Experimental determination of solubilities of di-calcium ethylenediaminetetraacetic acid hydrate [Ca2C10H12N2O8·7H2O(s)] in NaCl and MgCl2 solutions to high ionic strengths and its Pitzer model: Applications to geological disposal of nuclear waste and other low temperature environments

Xiong, Yongliang; Kirkes, Leslie; Westfall, Terry

doi:10.1016/j.chemgeo.2017.01.025

Title: Experimental determination of solubilities of di-calcium ethylenediaminetetraacetic acid hydrate [Ca2C10H12N2O8·7H2O(s)] in NaCl and MgCl2 solutions to high ionic strengths and its Pitzer model: Applications to geological disposal of nuclear waste and other low temperature environments

Journal Article · Sat Apr 01 00:00:00 EDT 2017 · Chemical Geology

DOI:https://doi.org/10.1016/j.chemgeo.2017.01.025· OSTI ID:1344455

Xiong, Yongliang; Kirkes, Leslie; Westfall, Terry

In this study, solubility measurements on di-calcium ethylenediaminetetraacetic acid [Ca₂C₁₀H₁₂N₂O₈(s), abbreviated as Ca₂EDTA(s)] as a function of ionic strength are conducted in NaCl solutions up to I = 5.0 mol•kg^–1 and in MgCl₂ solutions up to I = 7.5 mol•kg^–1, at room temperature (22.5 ± 0.5oC).

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Research Organization:: Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: AC04-94AL85000

OSTI ID:: 1344455

Alternate ID(s):: OSTI ID: 1344466; OSTI ID: 1397635

Report Number(s):: SAND2016-1275J; SAND-2016-1275J; 619421

Journal Information:: Chemical Geology, Vol. 454, Issue C; ISSN 0009-2541

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 5 works

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A Pitzer Model for Lead Oxide Solubilities in the Presence of Borate to High Ionic Strength Xiong, Yongliang; Kirkes, Leslie; Westfall, Terry Journal of Solution Chemistry, Vol. 47, Issue 12 https://doi.org/10.1007/s10953-018-0835-8	journal	November 2018

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Experimental Determination of Solubilities of Di-calcium Ethylenediaminetetraacetic Acid [Ca2C10H12N2O8(s)] in NaCl and MgCl2 Solutions to High Ionic Strengths and Its Pitzer Model: Applications to Geological Disposal of Nuclear Waste and O.

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Title: Experimental determination of solubilities of di-calcium ethylenediaminetetraacetic acid hydrate [Ca2C10H12N2O8·7H2O(s)] in NaCl and MgCl2 solutions to high ionic strengths and its Pitzer model: Applications to geological disposal of nuclear waste and other low temperature environments

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