Orientation-resolved domain mapping in tetragonal SrTiO3 using polarized Raman spectroscopy

Gray, Jr., Dodd J.; Merz, Tyler A.; Hikita, Yasuyuki; Hwang, Harold Y.; Mabuchi, Hideo

doi:10.1103/PhysRevB.94.214107

Title: Orientation-resolved domain mapping in tetragonal ${SrTiO}_{3}$ using polarized Raman spectroscopy

Journal Article · Fri Dec 16 00:00:00 EST 2016 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.94.214107· OSTI ID:1361076

Gray, Jr., Dodd J. ^[1]; Merz, Tyler A. ^[1]; Hikita, Yasuyuki ^[2]; Hwang, Harold Y. ^[3]; Mabuchi, Hideo ^[1]

Stanford Univ., Stanford, CA (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Stanford Univ., Stanford, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)

Here, we present microscopically resolved, polarized spectroscopy of Raman scattering collected from tetragonal SrTiO₃. The anisotropic response of first-order Raman peaks within a single tetragonal domain has been measured. From these data, we assign symmetries to the phonons seen in the first-order Raman spectrum which is normally complicated by uncontrolled domain structure. Using a translation stage, we map the local domain orientation of a 3–μm³ crystal volume near the laser focus and compare it to wide-field polarized images. This technique can be performed with readily available instruments and is relevant to the study of a wide range of related materials, interfaces, and devices.

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Research Organization:: SLAC National Accelerator Lab., Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: N66001-11-1-4106; AC02-76SF00515; DGE-114747

OSTI ID:: 1361076

Alternate ID(s):: OSTI ID: 1336852

Journal Information:: Physical Review B, Vol. 94, Issue 21; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 7 works

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Carrier density and disorder tuned superconductor-metal transition in a two-dimensional electron system Chen, Zhuoyu; Swartz, Adrian G.; Yoon, Hyeok Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-06444-2	journal	October 2018
Physics of SrTiO ₃ -based heterostructures and nanostructures: a review Pai, Yun-Yi; Tylan-Tyler, Anthony; Irvin, Patrick Reports on Progress in Physics, Vol. 81, Issue 3 https://doi.org/10.1088/1361-6633/aa892d	journal	February 2018
Physics of SrTiO$_3$-based heterostructures and nanostructures: a review Pai, Yun-Yi; Tylan-Tyler, Anthony; Irvin, Patrick arXiv https://doi.org/10.48550/arxiv.1702.07690	text	January 2017

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