A metastable liquid melted from a crystalline solid under decompression

doi:10.1038/ncomms14260

Title: A metastable liquid melted from a crystalline solid under decompression

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Authors:

Lin, Chuanlong; Smith, Jesse S.; Sinogeikin, Stanislav V.; Kono, Yoshio; ; Kenney-Benson, Curtis; Shen, Guoyin

Publication Date:: Mon Jan 23 00:00:00 EST 2017

Research Org.:: Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source (APS)

Sponsoring Org.:: DOE - BASIC ENERGY SCIENCES

OSTI Identifier:: 1340711

Resource Type:: Journal Article

Resource Relation:: Journal Name: Nature Communications; Journal Volume: 8; Journal Issue: 01, 2017

Country of Publication:: United States

Language:: ENGLISH

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                    Lin, Chuanlong, Smith, Jesse S., Sinogeikin, Stanislav V., Kono, Yoshio, Park, Changyong, Kenney-Benson, Curtis, and Shen, Guoyin. A metastable liquid melted from a crystalline solid under decompression.  United States: N. p., 2017. 
        Web.  doi:10.1038/ncomms14260.

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                    Lin, Chuanlong, Smith, Jesse S., Sinogeikin, Stanislav V., Kono, Yoshio, Park, Changyong, Kenney-Benson, Curtis, & Shen, Guoyin. A metastable liquid melted from a crystalline solid under decompression.  United States.  doi:10.1038/ncomms14260.

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                    Lin, Chuanlong, Smith, Jesse S., Sinogeikin, Stanislav V., Kono, Yoshio, Park, Changyong, Kenney-Benson, Curtis, and Shen, Guoyin. Mon .  
        "A metastable liquid melted from a crystalline solid under decompression".  United States.  
        doi:10.1038/ncomms14260.

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@article{osti_1340711,

  title        = {A metastable liquid melted from a crystalline solid under decompression},

  author       = {Lin, Chuanlong and Smith, Jesse S. and Sinogeikin, Stanislav V. and Kono, Yoshio and Park, Changyong and Kenney-Benson, Curtis and Shen, Guoyin},

  abstractNote = {},

  doi          = {10.1038/ncomms14260},

  journal      = {Nature Communications},

  number       = 01, 2017,

  volume       = 8,

  place        = {United States},

  year         = {Mon Jan 23 00:00:00 EST 2017},

  month        = {Mon Jan 23 00:00:00 EST 2017}

}

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Journal Article:

DOI: 10.1038/ncomms14260

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A metastable liquid melted from a crystalline solid under decompression

Lin, Chuanlong ; Smith, Jesse S. ; Sinogeikin, Stanislav V. ; ... - Nature Communications

A metastable liquid may exist under supercooling, sustaining the liquid below the melting point such as supercooled water and silicon. It may also exist as a transient state in solid–solid transitions, as demonstrated in recent studies of colloidal particles and glass-forming metallic systems. One important question is whether a crystalline solid may directly melt into a sustainable metastable liquid. By thermal heating, a crystalline solid will always melt into a liquid above the melting point. Here we report that a high-pressure crystalline phase of bismuth can melt into a metastable liquid below the melting line through a decompression process. Themore »« less
Cited by 5
DOI: 10.1038/ncomms14260

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Production of city gas from solid and liquid fuels. [Study of gasification of coal under pressure and combination with gasification of liquid hydrocarbons or with carburetion of H-rich gas from natural gas] (in Czech)

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Solution-liquid-solid growth of crystalline III-V semiconductors: An anology to vapor-liquid-solid growth

Trentler, T.J. ; Hickman, K.M. ; Goel, S.C. - Science

Until now, micrometer-scale or larger crystals of the III-V semiconductors have not been grown at low temperatures for lack of suitable crystallization mechanisms for highly covalent nonmolecular solids. A solution-liquid-solid mechanism for the growth of InP, InAs, and GaAs is described that uses simple, low-temperature ({le}203{degrees}C), solution-phase reactions. The materials are produced as polycrystalline fibers or near-single-crystal whiskers having widths of 10 to 150 nanometers and lengths of up to several micrometers. This mechanism shows that processes analogous to vapor-liquid-solid growth can operate at low temperatures; similar synthesis routes for other covalent solids may be possible. 26 refs., 7 figs.
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Metastable zirconia phases prepared from zirconium alkoxide and yttrium acetylacetonate: Part 1--Formation and characterization of metastable zirconia solid solutions

Shimazaki, M. ; Hirota, K. ; Yamaguchi, O. ; ... - Materials Research Bulletin; (United States)

In the ZrO[sub 2]-Y[sub 2]O[sub 3] system, metastable ZrO[sub 2] solid solutions containing up to [approximately]46 mol% Y[sub 2]O[sub 3] crystallize at low temperatures from amorphous materials prepared by the simultaneous hydrolysis of zirconium isopropoxide and yttrium acetylacetonate: t- and c-ZrO[sub 2] phases below and above 8 mol% Y[sub 2]O[sub 3], respectively. The variation of the lattice parameters of both phases is determined as a function of Y[sub 2]O[sub 3] content. The value of the lattice parameter of pure ZrO[sub 2] (tetragonal) is a = 0.5085 nm and c = 0.5170 nm. Powder characterization has been examined using c-ZrO[sub 2]more »« less
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