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Title: 2D materials advances: from large scale synthesis and controlled heterostructures to improved characterization techniques, defects and applications

Journal Article · · 2D Materials
 [1];  [1];  [2];  [2];  [2];  [3];  [4];  [5];  [6];  [7];  [8];  [9];  [10];  [11];  [4]; ORCiD logo [12];  [13];  [14];  [15];  [16] more »;  [3];  [17];  [18];  [19];  [20] « less
  1. Pennsylvania State Univ., University Park, PA (United States). Dept of Physics; Pennsylvania State Univ., University Park, PA (United States). Center for 2-Dimensional and Layered Materials
  2. Pennsylvania State Univ., University Park, PA (United States). Center for 2-Dimensional and Layered Materials; Pennsylvania State Univ., University Park, PA (United States). Dept of Materials Sciences and Engineering
  3. Pennsylvania State Univ., University Park, PA (United States). Center for 2-Dimensional and Layered Materials; Pennsylvania State Univ., University Park, PA (United States). Dept of Chemistry
  4. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Science (CNMS)
  5. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Molecular Foundry
  6. Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials; SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES)
  7. Univ. of Pittsburgh, PA (United States). Dept. of Chemical and Petroleum Engineering
  8. Univ. of Regensburg (Germany). Inst. fur Experimentelle und Angewandte Physik; Columbia Univ., New York, NY (United States). Dept. of Physics and Electrical Engineering
  9. Univ. of Kansas, Lawrence, KS (United States). Dept. of Physics and Astronomy
  10. Univ. of Virginia, Charlottesville, VA (United States). Dept. of Materials Science and Engineering
  11. Stanford Univ., CA (United States). Dept. of Materials Science and Engineering; SLAC National Accelerator Lab., Menlo Park, CA (United States)
  12. Univ. of Arizona, Tucson, AZ (United States). Dept. of Physics
  13. Univ. of Pennsylvania, Philadelphia, PA (United States). Dept. of Physics and Astronomy
  14. Lehigh Univ., Bethlehem, PA (United States). Dept. of Electrical and Computer Engineering
  15. Univ. of Chicago, IL (United States). Dept. of Chemistry and Inst. of Molecular Engineering
  16. Rutgers Univ., Piscataway, NJ (United States). Dept. of Materials Science and Engineering; Rutgers Univ., Piscataway, NJ (United States). Dept. of Electrical and Computer Engineering
  17. Univ. of California, Berkeley, CA (United States). Dept. of Electrical Engineering and Computer Sciences; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Sciences Division
  18. Northwestern Univ., Evanston, IL (United States). Dept. of Materials Science and Engineering; Northwestern Univ., Evanston, IL (United States). Dept of Chemistry
  19. Pennsylvania State Univ., University Park, PA (United States). Center for 2-Dimensional and Layered Materials; Pennsylvania State Univ., University Park, PA (United States). Dept of Materials Sciences and Engineering; Pennsylvania State Univ., University Park, PA (United States). Center for Atomically Thin Multifunctional Coatings (ATOMIC)
  20. Pennsylvania State Univ., University Park, PA (United States). Dept of Physics; Pennsylvania State Univ., University Park, PA (United States). Center for 2-Dimensional and Layered Materials; Pennsylvania State Univ., University Park, PA (United States). Dept of Materials Sciences and Engineering; Pennsylvania State Univ., University Park, PA (United States). Dept of Chemistry; Pennsylvania State Univ., University Park, PA (United States). Center for Atomically Thin Multifunctional Coatings (ATOMIC)

The rise of two-dimensional (2D) materials research took place following the isolation of graphene in 2004. These new 2D materials include transition metal dichalcogenides, mono-elemental 2D sheets, and several carbide- and nitride-based materials. The number of publications related to these emerging materials has been drastically increasing over the last five years. Thus, through this comprehensive review, we aim to discuss the most recent groundbreaking discoveries as well as emerging opportunities and remaining challenges. This review starts out by delving into the improved methods of producing these new 2D materials via controlled exfoliation, metal organic chemical vapor deposition, and wet chemical means. We look into recent studies of doping as well as the optical properties of 2D materials and their heterostructures. Recent advances towards applications of these materials in 2D electronics are also reviewed, and include the tunnel MOSFET and ways to reduce the contact resistance for fabricating high-quality devices. Finally, several unique and innovative applications recently explored are discussed as well as perspectives of this exciting and fast moving field.

Research Organization:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
AC02-76SF00515; AC02-05CH11231
OSTI ID:
1360213
Alternate ID(s):
OSTI ID: 1468337
Journal Information:
2D Materials, Vol. 3, Issue 4; ISSN 2053-1583
Publisher:
IOP PublishingCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 377 works
Citation information provided by
Web of Science

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High-Resolution Patterning of Graphene by Screen Printing with a Silicon Stencil for Highly Flexible Printed Electronics journal November 2014
Three-Dimensional Printing of High-Content Graphene Scaffolds for Electronic and Biomedical Applications journal February 2015
Rapid and Versatile Photonic Annealing of Graphene Inks for Flexible Printed Electronics journal September 2015
Gate-tunable carbon nanotube-MoS2 heterojunction p-n diode journal October 2013
Large-Area, Low-Voltage, Antiambipolar Heterojunctions from Solution-Processed Semiconductors journal December 2014
Gate-tunable memristive phenomena mediated by grain boundaries in single-layer MoS2 journal April 2015
Hybrid, Gate-Tunable, van der Waals p–n Heterojunctions from Pentacene and MoS 2 journal December 2015
Fabrication of solid-state nanopores with single-nanometre precision journal July 2003
Controllable Atomic Scale Patterning of Freestanding Monolayer Graphene at Elevated Temperature journal January 2013
Correlating Atomic Structure and Transport in Suspended Graphene Nanoribbons journal June 2014
Controlled Sculpture of Black Phosphorus Nanoribbons journal May 2016
Local electrical potential detection of DNA by nanowire–nanopore sensors journal December 2011
Detecting the translocation of DNA through a nanopore using graphene nanoribbons journal November 2013
Toward Sensitive Graphene Nanoribbon–Nanopore Devices by Preventing Electron Beam-Induced Damage journal November 2013
Cross-Talk Between Ionic and Nanoribbon Current Signals in Graphene Nanoribbon-Nanopore Sensors for Single-Molecule Detection journal October 2015
In Situ Electronic Characterization of Graphene Nanoconstrictions Fabricated in a Transmission Electron Microscope journal December 2011
In Situ Transmission Electron Microscopy Modulation of Transport in Graphene Nanoribbons journal April 2016
Electrical Transport Measured in Atomic Carbon Chains journal July 2013
Suspended Solid-state Membranes on Glass Chips with Sub 1-pF Capacitance for Biomolecule Sensing Applications journal December 2015
Measurement of DNA Translocation Dynamics in a Solid-State Nanopore at 100 ns Temporal Resolution journal June 2016
Electron beam nanosculpting of suspended graphene sheets journal September 2008
Graphene as a subnanometre trans-electrode membrane journal August 2010
Atomically Thin Molybdenum Disulfide Nanopores with High Sensitivity for DNA Translocation journal February 2014
Boron Nitride Nanopores: Highly Sensitive DNA Single-Molecule Detectors journal June 2013
Nanopore Fabrication by Controlled Dielectric Breakdown journal March 2014
Fabricating nanopores with diameters of sub-1 nm to 3 nm using multilevel pulse-voltage injection journal May 2014
Electrical pulse fabrication of graphene nanopores in electrolyte solution journal May 2015
Electrochemical Reaction in Single Layer MoS 2 : Nanopores Opened Atom by Atom journal April 2015
DNA Translocation in Nanometer Thick Silicon Nanopores journal May 2015
Ionic Liquids for Electrolyte-Gating of ZnO Field-Effect Transistors journal June 2012
Proximity Effect in Graphene–Topological-Insulator Heterostructures journal March 2014
Exciton Mapping at Subwavelength Scales in Two-Dimensional Materials journal March 2015
Exciton formation in monolayer transition metal dichalcogenides journal January 2016
Efficient Excitonic Photoluminescence in Direct and Indirect Band Gap Monolayer MoS 2 journal September 2015
Two-Dimensional Heterojunctions from Nonlocal Manipulations of the Interactions journal March 2016
Photonics and optoelectronics of 2D semiconductor transition metal dichalcogenides journal March 2016
High-temperature superfluidity with indirect excitons in van der Waals heterostructures journal July 2014
Probing the Dynamics of the Metallic-to-Semiconducting Structural Phase Transformation in MoS 2 Crystals journal July 2015
The Reemergence of Chemistry for Post-Graphene Two-Dimensional Nanomaterials journal May 2015
Chemically Tailoring Semiconducting Two-Dimensional Transition Metal Dichalcogenides and Black Phosphorus journal April 2016
Defects at the Two-Dimensional Limit journal July 2015
Point Defects and Grain Boundaries in Rotationally Commensurate MoS 2 on Epitaxial Graphene journal March 2016
Probing Out-of-Plane Charge Transport in Black Phosphorus with Graphene-Contacted Vertical Field-Effect Transistors journal March 2016
Synthesis of borophenes: Anisotropic, two-dimensional boron polymorphs journal December 2015
Direct and Scalable Deposition of Atomically Thin Low-Noise MoS 2 Membranes on Apertures journal June 2015
Ultrasharp interfaces grown with Van Der Waals epitaxy journal August 1986
Covalently interconnected transition metal dichalcogenide networks via defect engineering for high-performance electronic devices. text January 2021
Spin-galvanic effect text January 2002
Controlling electron-phonon interactions in graphene at ultra high carrier densities text January 2010
In-situ electronic characterization of graphene nanoconstrictions fabricated in a transmission electron microscope text January 2011
Proximity effect in graphene-topological insulator heterostructures text January 2013
Nanopore Fabrication by Controlled Dielectric Breakdown text January 2013
Large-area, low-voltage, anti-ambipolar heterojunctions from solution-processed semiconductors text January 2014
Quality heterostructures from two dimensional crystals unstable in air by their assembly in inert atmosphere text January 2015
Atomically Thin Resonant Tunnel Diodes built from Synthetic van der Waals Heterostructures text January 2015
Gate-tunable Memristive Phenonmena Mediated by Grain Boundaries in Single Layer MoS2 text January 2015
Esaki diodes in van der Waals heterojunctions with broken-gap energy band alignment text January 2015
Compliant substrate epitaxy: Au on MoS$_2$ text January 2015
Environmental, Thermal, and Electrical Susceptibility of Black Phosphorus Field Effect Transistors preprint January 2015
Pressure-induced commensurate stacking of graphene on boron nitride text January 2016
Spintronics: fundamentals and applications text January 2004

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Scalable Synthesis of Ti 3 C 2 T x MXene journal March 2020
Nanosculpting of Atomically Thin 2D Materials for Site-Specific Photoluminescence Modulation journal February 2018
Long‐Term Stability Control of CVD‐Grown Monolayer MoS 2 journal March 2019
Laser Synthesis, Processing, and Spectroscopy of Atomically-Thin Two Dimensional Materials book January 2018
n- and p-type ohmic contacts at monolayer gallium nitride–metal interfaces journal January 2018
Bi 2 O 3 monolayers from elemental liquid bismuth journal January 2018
Stability limits of elemental 2D metals in graphene pores journal January 2019
A new paradigm of ultrathin 2D nanomaterial adsorbents in aqueous media: graphene and GO, MoS 2 , MXenes, and 2D MOFs journal January 2019
Hybrid catalyst with monoclinic MoTe 2 and platinum for efficient hydrogen evolution journal July 2019
Thermal nonlinear refractive index of graphene based saturable absorber in mode-locked fiber lasers journal October 2018
Investigation of nickel ammonia phosphate with different morphologies as a new high-efficiency flame retardant for epoxy resin journal August 2019
Ultrafast transient absorption measurements of photocarrier dynamics in monolayer and bulk ReSe 2 journal January 2018
Introducing Magnetism into 2D Nonmagnetic Inorganic Layered Crystals: A Brief Review from First-Principles Aspects journal January 2018
Electric Double Layer Field-Effect Transistors Using Two-Dimensional (2D) Layers of Copper Indium Selenide (CuIn7Se11) journal June 2019
Nanotip Contacts for Electric Transport and Field Emission Characterization of Ultrathin MoS2 Flakes journal January 2020
Defect Engineering in 2D Materials: Precise Manipulation and Improved Functionalities journal December 2019
Direct observation of the CVD growth of monolayer MoS 2 using in situ optical spectroscopy journal January 2019
Tuning the Electronic and Photonic Properties of Monolayer MoS 2 via In Situ Rhenium Substitutional Doping journal February 2018
Mechanically Flexible Conductors for Stretchable and Wearable E‐Skin and E‐Textile Devices journal May 2019
Design, Synthesis, and Surface Modification of Materials Based on Transition-Metal Dichalcogenides for Biomedical Applications journal November 2017
A review on nanomaterial-based field effect transistor technology for biomarker detection journal November 2019
Solution synthesis of few-layer WTe 2 and Mo x W 1−x Te 2 nanostructures journal January 2017
Control of spintronic and electronic properties of bimetallic and vacancy-ordered vanadium carbide MXenes via surface functionalization journal January 2019
Ultralow thermal conductivity of turbostratically disordered MoSe 2 ultra-thin films and implications for heterostructures journal April 2019
Simulation study on comprehensive sensing enhancement of BlueP/MoS 2 - and BlueP/WS 2 -based fluoride fiber surface plasmon resonance sensors: analysis founded on damping, field, and optical power journal January 2019
Manufacturing strategies for wafer-scale two-dimensional transition metal dichalcogenide heterolayers journal February 2020
Thin 2D: The New Dimensionality in Gas Sensing journal July 2017
Transport and Field Emission Properties of MoS2 Bilayers journal March 2018
Probing Interfacial Surface State Excitons in Nanoscale Synthesized Cu x S/MoS 2 Heterostructure journal January 2019
Hole Injection and Rectifying Heterojunction Photodiodes through Vacancy Engineering in MoS 2 journal April 2019
Recent advances in the nanoengineering of electrocatalysts for CO 2 reduction journal January 2018
Adsorption of gas molecules on a graphitic GaN sheet and its implications for molecule sensors journal January 2017
Advances of 2D bismuth in energy sciences journal January 2020
Highly concentrated and stabilizer-free transition-metal dichalcogenide dispersions in low-boiling point solvent for flexible electronics journal January 2019
Observation of charge transfer in mixed-dimensional heterostructures formed by transition metal dichalcogenide monolayers and PbS quantum dots journal December 2019
Nanoreinforcements of Two-Dimensional Nanomaterials for Flame Retardant Polymeric Composites: An Overview journal December 2019
Optical Properties and Photocarrier Dynamics of Bi 2 O 2 Se Monolayer and Nanoplates journal March 2020
Batch production of 6-inch uniform monolayer molybdenum disulfide catalyzed by sodium in glass journal March 2018
Electrostatically driven scalable synthesis of MoS 2 –graphene hybrid films assisted by hydrophobins journal January 2017
Wafer-recyclable, environment-friendly transfer printing for large-scale thin-film nanoelectronics journal July 2018
The Role of Graphene and Other 2D Materials in Solar Photovoltaics journal September 2018
Temperature‐induced phonon behavior in titanium disulfide (TiS 2 ) nanosheets journal May 2019
Centimeter-scale Green Integration of Layer-by-Layer 2D TMD vdW Heterostructures on Arbitrary Substrates by Water-Assisted Layer Transfer journal February 2019
CMOS-compatible batch processing of monolayer MoS 2 MOSFETs journal March 2018
Mobility and Decay Dynamics of Charge Carriers in One-Dimensional Selenium van der Waals Solid journal August 2017
Charge Mobility and Recombination Mechanisms in Tellurium van der Waals Solid journal December 2018
Probing Exfoliated Graphene Layers and Their Lithiation with Microfocused X-rays journal May 2019
Fabrication of Subnanometer-Precision Nanopores in Hexagonal Boron Nitride journal November 2017
Growth of ‘W’ doped molybdenum disulfide on graphene transferred molybdenum substrate journal May 2018
Review Article: Progress in fabrication of transition metal dichalcogenides heterostructure systems
  • Dong, Rui; Kuljanishvili, Irma
  • Journal of Vacuum Science & Technology B, Nanotechnology and Microelectronics: Materials, Processing, Measurement, and Phenomena, Vol. 35, Issue 3 https://doi.org/10.1116/1.4982736
journal May 2017
Feasible Route for a Large Area Few-Layer MoS2 with Magnetron Sputtering journal August 2018
Electronic and Optical Properties of Two-Dimensional Tellurene: From First-Principles Calculations journal July 2019

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