Tipping the magnetic instability in paramagnetic Sr3Ru2O7 by Fe impurities [Tipping the magnetic instability in paramagnetic Sr3Ru2O7 by modest Fe substitution]

Zhu, M.; Wang, Y.; Li, P. G.; Ge, J. J.; Tian, W.; Keavney, D.; Mao, Z. Q.; Ke, X.

doi:10.1103/PhysRevB.95.174430

Title: Tipping the magnetic instability in paramagnetic $S r_{3} R u_{2} O_{7}$ by Fe impurities [Tipping the magnetic instability in paramagnetic $S r_{3} R u_{2} O_{7}$ by modest Fe substitution]

Journal Article · Fri May 19 00:00:00 EDT 2017 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.95.174430· OSTI ID:1363902

Zhu, M. ^[1]; Wang, Y. ^[2]; Li, P. G. ^[2]; Ge, J. J. ^[2]; Tian, W. ^[3]; Keavney, D. ^[4]; Mao, Z. Q. ^[2]; Ke, X. ^[1]

Michigan State Univ., East Lansing, MI (United States)
Tulane Univ., New Orleans, LA (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)

We report the magnetic and electronic properties of the bilayer ruthenate Sr₃Ru₂O₇ upon Fe substitution for Ru. We find that Sr₃(Ru_1-xFe_x)₂O₇ shows spin-glass-like phase below 4 K for x = 0.01 and commensurate E-type antiferromagnetically ordered insulating ground state characterized by the propagation vector q_c = (0.25 0.25 0) for x ≥ 0.03, in contrast to the paramagnetic metallic state in the parent compound with strong spin fluctuations occurring at wave vectors q = (0.09 0 0) and (0.25 0 0). The observed antiferromagnetic ordering is quasitwo-dimensional with very short correlation length along the c axis, a feature similar to the Mndoped Sr₃Ru₂O₇. Lastly, our results suggest that this ordered ground state is associated with the intrinsic magnetic instability in the pristine compound, which can be readily tipped by the local magnetic coupling between the 3d orbitals of the magnetic dopants and Ru 4d orbitals.

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Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22), Experimental Program to Stimulate Competitive Research (EPSCoR); USDOE

Grant/Contract Number:: AC02-06CH11357; SC0012432

OSTI ID:: 1363902

Alternate ID(s):: OSTI ID: 1357936

Journal Information:: Physical Review B, Vol. 95, Issue 17; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 4 works

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Title: Tipping the magnetic instability in paramagnetic $S r_{3} R u_{2} O_{7}$ by Fe impurities [Tipping the magnetic instability in paramagnetic $S r_{3} R u_{2} O_{7}$ by modest Fe substitution]