Energy dissipation from a correlated system driven out of equilibrium

Rameau, J. D.; Freutel, S.; Kemper, A. F.; Sentef, M. A.; Freericks, J. K.; Avigo, I.; Ligges, M.; Rettig, L.; Yoshida, Y.; Eisaki, H.; Schneeloch, J.; Zhong, R. D.; Xu, Z. J.; Gu, G. D.; Johnson, P. D.; Bovensiepen, U.

doi:10.1038/ncomms13761

Title: Energy dissipation from a correlated system driven out of equilibrium

Journal Article · Tue Dec 20 00:00:00 EST 2016 · Nature Communications

DOI:https://doi.org/10.1038/ncomms13761· OSTI ID:1338600

Rameau, J. D. ^[1]; Freutel, S. ^[2]; Kemper, A. F. ^[3]; Sentef, M. A. ^[4]; Freericks, J. K. ^[5]; Avigo, I. ^[2]; Ligges, M. ^[2]; Rettig, L. ^[2]; Yoshida, Y. ^[6]; Eisaki, H. ^[6]; Schneeloch, J. ^[1]; Zhong, R. D. ^[1]; Xu, Z. J. ^[1]; Gu, G. D. ^[1]; Johnson, P. D. ^[1];

^[2]

Brookhaven National Lab. (BNL), Upton, NY (United States)
Univ. Duisburg-Essen, Duisburg (Germany). Faculty of Physics and Center for Nanointegration Duisburg-Essen
North Carolina State Univ., Raleigh, NC (United States). Dept. of Physics; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Univ. of Bonn (Germany). Helmholtz Inst. for Radiation and Nuclear Physics (HISKP); Max Planck Inst. for the Structure and Dynamics of Matter, Hamburg (Germany). Center for Free Electron Laser Science
Georgetown Univ., Washington, DC (United States)
National Inst. of Advanced Industrial Science and Technology, Tsukuba (Japan)

In complex materials various interactions have important roles in determining electronic properties. Angle-resolved photoelectron spectroscopy (ARPES) is used to study these processes by resolving the complex single-particle self-energy and quantifying how quantum interactions modify bare electronic states. However, ambiguities in the measurement of the real part of the self-energy and an intrinsic inability to disentangle various contributions to the imaginary part of the self-energy can leave the implications of such measurements open to debate. Here we employ a combined theoretical and experimental treatment of femtosecond time-resolved ARPES (tr-ARPES) show how population dynamics measured using tr-ARPES can be used to separate electron-boson interactions from electron-electron interactions. We demonstrate a quantitative analysis of a well-defined electron-boson interaction in the unoccupied spectrum of the cuprate Bi 2 Sr 2 CaCu 2 O 8+x characterized by an excited population decay time that maps directly to a discrete component of the equilibrium self-energy not readily isolated by static ARPES experiments.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States); Energy Frontier Research Centers (EFRC) (United States). Center for Emergent Superconductivity (CES); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); European Union (EU)

Grant/Contract Number:: SC0012704; AC02-05CH11231; FG02-08ER46542; PR-2011-0003; 2009-BNL-PM015; 280555

OSTI ID:: 1338600

Alternate ID(s):: OSTI ID: 1411564

Report Number(s):: BNL-113262-2016-JA; R&D Project: PO016; PO010; KC0202020; KC0201060

Journal Information:: Nature Communications, Vol. 7; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 54 works

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