Emergent ferromagnetism and T-linear scattering in USb2 at high pressure [Emergent ferromagnetism in USb2 under pressure]

Jeffries, Jason R.; Stillwell, Ryan L.; Weir, Samuel T.; Vohra, Yogesh K.; Butch, Nicholas P.

doi:10.1103/PhysRevB.93.184406

Title: Emergent ferromagnetism and $T$ -linear scattering in $USb_{2}$ at high pressure [Emergent ferromagnetism in USb₂ under pressure]

Journal Article · Mon May 09 00:00:00 EDT 2016 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.93.184406· OSTI ID:1342040

Jeffries, Jason R. ^[1]; Stillwell, Ryan L. ^[1]; Weir, Samuel T. ^[1]; Vohra, Yogesh K. ^[2]; Butch, Nicholas P. ^[3]

Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Univ. of Alabama, Birmingham, AL (United States)
National Institute of Standards and Technology, Gaithersburg, MD (United States)

The material USb₂ is a correlated, moderately heavy-electron compound within the uranium dipnictide (UX₂) series. It is antiferromagnetic with a relatively high transition temperature T_N = 204K and a large U-U separation. While the uranium atoms in the lighter dipnictides are considered to be localized, those of USb₂ exhibit hybridization and itineracy, promoting uncertainty as to the continuity of the magnetic order within the UX₂. We have explored the evolution of the magnetic order by employing magnetotransport measurements as a function of pressure and temperature. We find that the T_N in USb₂ is enhanced, moving towards that of its smaller sibling UAs₂. But, long before reaching a T_N as high as UAs₂, the antiferromagnetism of USb₂ is abruptly destroyed in favor of another magnetic ground state. We identify this pressure-induced ground state as being ferromagnetic based on the appearance of a strong anomalous Hall effect in the transverse resistance in magnetic field. At last with pressure, this emergent ferromagnetic state is suppressed and ultimately destroyed in favor of a non-Fermi-liquid ground state.

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Research Organization:: Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: AC52-07NA27344; 14-ERD-041; NA0002014

OSTI ID:: 1342040

Alternate ID(s):: OSTI ID: 1252120

Report Number(s):: LLNL-JRNL-681439; PRBMDO

Journal Information:: Physical Review B, Vol. 93, Issue 18; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 18 works

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High temperature singlet-based magnetism from Hund’s rule correlations Miao, Lin; Basak, Rourav; Ran, Sheng Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-08497-3	journal	February 2019
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Orbital-selective Kondo-lattice and enigmatic f-electrons emerging from inside the antiferromagnetic phase of a heavy fermion Giannakis, Ioannis; Leshen, Justin; Kavai, Mariam arXiv https://doi.org/10.48550/arxiv.1906.01742	text	January 2019
High temperature singlet-based magnetism from Hund's rule correlations Miao, Lin; Basak, Rourav; Ran, Sheng arXiv https://doi.org/10.48550/arxiv.1906.09474	text	January 2019

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Title: Emergent ferromagnetism and $T$ -linear scattering in $USb_{2}$ at high pressure [Emergent ferromagnetism in USb₂ under pressure]