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Title: Magnetic transition temperatures follow crystallographic symmetry in Samarium under high-pressures and low-temperatures

Journal Article · · Journal of Physics. Condensed Matter
 [1];  [1];  [2]
  1. Univ. of Alabama at Birmingham, Birmingham, AL (United States)
  2. Saint Augustine's Univ., Raleigh, NC (United States)

Magnetic ordering temperatures in rare earth metal samarium (Sm) have been studied using an ultrasensitive electrical transport measurement technique in a designer diamond anvil cell to high-pressure up to 47 GPa and low-temperature to 10 K. The two magnetic transitions at 106 K and 14 K in the α-Sm phase, attributed to antiferromagnetic ordering on hexagonal and cubic layers respectively, collapse in to one magnetic transition near 10 GPa when Sm assumes a double hexagonal close packed (dhcp) phase. On further increase in pressure above 34 GPa, the magnetic transitions split again as Sm adopts a hexagonal-hP3 structure indicating different magnetic transition temperatures for different crystallographic sites. A model for magnetic ordering for the hexagonal-hP3 phase in samarium has been proposed based on the experimental data. The magnetic transition temperatures closely follow the crystallographic symmetry during α-Sm → dhcp → fcc/dist.fcc → hP3 structure sequence at high-pressures and low-temperatures.

Research Organization:
Univ. of Alabama, Birmingham, AL (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
NA0002928; DMR-1460392
OSTI ID:
1334960
Journal Information:
Journal of Physics. Condensed Matter, Vol. 29, Issue 6; ISSN 0953-8984
Publisher:
IOP PublishingCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 5 works
Citation information provided by
Web of Science

References (13)

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High-pressure magnetic susceptibility experiments on the heavy lanthanides Gd, Tb, Dy, Ho, Er, and Tm journal May 2005
Magnetic and structural phase transitions in erbium at low temperatures and high pressures journal October 2011
Magnetic ordering temperatures in rare earth metal dysprosium under ultrahigh pressures journal April 2014
Anomalous pressure dependence of magnetic ordering temperature in Tb revealed by resistivity measurements to 141 GPa: Comparison with Gd and Dy journal May 2015
Phase transitions in samarium at high pressures journal January 1987
Intermediate 4 f bonding structure for samarium under pressure journal September 1994
The distorted-fcc phase of samarium journal May 2014
Studies on the pressure-temperature phase diagram of Nd, Sm, Gd and Dy journal July 1978
Fabrication of Diamond Based Sensors for Use in Extreme Environments journal April 2015
High pressure superconductivity in iron-based layered compounds studied using designer diamonds journal May 2009

Cited By (2)

High-pressure structural systematics in samarium up to 222 GPa journal May 2020
High-pressure structural systematics in samarium up to 222 GPa text January 2020

Figures / Tables (5)


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