Thin-film semiconductor perspective of organometal trihalide perovskite materials for high-efficiency solar cells

Xiao, Zhengguo; Yuan, Yongbo; Wang, Qi; Shao, Yuchuan; Bai, Yang; Deng, Yehao; Dong, Qingfeng; Hu, Miao; Bi, Cheng; Huang, Jinsong

doi:10.1016/j.mser.2015.12.002

Title: Thin-film semiconductor perspective of organometal trihalide perovskite materials for high-efficiency solar cells

Journal Article · Fri Feb 19 00:00:00 EST 2016 · Materials Science and Engineering. R, Reports

DOI:https://doi.org/10.1016/j.mser.2015.12.002· OSTI ID:1342525

Xiao, Zhengguo ^[1]; Yuan, Yongbo ^[1]; Wang, Qi ^[1]; Shao, Yuchuan ^[1]; Bai, Yang ^[1]; Deng, Yehao ^[1]; Dong, Qingfeng ^[1]; Hu, Miao ^[1]; Bi, Cheng ^[1]; Huang, Jinsong ^[1]

Univ. of Nebraska-Lincoln, Lincoln, NE (United States)

Here, organometal trihalide perovskites (OTPs) are arising as a new generation of low-cost active materials for solar cells with efficiency rocketing from 3.5% to over 20% within only five years. From “dye” in dye-sensitized solar cells (DSSCs) to “hole conductors” and “electron conductors” in mesoscopic heterojunction solar cells, there has been a dramatic conceptual evolution on the function of OTPs in photovoltaic devices. OTPs were originally used as dyes in Grätzel cells, achieving a high efficiency above 15% which, however, did not manifest the excellent charge transport properties of OTPs. An analogy of OTPs to traditional semiconductors was drawn after the demonstration of highly efficient planar heterojunction structure OTP devices and the observation of their excellent bipolar transport properties with a large diffusion length exceeding 100 nm in CH₃NH₃PbI₃ (MAPbI₃) polycrystalline thin films. This review aims to provide the most recent advances in the understanding of the origin of the high OTP device efficiency. Specifically, we will focus on reviewing the progress in understanding (1) the characterization of fantastic optoelectronic property of OTPs, (2) the unusual defect physics that originate the optoelectronic property, (3) morphology control of the perovskite film from fabrication process and film post-treatment, (4) device interface and charge transport layers that dramatically impact device efficiency in the OTP thin-film devices, (5) photocurrent hysteresis, (6) tandem solar cells and (7) stability of the perovskite materials and solar cell devices.

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Research Organization:: Univ. of Nebraska, Lincoln, NE (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE)

Grant/Contract Number:: EE0006709

OSTI ID:: 1342525

Alternate ID(s):: OSTI ID: 1342750; OSTI ID: 1359596

Journal Information:: Materials Science and Engineering. R, Reports, Vol. 101, Issue C; ISSN 0927-796X

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 107 works

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Top Laminated Graphene Electrode in a Semitransparent Polymer Solar Cell by Simultaneous Thermal Annealing/Releasing Method Lee, Yu-Ying; Tu, Kun-Hua; Yu, Chen-Chieh ACS Nano, Vol. 5, Issue 8 https://doi.org/10.1021/nn201940j	journal	July 2011
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High efficiency single-junction semitransparent perovskite solar cells Roldán-Carmona, Cristina; Malinkiewicz, Olga; Betancur, Rafael Energy Environ. Sci., Vol. 7, Issue 9 https://doi.org/10.1039/C4EE01389A	journal	January 2014
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Multilayer Transparent Top Electrode for Solution Processed Perovskite/Cu(In,Ga)(Se,S) ₂ Four Terminal Tandem Solar Cells Yang, Yang (Michael); Chen, Qi; Hsieh, Yao-Tsung ACS Nano, Vol. 9, Issue 7 https://doi.org/10.1021/acsnano.5b03189	journal	June 2015
High-performance semitransparent perovskite solar cells with solution-processed silver nanowires as top electrodes Guo, Fei; Azimi, Hamed; Hou, Yi Nanoscale, Vol. 7, Issue 5 https://doi.org/10.1039/C4NR06033D	journal	January 2015
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A Layered Hybrid Perovskite Solar-Cell Absorber with Enhanced Moisture Stability Smith, Ian C.; Hoke, Eric T.; Solis-Ibarra, Diego Angewandte Chemie, Vol. 126, Issue 42 https://doi.org/10.1002/ange.201406466	journal	September 2014
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Stabilization of the Trigonal High-Temperature Phase of Formamidinium Lead Iodide Binek, Andreas; Hanusch, Fabian C.; Docampo, Pablo The Journal of Physical Chemistry Letters, Vol. 6, Issue 7 https://doi.org/10.1021/acs.jpclett.5b00380	journal	March 2015
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Polaronic transport in CH3NH3PbI3 single crystals Jin, Lei; Qian, Yuqin; Zhang, Yipei Journal of Materials Science: Materials in Electronics, Vol. 31, Issue 3 https://doi.org/10.1007/s10854-019-02713-y	journal	December 2019
Composition-Dependent Degradation of Hybrid and Inorganic Lead Perovskites in Ambient Conditions Calisi, Nicola; Caporali, Stefano; Milanesi, Alessio Topics in Catalysis, Vol. 61, Issue 9-11 https://doi.org/10.1007/s11244-018-0922-5	journal	April 2018
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Argon Plasma Treatment to Tune Perovskite Surface Composition for High Efficiency Solar Cells and Fast Photodetectors Y., Fang,; X., Xiao,; Y., Gao, The University of North Carolina at Chapel Hill University Libraries https://doi.org/10.17615/8gyw-8442	text	January 2018
Thin single crystal perovskite solar cells to harvest below-bandgap light absorption Shi, Tang,; Yehao, Deng,; Xun, Xiao, The University of North Carolina at Chapel Hill University Libraries https://doi.org/10.17615/fs7k-w655	text	January 2017
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