doi.org/10.1103/physrevlett.92.123002	journal	March 2004
Direct current slice imaging Townsend, Dave; Minitti, Michael P.; Suits, Arthur G. Review of Scientific Instruments, Vol. 74, Issue 4 https://doi.org/10.1063/1.1544053	journal	April 2003
Velocity map photoelectron-photoion coincidence imaging on a single detector Lehmann, C. Stefan; Ram, N. Bhargava; Janssen, Maurice H. M. Review of Scientific Instruments, Vol. 83, Issue 9 https://doi.org/10.1063/1.4749843	journal	September 2012
K-shell photoionization of CO and N ₂ : is there a link between the photoelectron angular distribution and the molecular decay dynamics? Weber, Th; Jagutzki, O.; Hattass, M. Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 34, Issue 18 https://doi.org/10.1088/0953-4075/34/18/305	journal	September 2001
A photoelectron-photoion coincidence spectrometer for the study of translational energy release distributions Powis, I.; Mansell, P. I.; Danby, C. J. International Journal of Mass Spectrometry and Ion Physics, Vol. 32, Issue 1 https://doi.org/10.1016/0020-7381(79)80079-0	journal	November 1979
Nuclear spatial delocalization silences electron density oscillations in 2-phenyl-ethyl-amine (PEA) and 2-phenylethyl-N,N-dimethylamine (PENNA) cations Jenkins, Andrew J.; Vacher, Morgane; Bearpark, Michael J. The Journal of Chemical Physics, Vol. 144, Issue 10 https://doi.org/10.1063/1.4943273	journal	March 2016
Femtosecond time-resolved photoelectron–photoion coincidence imaging studies of dissociation dynamics Davies, J. A.; LeClaire, J. E.; Continetti, R. E. The Journal of Chemical Physics, Vol. 111, Issue 1 https://doi.org/10.1063/1.479248	journal	July 1999
Femtosecond Dynamics after Ionization: 2-Phenylethyl- N , N -dimethylamine as a Model System for Nonresonant Downhill Charge Transfer in Peptides Lehr, L.; Horneff, T.; Weinkauf, R. The Journal of Physical Chemistry A, Vol. 109, Issue 36 https://doi.org/10.1021/jp0210935	journal	September 2005
Nuclear Motion Driven Ultrafast Photodissociative Charge Transfer of the PENNA Cation: An Experimental and Computational Study Sun, Shoutian; Mignolet, Benoit; Fan, Lin The Journal of Physical Chemistry A, Vol. 121, Issue 7 https://doi.org/10.1021/acs.jpca.6b12310	journal	February 2017
Dissociative Energy Flow, Vibrational Energy Redistribution, and Conformeric Structural Dynamics in Bifunctional Amine Model Systems ^† Bush, Joseph C.; Minitti, Michael P.; Weber, Peter M. The Journal of Physical Chemistry A, Vol. 114, Issue 42 https://doi.org/10.1021/jp101881x	journal	October 2010
Velocity map imaging of ions and electrons using electrostatic lenses: Application in photoelectron and photofragment ion imaging of molecular oxygen Eppink, André T. J. B.; Parker, David H. Review of Scientific Instruments, Vol. 68, Issue 9 https://doi.org/10.1063/1.1148310	journal	September 1997
Coincidence ion imaging with a fast frame camera Lee, Suk Kyoung; Cudry, Fadia; Lin, Yun Fei Review of Scientific Instruments, Vol. 85, Issue 12 https://doi.org/10.1063/1.4903856	journal	December 2014
A velocity map imaging spectrometer for electron–ion and ion–ion coincidence experiments with synchrotron radiation Rolles, D.; Pešić, Z. D.; Perri, M. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 261, Issue 1-2 https://doi.org/10.1016/j.nimb.2007.04.186	journal	August 2007
Ultrafast charge migration in 2-phenylethyl-N,N-dimethylamine Lünnemann, Siegfried; Kuleff, Alexander I.; Cederbaum, Lorenz S. Chemical Physics Letters, Vol. 450, Issue 4-6 https://doi.org/10.1016/j.cplett.2007.11.031	journal	January 2008
Ion–electron velocity vector correlations in dissociative photoionization of simple molecules using electrostatic lenses Lebech, M.; Houver, J. C.; Dowek, D. Review of Scientific Instruments, Vol. 73, Issue 4 https://doi.org/10.1063/1.1458063	journal	April 2002
Photoelectron-photoion coincidence spectroscopy Danby, C. J.; Eland, J. H. D. International Journal of Mass Spectrometry and Ion Physics, Vol. 8, Issue 2 https://doi.org/10.1016/0020-7381(72)80005-6	journal	February 1972
Improved sliced velocity map imaging apparatus optimized for H photofragments Ryazanov, Mikhail; Reisler, Hanna The Journal of Chemical Physics, Vol. 138, Issue 14 https://doi.org/10.1063/1.4798929	journal	April 2013
Charge migration in the bifunctional PENNA cation induced and probed by ultrafast ionization: a dynamical study Mignolet, B.; Levine, R. D.; Remacle, F. Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 47, Issue 12 https://doi.org/10.1088/0953-4075/47/12/124011	journal	June 2014
Note: An improved 3D imaging system for electron-electron coincidence measurements Lin, Yun Fei; Lee, Suk Kyoung; Adhikari, Pradip Review of Scientific Instruments, Vol. 86, Issue 9 https://doi.org/10.1063/1.4931684	journal	September 2015
Self‐consistent molecular orbital methods. XXIII. A polarization‐type basis set for second‐row elements Francl, Michelle M.; Pietro, William J.; Hehre, Warren J. The Journal of Chemical Physics, Vol. 77, Issue 7, p. 3654-3665 https://doi.org/10.1063/1.444267	journal	October 1982
Local Ionization in 2-Phenylethyl- N , N -dimethylamine: Charge Transfer and Dissociation Directly after Ionization Weinkauf, R.; Lehr, L.; Metsala, A. The Journal of Physical Chemistry A, Vol. 107, Issue 16 https://doi.org/10.1021/jp021092c	journal	April 2003
Suppression of hot electrons in threshold photoelectron photoion coincidence spectroscopy using velocity focusing optics Sztáray, Bálint; Baer, Tomas Review of Scientific Instruments, Vol. 74, Issue 8 https://doi.org/10.1063/1.1593788	journal	August 2003
Charge migration following ionization in systems with chromophore-donor and amine-acceptor sites Lünnemann, Siegfried; Kuleff, Alexander I.; Cederbaum, Lorenz S. The Journal of Chemical Physics, Vol. 129, Issue 10 https://doi.org/10.1063/1.2970088	journal	September 2008
Control of electronic dynamics visualized by angularly resolved photoelectron spectra: A dynamical simulation with an IR pump and XUV attosecond-pulse-train probe Mignolet, B.; Levine, R. D.; Remacle, F. Physical Review A, Vol. 89, Issue 2 https://doi.org/10.1103/physreva.89.021403	journal	February 2014
Long-range corrected hybrid density functionals with damped atom–atom dispersion corrections Chai, Jeng-Da; Head-Gordon, Martin Physical Chemistry Chemical Physics, Vol. 10, Issue 44 https://doi.org/10.1039/b810189b	journal	January 2008
An Antifungal Polycyclic Tetramate Macrolactam, Heat-Stable Antifungal Factor (HSAF), Is a Novel Oxidative Stress Modulator in Lysobacter enzymogenes Yu, Lingjun; Li, Hui; Zhou, Zaichun Applied and Environmental Microbiology, Vol. 87, Issue 10 https://doi.org/10.1128/aem.03105-20	journal	April 2021

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A coincidence velocity map imaging spectrometer for ions and high-energy electrons to study inner-shell photoionization of gas-phase molecules Ablikim, Utuq; Bomme, Cédric; Osipov, Timur Review of Scientific Instruments, Vol. 90, Issue 5 https://doi.org/10.1063/1.5093420	journal	May 2019
Direct in-situ single-shot measurements of the absolute carrier-envelope phases of ultrashort pulses Debrah, Duke A.; Stewart, Gabriel A.; Basnayake, Gihan Optics Letters, Vol. 44, Issue 14 https://doi.org/10.1364/ol.44.003582	journal	January 2019
A Coincidence Velocity Map Imaging Spectrometer for Ions and High-Energy Electrons to Study Inner-Shell Photoionization of Gas-Phase Molecules Ablikim, Utuq; Bomme, Cédric; Osipov, Timur arXiv https://doi.org/10.48550/arxiv.1904.09938	text	January 2019

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Title: A new electron-ion coincidence 3D momentum-imaging method and its application in probing strong field dynamics of 2-phenylethyl-N, N-dimethylamine

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