Laser fluence dependence on emission dynamics of ultrafast laser induced copper plasma
Abstract
The characteristic emission features of a laser-produced plasma strongly depend strongly on the laser fluence. We investigated the spatial and temporal dynamics of neutrals and ions in femtosecond laser (800 nm, ~40 fs, Ti:Sapphire) induced copper plasma in vacuum using both optical emission spectroscopy (OES) and spectrally resolved two-dimensional (2D) imaging methods over a wide fluence range of 0.5-77.5 J/cm2. 2D fast gated monochromatic images showed distinct plume splitting between the neutral and ions especially at moderate to higher fluence ranges. OES studies at low to moderate laser fluence regime confirm intense neutral line emission over the ion emission whereas this trend changes at higher laser fluence with dominance of the latter. This evidences a clear change in the physical processes involved in femtosecond laser matter interaction at high input laser intensity. Furthermore, the obtained ion dynamics resulting from the OES, and spectrally resolved 2D imaging are compared with charged particle measurement employing Faraday cup and Langmuir probe and results showed good correlation.
- Authors:
-
- Raman Research Institute, Bangalore (India); Complessoe Univ. Monte S. Angelo, Napoli (Italy)
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Purdue Univ., West Lafayette, IN (United States)
- Raman Research Institute, Bangalore (India)
- Complessoe Univ. Monte S. Angelo, Napoli (Italy)
- Publication Date:
- Research Org.:
- Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1339811
- Report Number(s):
- PNNL-SA-119809
Journal ID: ISSN 0021-8979; DN2001000
- Grant/Contract Number:
- AC05-76RL01830
- Resource Type:
- Journal Article: Accepted Manuscript
- Journal Name:
- Journal of Applied Physics
- Additional Journal Information:
- Journal Volume: 120; Journal Issue: 18; Journal ID: ISSN 0021-8979
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 70 PLASMA PHYSICS AND FUSION TECHNOLOGY; laser ablation (LA); Laser-produced plasma
Citation Formats
Anoop, K. K., Harilal, S. S., Philip, Reji, Bruzzese, R., and Amoruso, S. Laser fluence dependence on emission dynamics of ultrafast laser induced copper plasma. United States: N. p., 2016.
Web. doi:10.1063/1.4967313.
Anoop, K. K., Harilal, S. S., Philip, Reji, Bruzzese, R., & Amoruso, S. Laser fluence dependence on emission dynamics of ultrafast laser induced copper plasma. United States. https://doi.org/10.1063/1.4967313
Anoop, K. K., Harilal, S. S., Philip, Reji, Bruzzese, R., and Amoruso, S. 2016.
"Laser fluence dependence on emission dynamics of ultrafast laser induced copper plasma". United States. https://doi.org/10.1063/1.4967313. https://www.osti.gov/servlets/purl/1339811.
@article{osti_1339811,
title = {Laser fluence dependence on emission dynamics of ultrafast laser induced copper plasma},
author = {Anoop, K. K. and Harilal, S. S. and Philip, Reji and Bruzzese, R. and Amoruso, S.},
abstractNote = {The characteristic emission features of a laser-produced plasma strongly depend strongly on the laser fluence. We investigated the spatial and temporal dynamics of neutrals and ions in femtosecond laser (800 nm, ~40 fs, Ti:Sapphire) induced copper plasma in vacuum using both optical emission spectroscopy (OES) and spectrally resolved two-dimensional (2D) imaging methods over a wide fluence range of 0.5-77.5 J/cm2. 2D fast gated monochromatic images showed distinct plume splitting between the neutral and ions especially at moderate to higher fluence ranges. OES studies at low to moderate laser fluence regime confirm intense neutral line emission over the ion emission whereas this trend changes at higher laser fluence with dominance of the latter. This evidences a clear change in the physical processes involved in femtosecond laser matter interaction at high input laser intensity. Furthermore, the obtained ion dynamics resulting from the OES, and spectrally resolved 2D imaging are compared with charged particle measurement employing Faraday cup and Langmuir probe and results showed good correlation.},
doi = {10.1063/1.4967313},
url = {https://www.osti.gov/biblio/1339811},
journal = {Journal of Applied Physics},
issn = {0021-8979},
number = 18,
volume = 120,
place = {United States},
year = {Tue Nov 08 00:00:00 EST 2016},
month = {Tue Nov 08 00:00:00 EST 2016}
}
Web of Science
Works referenced in this record:
Stark broadening calculations of neutral copper spectral lines and temperature dependence
journal, October 2010
- Zmerli, B.; Ben Nessib, N.; Dimitrijević, M. S.
- Physica Scripta, Vol. 82, Issue 5
Experimental Identification of “Vacuum Heating” at Femtosecond-Laser-Irradiated Metal Surfaces
journal, May 1999
- Grimes, M. K.; Rundquist, A. R.; Lee, Y. -S.
- Physical Review Letters, Vol. 82, Issue 20
Dynamics of molecular emission features from nanosecond, femtosecond laser and filament ablation plasmas
journal, January 2016
- Harilal, S. S.; Yeak, J.; Brumfield, B. E.
- Journal of Analytical Atomic Spectrometry, Vol. 31, Issue 6
High-order harmonic generation in a laser plasma: a review of recent achievements
journal, October 2007
- Ganeev, R. A.
- Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 40, Issue 22
Resistivity of a Simple Metal from Room Temperature to K
journal, November 1988
- Milchberg, H. M.; Freeman, R. R.; Davey, S. C.
- Physical Review Letters, Vol. 61, Issue 20
Ablation of solids by femtosecond lasers: Ablation mechanism and ablation thresholds for metals and dielectrics
journal, March 2002
- Gamaly, E. G.; Rode, A. V.; Luther-Davies, B.
- Physics of Plasmas, Vol. 9, Issue 3
Microscopic and macroscopic modeling of femtosecond laser ablation of metals
journal, December 2015
- Povarnitsyn, Mikhail E.; Fokin, Vladimir B.; Levashov, Pavel R.
- Applied Surface Science, Vol. 357
Femtosecond laser ablation of silicon–modification thresholds and morphology
journal, January 2002
- Bonse, J.; Baudach, S.; Krüger, J.
- Applied Physics A, Vol. 74, Issue 1
Femtosecond laser ablation of aluminum in vacuum and air at high laser intensity
journal, October 2013
- Zhao, Xin; Shin, Yung C.
- Applied Surface Science, Vol. 283
Ultra-short pulse laser ablation of metals: threshold fluence, incubation coefficient and ablation rates
journal, May 2010
- Byskov-Nielsen, Jeppe; Savolainen, Juha-Matti; Christensen, Martin Snogdahl
- Applied Physics A, Vol. 101, Issue 1
Laser-induced plasma temperature
journal, July 2014
- Zhang, Shudi; Wang, Xiaohua; He, Miaohong
- Spectrochimica Acta Part B: Atomic Spectroscopy, Vol. 97
Laser ablation and micromachining with ultrashort laser pulses
journal, January 1997
- Liu, X.; Du, D.; Mourou, G.
- IEEE Journal of Quantum Electronics, Vol. 33, Issue 10
Shock Wave Mediated Plume Chemistry for Molecular Formation in Laser Ablation Plasmas
journal, January 2016
- Harilal, Sivanandan S.; Brumfield, Brian E.; Cannon, Bret D.
- Analytical Chemistry, Vol. 88, Issue 4
Femtosecond, picosecond, and nanosecond laser microablation: laser plasma and crater investigation
conference, April 2001
- Semerok, Alexandre F.; Salle, Beatrice; Lacour, Jean-Luc
- 26th European Conference on Laser Interaction with Matter (ECLIM 2000), SPIE Proceedings
Experimental and theoretical study of Al plasma under femtosecond laser pulses
journal, May 2009
- Komarov, P. S.; Ashitkov, S. I.; Ovchinnikov, A. V.
- Journal of Physics A: Mathematical and Theoretical, Vol. 42, Issue 21
Femtosecond laser pulse irradiation of solid targets as a general route to nanoparticle formation in a vacuum
journal, January 2005
- Amoruso, S.; Ausanio, G.; Bruzzese, R.
- Physical Review B, Vol. 71, Issue 3, Article No. 033406
Femtosecond Laser-Induced Breakdown Spectroscopy: Physics, Applications, and Perspectives
journal, October 2007
- Gurevich, E. L.; Hergenröder, R.
- Applied Spectroscopy, Vol. 61, Issue 10
Dynamics of Plume Propagation and Splitting during Pulsed-Laser Ablation
journal, August 1997
- Wood, R. F.; Chen, K. R.; Leboeuf, J. N.
- Physical Review Letters, Vol. 79, Issue 8
Molecular-dynamics study of ablation of solids under femtosecond laser pulses
journal, May 2003
- Perez, Danny; Lewis, Laurent J.
- Physical Review B, Vol. 67, Issue 18
Structure formation on the surface of indium phosphide irradiated by femtosecond laser pulses
journal, January 2005
- Bonse, J.; Munz, M.; Sturm, H.
- Journal of Applied Physics, Vol. 97, Issue 1
Ultrashort laser ablation of bulk copper targets: Dynamics and size distribution of the generated nanoparticles
journal, June 2014
- Tsakiris, N.; Anoop, K. K.; Ausanio, G.
- Journal of Applied Physics, Vol. 115, Issue 24
Hot electron generation via vacuum heating process in femtosecond laser–solid interactions
journal, June 2001
- Chen, L. M.; Zhang, J.; Dong, Q. L.
- Physics of Plasmas, Vol. 8, Issue 6
Consequences of femtosecond laser filament generation conditions in standoff laser induced breakdown spectroscopy
journal, January 2016
- Harilal, S. S.; Yeak, J.; Brumfield, B. E.
- Optics Express, Vol. 24, Issue 16
Selected problems of laser ablation theory
journal, March 2002
- Anisimov, Sergei I.; Luk'yanchuk, B. S.
- Physics-Uspekhi, Vol. 45, Issue 3
Multidiagnostic analysis of ion dynamics in ultrafast laser ablation of metals over a large fluence range
journal, February 2015
- Anoop, K. K.; Polek, M. P.; Bruzzese, R.
- Journal of Applied Physics, Vol. 117, Issue 8
Convoluted effect of laser fluence and pulse duration on the property of a nanosecond laser-induced plasma into an argon ambient gas at the atmospheric pressure
journal, January 2013
- Bai, Xueshi; Ma, Qianli; Motto-Ros, Vincent
- Journal of Applied Physics, Vol. 113, Issue 1
Morphological changes in ultrafast laser ablation plumes with varying spot size
journal, January 2015
- Harilal, S. S.; Diwakar, P. K.; Polek, M. P.
- Optics Express, Vol. 23, Issue 12
Multi-diagnostic comparison of femtosecond and nanosecond pulsed laser plasmas
journal, September 2002
- Zhang, Z.; VanRompay, P. A.; Nees, J. A.
- Journal of Applied Physics, Vol. 92, Issue 5
Temporally and spectrally resolved analysis of a copper plasma plume produced by ultrafast laser ablation
journal, March 2009
- Wang, X.; Amoruso, S.; Xia, J.
- Applied Surface Science, Vol. 255, Issue 10
Hydrodynamic simulations of metal ablation by femtosecond laser irradiation
journal, April 2005
- Colombier, J. P.; Combis, P.; Bonneau, F.
- Physical Review B, Vol. 71, Issue 16
Femtosecond laser ablation properties of borosilicate glass
journal, November 2004
- Ben-Yakar, Adela; Byer, Robert L.
- Journal of Applied Physics, Vol. 96, Issue 9
Ablation thresholds of metals with femtosecond laser pulses
conference, June 2001
- Hashida, Masaki; Semerok, Alexandre F.; Gobert, Olivier
- Nonresonant Laser-Matter Interaction (NLMI-10), SPIE Proceedings
A review of ultrashort pulsed laser ablation of materials
journal, February 1998
- Shirk, M. D.; Molian, P. A.
- Journal of Laser Applications, Vol. 10, Issue 1
Femtosecond laser surface structuring of silicon using optical vortex beams generated by a q-plate
journal, June 2014
- Anoop, K. K.; Rubano, A.; Fittipaldi, R.
- Applied Physics Letters, Vol. 104, Issue 24
Femtosecond laser ablation of copper at high laser fluence: Modeling and experimental comparison
journal, January 2016
- Cheng, C. W.; Wang, S. Y.; Chang, K. P.
- Applied Surface Science, Vol. 361
Ultrafast (femtosecond) laser refractive surgery
journal, January 2002
- Sugar, Alan
- Current Opinion in Ophthalmology, Vol. 13, Issue 4
Superhydrophobic Surfaces Prepared by Microstructuring of Silicon Using a Femtosecond Laser
journal, May 2006
- Baldacchini, Tommaso; Carey, James E.; Zhou, Ming
- Langmuir, Vol. 22, Issue 11
Spectral Evidence for Collisionless Absorption in Subpicosecond Laser-Solid Interactions
journal, December 1999
- Hansen, C. T.; Wilks, S. C.; Young, P. E.
- Physical Review Letters, Vol. 83, Issue 24
Femtosecond laser ablation ICP-MS
journal, January 2002
- Russo, Richard E.; Mao, Xianglei; Gonzalez, Jhanis J.
- J. Anal. At. Spectrom., Vol. 17, Issue 9
The interaction of femtosecond and nanosecond laser pulses with the surface of glass
journal, May 2003
- Kasaai, Mohammad R.; Kacham, Vijayalakshmi; Theberge, Francis
- Journal of Non-Crystalline Solids, Vol. 319, Issue 1-2
Fast ion generation in femtosecond laser ablation of a metallic target at moderate laser intensity
journal, August 2014
- Anoop, K. K.; Ni, Xiaochang; Wang, Xuan
- Laser Physics, Vol. 24, Issue 10
Double-peak distribution of electron and ion emission profile during femtosecond laser ablation of metals
journal, January 2002
- Amoruso, S.; Wang, X.; Altucci, C.
- Applied Surface Science, Vol. 186, Issue 1-4
Simple technique for measurements of pulsed Gaussian-beam spot sizes
journal, January 1982
- Liu, J. M.
- Optics Letters, Vol. 7, Issue 5
Ion emission from a metal surface through a multiphoton process and optical field ionization
journal, March 2010
- Hashida, Masaki; Namba, Shin; Okamuro, Kiminori
- Physical Review B, Vol. 81, Issue 11
Two-dimensional imaging of atomic and nanoparticle components in copper plasma plume produced by ultrafast laser ablation
journal, January 2014
- Anoop, K. K.; Ni, Xiaochang; Bianco, M.
- Applied Physics A, Vol. 117, Issue 1
Spectroscopic Imaging of Laser-Induced Plasma
journal, January 1996
- Bulatov, Valery; Xu, Liang; Schechter, Israel
- Analytical Chemistry, Vol. 68, Issue 17
Direct femtosecond laser surface nano/microstructuring and its applications: Direct femtosecond laser surface nano/microstructuring and its applications
journal, August 2012
- Vorobyev, Anatoliy Y.; Guo, Chunlei
- Laser & Photonics Reviews, Vol. 7, Issue 3
Works referencing / citing this record:
A compact non-differential approach for modeling laser ablation plasma dynamics
journal, February 2017
- Irimiciuc, S. A.; Gurlui, S.; Nica, P.
- Journal of Applied Physics, Vol. 121, Issue 8
Investigation of femtosecond laser-produced plasma from various metallic targets using the Langmuir probe characteristic
journal, October 2017
- Nica, P.; Gurlui, S.; Osiac, M.
- Physics of Plasmas, Vol. 24, Issue 10
Pulse width dependent dynamics of laser-induced plasma from a Ni thin film
journal, February 2019
- Thomas, Jinto; Joshi, Hem Chandra; Kumar, Ajai
- Journal of Physics D: Applied Physics, Vol. 52, Issue 13
Progress of laser-induced breakdown spectroscopy in nuclear industry applications
journal, October 2019
- Wu, Jian; Qiu, Yan; Li, Xingwen
- Journal of Physics D: Applied Physics, Vol. 53, Issue 2
Ultrafast dynamics observation during femtosecond laser-material interaction
journal, September 2019
- Guo, Baoshan; Sun, Jingya; Lu, YongFeng
- International Journal of Extreme Manufacturing, Vol. 1, Issue 3
Ge-Sb-Te Chalcogenide Thin Films Deposited by Nanosecond, Picosecond, and Femtosecond Laser Ablation
journal, May 2019
- Bulai, Georgiana; Pompilian, Oana; Gurlui, Silviu
- Nanomaterials, Vol. 9, Issue 5
Structure-Mediated Excitation of Air Plasma and Silicon Plasma Expansion in Femtosecond Laser Pulses Ablation
journal, January 2018
- Wang, Qingsong; Jiang, Lan; Sun, Jingya
- Research, Vol. 2018
Ge-Sb-Te Chalcogenide Thin Films Deposited by Nanosecond, Picosecond, and Femtosecond Laser Ablation
journal, May 2019
- Bulai, Georgiana; Pompilian, Oana; Gurlui, Silviu
- Nanomaterials, Vol. 9, Issue 5