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Title: Assessing theoretical uncertainties in fission barriers of superheavy nuclei

Journal Article · · Physical Review C
 [1];  [1];  [1];  [2]
  1. Mississippi State Univ., Mississippi State, MS (United States)
  2. Technische Univ. Munchen, Garching (Germany)

Here, theoretical uncertainties in the predictions of inner fission barrier heights in superheavy elements have been investigated in a systematic way for a set of state-of-the-art covariant energy density functionals which represent major classes of the functionals used in covariant density functional theory. They differ in basic model assumptions and fitting protocols. Both systematic and statistical uncertainties have been quantified where the former turn out to be larger. Systematic uncertainties are substantial in superheavy elements and their behavior as a function of proton and neutron numbers contains a large random component. The benchmarking of the functionals to the experimental data on fission barriers in the actinides allows to reduce the systematic theoretical uncertainties for the inner fission barriers of unknown superheavy elements. However, even then they on average increase on moving away from the region where benchmarking has been performed. In addition, a comparison with the results of non-relativistic approaches is performed in order to define full systematic theoretical uncertainties over the state-of-the-art models. Even for the models benchmarked in the actinides, the difference in the inner fission barrier height of some superheavy elements reaches $5-6$ MeV. This uncertainty in the fission barrier heights will translate into huge (many tens of the orders of magnitude) uncertainties in the spontaneous fission half-lives.

Research Organization:
Mississippi State Univ., Mississippi State, MS (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Nuclear Physics (NP)
Grant/Contract Number:
NA0002925; SC0013037
OSTI ID:
1356774
Alternate ID(s):
OSTI ID: 1359981
Journal Information:
Physical Review C, Vol. 95, Issue 5; ISSN 2469-9985
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 48 works
Citation information provided by
Web of Science

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Cited By (5)

Neck configuration of Cm and Cf nuclei in the fission state within the relativistic mean field formalism journal November 2019
Experimental survey of the production of α -decaying heavy elements in U 238 + Th 232 reactions at 7.5–6.1 MeV/nucleon journal June 2018
Decay properties and reaction dynamics of zirconium isotopes in the relativistic mean-field model journal February 2018
Ground state properties and shape evolution in Pt isotopes within the covariant density functional theory journal October 2019
Microscopic self-consistent description of induced fission dynamics: finite temperature effects text January 2018