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Title: Expansion of the tetragonal magnetic phase with pressure in the iron arsenide superconductor Ba 1 - x K x Fe 2 As 2

Journal Article · · Physical Review B
 [1];  [1];  [1];  [1];  [1];  [1];  [1];  [2];  [2];  [3];  [4];  [5];  [1];  [6]
  1. Univ. de Sherbrooke, Sherbrooke, QC (Canada)
  2. Ames Lab., Ames, IA (United States)
  3. Ames Lab., Ames, IA (United States); Iowa State Univ., Ames, IA (United States)
  4. Nanjing Univ., Nanjing (China)
  5. Nanjing Univ., Nanjing (China); Canadian Institute for Advanced Research, Toronto, ON (Canada)
  6. Univ. de Sherbrooke, Sherbrooke, QC (Canada); Canadian Institute for Advanced Research, Toronto, ON (Canada)

In the temperature-concentration phase diagram of most iron-based superconductors, antiferromagnetic order is gradually suppressed to zero at a critical point, and a dome of superconductivity forms around that point. The nature of the magnetic phase and its fluctuations is of fundamental importance for elucidating the pairing mechanism. In Ba1–xKxFe2As2 and Ba1–xNaxFe2As2, it has recently become clear that the usual stripelike magnetic phase, of orthorhombic symmetry, gives way to a second magnetic phase, of tetragonal symmetry, near the critical point, in the range from x = 0.24 to x = 0.28 for Ba1–xKxFe2As2. In a prior study, an unidentified phase was discovered for x < 0.24 but under applied pressure, whose onset was detected as a sharp anomaly in the resistivity. Here we report measurements of the electrical resistivity of Ba1–xKxFe2As2 under applied hydrostatic pressures up to 2.75 GPa, for x = 0.22, 0.24, and 0.28. The critical pressure above which the unidentified phase appears is seen to decrease with increasing x and vanish at x = 0.24, thereby linking the pressure-induced phase to the tetragonal magnetic phase observed at ambient pressure. In the temperature-concentration phase diagram of Ba1–xKxFe2As2, we find that pressure greatly expands the tetragonal magnetic phase, while the stripelike phase shrinks. As a result, this reveals that pressure may be a powerful tuning parameter with which to explore the interplay between magnetism and superconductivity in this material.

Research Organization:
Ames Lab., Ames, IA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-07CH11358; 2011CBA00100
OSTI ID:
1337668
Alternate ID(s):
OSTI ID: 1245047
Report Number(s):
IS-J-8986; PRBMDO
Journal Information:
Physical Review B, Vol. 93, Issue 14; ISSN 2469-9950
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 19 works
Citation information provided by
Web of Science

References (27)

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Spin reorientation in Ba 0.65 Na 0.35 Fe 2 As 2 studied by single-crystal neutron diffraction journal February 2015
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Cited By (6)

Hedgehog spin-vortex crystal stabilized in a hole-doped iron-based superconductor journal February 2018
Strain tuning and anisotropic spin correlations in iron-based systems journal August 2019
Optical and photoemission investigation of structural and magnetic transitions in the iron-based superconductor Sr 0.67 Na 0.33 Fe 2 As 2 journal December 2019
Preferred Magnetic Excitations in the Iron-Based Sr 1 x Na x Fe 2 As 2 Superconductor journal January 2019
Hedgehog spin-vortex crystal stabilized in a hole-doped iron-based superconductor text January 2017
Strain tuning and anisotropic spin correlations in iron-based systems text January 2019

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