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Title: Detection near 1-nm with a laminar-flow, water-based condensation particle counter

Journal Article · · Aerosol Science and Technology
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  1. Aerosol Dynamics Inc., Berkeley, CA (United States)
  2. Brookhaven National Lab. (BNL), Upton, NY (United States)
  3. Lisa Univ. Paris Est Creteil, Paris (France)

Presented is a laminar-flow, water-based condensation particle counter capable of particle detection near 1 nm. This instrument employs a three-stage, laminar-flow growth tube with a “moderator” stage that reduces the temperature and water content of the output flow without reducing the peak supersaturation, and makes feasible operation at the large temperature differences necessary for achieving high supersaturations. The instrument has an aerosol flow of 0.3 L/min, and does not use a filtered sheath flow. It is referred to as a “versatile” water condensation particle counter, or vWCPC, as operating temperatures can be adjusted in accordance with the cut-point desired. When operated with wall temperatures of ~2°C, >90°C, and ~22°C for the three stages, respectively, the vWCPC detects particles generated from a heated nichrome wire with a 50% efficiency cut-point near 1.6 nm mobility diameter. At these operating temperatures, it also detects 10–20% of large molecular ions formed from passing filtered ambient air through a bipolar ion source. Decreasing the temperature difference between the first two stages, with the first and second stages operated at 10 and 90°C, respectively, essentially eliminates the response to charger ions, and raises the 50% efficiency cut-point for the nichrome wire particles to 1.9 nm mobility diameter. Here, the time response, as measured by rapid removal of an inlet filter, yields a characteristic time constant of 195 ms.

Research Organization:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Biological and Environmental Research (BER)
Grant/Contract Number:
SC00112704
OSTI ID:
1350916
Report Number(s):
BNL-113749-2017-JA; R&D Project: 2016-BNL-EE630EECA-Budg; KP1701000
Journal Information:
Aerosol Science and Technology, Vol. 51, Issue 3; ISSN 0278-6826
Publisher:
American Association for Aerosol ResearchCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 34 works
Citation information provided by
Web of Science

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Cited By (7)

A diethylene glycol condensation particle counter for rapid sizing of sub-3 nm atmospheric clusters journal August 2018
B3010: a boosted TSI 3010 condensation particle counter for airborne studies journal January 2019
Laboratory and field evaluation of the Aerosol Dynamics Inc. concentrator (ADIc) for aerosol mass spectrometry journal January 2019
On the time response determination of condensation particle counters text January 2018
On the time response determination of condensation particle counters journal April 2018
Laboratory and field evaluation of the Aerosol Dynamics Inc. concentrator (ADIc) for aerosol mass spectrometry journal March 2019
On the time response determination of condensation particle counters text January 2018