Variation in superconducting transition temperature due to tetragonal domains in two-dimensionally doped SrTiO3

Noad, Hilary; Spanton, Eric M.; Nowack, Katja C.; Inoue, Hisashi; Kim, Minu; Merz, Tyler A.; Bell, Christopher; Hikita, Yasuyuki; Xu, Ruqing; Liu, Wenjun; Vailionis, Arturas; Hwang, Harold Y.; Moler, Kathryn A.

doi:10.1103/PhysRevB.94.174516

Title: Variation in superconducting transition temperature due to tetragonal domains in two-dimensionally doped ${SrTiO}_{3}$

Journal Article · Mon Nov 28 00:00:00 EST 2016 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.94.174516· OSTI ID:1328993

Noad, Hilary ^[1]; Spanton, Eric M. ^[1]; Nowack, Katja C. ^[2]; Inoue, Hisashi ^[2]; Kim, Minu ^[3]; Merz, Tyler A. ^[1]; Bell, Christopher ^[4]; Hikita, Yasuyuki ^[3]; Xu, Ruqing ^[5]; Liu, Wenjun ^[5]; Vailionis, Arturas ^[2]; Hwang, Harold Y. ^[1]; Moler, Kathryn A. ^[1]

SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., Stanford, CA (United States)
Stanford Univ., Stanford, CA (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States); Univ. of Bristol, Bristol (United Kingdom)
Argonne National Lab. (ANL), Argonne, IL (United States)

Strontium titanate is a low-temperature, non–Bardeen-Cooper-Schrieffer superconductor that superconducts to carrier concentrations lower than in any other system and exhibits avoided ferroelectricity at low temperatures. Neither the mechanism of superconductivity in strontium titanate nor the importance of the structure and dielectric properties for the superconductivity are well understood. We studied the effects of twin structure on superconductivity in a 5.5-nm-thick layer of niobium-doped SrTiO₃ embedded in undoped SrTiO₃. We used a scanning superconducting quantum interference device susceptometer to image the local diamagnetic response of the sample as a function of temperature. We observed regions that exhibited a superconducting transition temperature T_c ≳ 10% higher than the temperature at which the sample was fully superconducting. The pattern of these regions varied spatially in a manner characteristic of structural twin domains. Some regions are too wide to originate on twin boundaries; therefore, we propose that the orientation of the tetragonal unit cell with respect to the doped plane affects T_c. Finally, our results suggest that the anisotropic dielectric properties of SrTiO₃ are important for its superconductivity and need to be considered in any theory of the mechanism of the superconductivity.

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Research Organization:: SLAC National Accelerator Lab., Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-76SF00515; AC02-06CH11357

OSTI ID:: 1328993

Alternate ID(s):: OSTI ID: 1333608

Report Number(s):: SLAC-PUB-16840; PRBMDO

Journal Information:: Physical Review B, Vol. 94, Issue 17; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 26 works

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References (61)

Intrinsic spin-orbit coupling in superconducting $δ$ -doped SrTiO $_{3}$ heterostructures Kim, M.; Kozuka, Y.; Bell, C. Physical Review B, Vol. 86, Issue 8 https://doi.org/10.1103/PhysRevB.86.085121	journal	August 2012
Critical Doping for the Onset of a Two-Band Superconducting Ground State in ${SrTiO}_{3 - δ}$ Lin, Xiao; Bridoux, German; Gourgout, Adrien Physical Review Letters, Vol. 112, Issue 20 https://doi.org/10.1103/PhysRevLett.112.207002	journal	May 2014
Local electrostatic imaging of striped domain order in LaAlO3/SrTiO3 Honig, M.; Sulpizio, J. A.; Drori, J. Nature Materials, Vol. 12, Issue 12 https://doi.org/10.1038/nmat3810	journal	November 2013
Interface-induced superconductivity and strain-dependent spin density waves in FeSe/SrTiO3 thin films Tan, Shiyong; Zhang, Yan; Xia, Miao Nature Materials, Vol. 12, Issue 7 https://doi.org/10.1038/nmat3654	journal	May 2013
Depth resolved domain mapping in tetragonal SrTiO3 by micro-Laue diffraction Merz, T. A.; Noad, H.; Xu, R. Applied Physics Letters, Vol. 108, Issue 18 https://doi.org/10.1063/1.4948351	journal	May 2016
Stripes of increased diamagnetic susceptibility in underdoped superconducting $Ba {({Fe}_{1 - x} {Co}_{x})}_{2} {As}_{2}$ single crystals: Evidence for an enhanced superfluid density at twin boundaries Kalisky, B.; Kirtley, J. R.; Analytis, J. G. Physical Review B, Vol. 81, Issue 18 https://doi.org/10.1103/PhysRevB.81.184513	journal	May 2010
Dependence of the Superconducting Transition Temperature on Carrier Concentration in Semiconducting SrTi $O_{3}$ Schooley, J. F.; Hosler, W. R.; Ambler, E. Physical Review Letters, Vol. 14, Issue 9 https://doi.org/10.1103/PhysRevLett.14.305	journal	March 1965
X‐Ray Diffractometry of Low‐Temperature Phase Transformations in Strontium Titanate Lytle, Farrel W. Journal of Applied Physics, Vol. 35, Issue 7 https://doi.org/10.1063/1.1702820	journal	July 1964
Soft-Mode Superconductivity in $SrTi O_{3 - x}$ Appel, J. Physical Review, Vol. 180, Issue 2 https://doi.org/10.1103/PhysRev.180.508	journal	April 1969
Theory of Superconductivity in Polar Semiconductors and Its Application to N-Type Semiconducting SrTiO ₃ Takada, Yasutami Journal of the Physical Society of Japan, Vol. 49, Issue 4 https://doi.org/10.1143/JPSJ.49.1267	journal	October 1980
Polychromatic X-ray microdiffraction studies of mesoscale structure and dynamics Ice, G. E.; Larson, B. C.; Yang, W. Journal of Synchrotron Radiation, Vol. 12, Issue 2 https://doi.org/10.1107/S0909049504026949	journal	February 2005
A Quantum Critical Point Lying Beneath the Superconducting Dome in Iron Pnictides Shibauchi, T.; Carrington, A.; Matsuda, Y. Annual Review of Condensed Matter Physics, Vol. 5, Issue 1 https://doi.org/10.1146/annurev-conmatphys-031113-133921	journal	March 2014
Interface superconductivity in ${LaAlO}_{3} - {SrTiO}_{3}$ heterostructures Klimin, S. N.; Tempere, J.; Devreese, J. T. Physical Review B, Vol. 89, Issue 18 https://doi.org/10.1103/PhysRevB.89.184514	journal	May 2014
Mechanism of superconductivity in SrTiO3 Baratoff, Alexis; Binnig, Gerd Physica B+C, Vol. 108, Issue 1-3 https://doi.org/10.1016/0378-4363(81)90966-9	journal	August 1981
Fermi Surface and Superconductivity in Low-Density High-Mobility $δ$ -Doped ${SrTiO}_{3}$ Kim, M.; Bell, C.; Kozuka, Y. Physical Review Letters, Vol. 107, Issue 10 https://doi.org/10.1103/PhysRevLett.107.106801	journal	August 2011
Superconductivity above 100 K in single-layer FeSe films on doped SrTiO3 Ge, Jian-Feng; Liu, Zhi-Long; Liu, Canhua Nature Materials, Vol. 14, Issue 3 https://doi.org/10.1038/nmat4153	journal	November 2014
Enhancing the electron mobility via delta-doping in SrTiO3 Kozuka, Y.; Kim, M.; Ohta, H. Applied Physics Letters, Vol. 97, Issue 22 https://doi.org/10.1063/1.3524198	journal	November 2010
Gate-tuned superfluid density at the superconducting LaAlO $_{3}$ /SrTiO $_{3}$ interface Bert, Julie A.; Nowack, Katja C.; Kalisky, Beena Physical Review B, Vol. 86, Issue 6 https://doi.org/10.1103/PhysRevB.86.060503	journal	August 2012
Monodomain strontium titanate Müller, K. A.; Berlinger, W.; Capizzi, M. Solid State Communications, Vol. 8, Issue 7 https://doi.org/10.1016/0038-1098(70)90302-9	journal	April 1970
Superconducting Transition Temperatures of Semiconducting SrTi $O_{3}$ Koonce, C. S.; Cohen, Marvin L.; Schooley, J. F. Physical Review, Vol. 163, Issue 2 https://doi.org/10.1103/PhysRev.163.380	journal	November 1967
Superconductivity in the two-dimensional electron gas induced by high-energy optical phonon mode and large polarization of the ${SrTiO}_{3}$ substrate Rosenstein, Baruch; Shapiro, B. Ya.; Shapiro, I. Physical Review B, Vol. 94, Issue 2 https://doi.org/10.1103/PhysRevB.94.024505	journal	July 2016
What lies beneath the dome? Broun, D. M. Nature Physics, Vol. 4, Issue 3 https://doi.org/10.1038/nphys909	journal	March 2008
Nonmonotonic anisotropy in charge conduction induced by antiferrodistortive transition in metallic ${SrTiO}_{3}$ Tao, Qian; Loret, Bastien; Xu, Bin Physical Review B, Vol. 94, Issue 3 https://doi.org/10.1103/PhysRevB.94.035111	journal	July 2016
Scanning superconducting quantum interference device microscope in a dilution refrigerator Björnsson, Per G.; Gardner, Brian W.; Kirtley, John R. Review of Scientific Instruments, Vol. 72, Issue 11 https://doi.org/10.1063/1.1406931	journal	November 2001
Phase diagram and electronic indication of high-temperature superconductivity at 65 K in single-layer FeSe films He, Shaolong; He, Junfeng; Zhang, Wenhao Nature Materials, Vol. 12, Issue 7 https://doi.org/10.1038/nmat3648	journal	May 2013
Ferroelectric quantum criticality Rowley, S. E.; Spalek, L. J.; Smith, R. P. Nature Physics, Vol. 10, Issue 5 https://doi.org/10.1038/nphys2924	journal	March 2014
Interfacial mode coupling as the origin of the enhancement of Tc in FeSe films on SrTiO3 Lee, J. J.; Schmitt, F. T.; Moore, R. G. Nature, Vol. 515, Issue 7526 https://doi.org/10.1038/nature13894	journal	November 2014
Interface superconductor with gap behaviour like a high-temperature superconductor Richter, C.; Boschker, H.; Dietsche, W. Nature, Vol. 502, Issue 7472 https://doi.org/10.1038/nature12494	journal	October 2013
Electron pairing without superconductivity Cheng, Guanglei; Tomczyk, Michelle; Lu, Shicheng Nature, Vol. 521, Issue 7551 https://doi.org/10.1038/nature14398	journal	May 2015
Rietveld analysis of strontium titanate in the Müller state Kiat, J. M.; Roisnel, Thierry Journal of Physics: Condensed Matter, Vol. 8, Issue 19 https://doi.org/10.1088/0953-8984/8/19/021	journal	May 1996
Gradiometric micro-SQUID susceptometer for scanning measurements of mesoscopic samples Huber, Martin E.; Koshnick, Nicholas C.; Bluhm, Hendrik Review of Scientific Instruments, Vol. 79, Issue 5 https://doi.org/10.1063/1.2932341	journal	May 2008
Phonon mechanism in the most dilute superconductor n -type SrTiO ₃ Gor’kov, Lev P. Proceedings of the National Academy of Sciences, Vol. 113, Issue 17 https://doi.org/10.1073/pnas.1604145113	journal	April 2016
Locally enhanced conductivity due to the tetragonal domain structure in LaAlO3/SrTiO3 heterointerfaces Kalisky, Beena; Spanton, Eric M.; Noad, Hilary Nature Materials, Vol. 12, Issue 12 https://doi.org/10.1038/nmat3753	journal	September 2013
Violation of Anderson’s theorem for superconductors with nonretarded interactions Fay, D.; Appel, J. Physical Review B, Vol. 51, Issue 21 https://doi.org/10.1103/PhysRevB.51.15604	journal	June 1995
Theory of dirty superconductors Anderson, P. W. Journal of Physics and Chemistry of Solids, Vol. 11, Issue 1-2 https://doi.org/10.1016/0022-3697(59)90036-8	journal	September 1959
Two-Phonon Deformation Potential and Superconductivity in Degenerate Semiconductors Ngai, K. L. Physical Review Letters, Vol. 32, Issue 5 https://doi.org/10.1103/PhysRevLett.32.215	journal	February 1974
Quantum Critical Origin of the Superconducting Dome in ${SrTiO}_{3}$ Edge, Jonathan M.; Kedem, Yaron; Aschauer, Ulrich Physical Review Letters, Vol. 115, Issue 24 https://doi.org/10.1103/PhysRevLett.115.247002	journal	December 2015
Current Distribution in Superconducting Films Carrying Quantized Fluxoids Pearl, J. Applied Physics Letters, Vol. 5, Issue 4 https://doi.org/10.1063/1.1754056	journal	August 1964
Microscopic Examination of SrTiO ₃ at Low Temperatures Sawaguchi, Etsuro; Kikuchi, Atsushi; Kodera, Yōichi Journal of the Physical Society of Japan, Vol. 18, Issue 3 https://doi.org/10.1143/JPSJ.18.459	journal	March 1963
Interpretation of the temperature dependence of the electromagnetic penetration depth in ${YBa}_{2}$ ${Cu}_{3}$ $O_{7 - δ}$ Annett, James; Goldenfeld, Nigel; Renn, S. R. Physical Review B, Vol. 43, Issue 4 https://doi.org/10.1103/PhysRevB.43.2778	journal	February 1991
Fermi Surface of the Most Dilute Superconductor Lin, Xiao; Zhu, Zengwei; Fauqué, Benoît Physical Review X, Vol. 3, Issue 2 https://doi.org/10.1103/PhysRevX.3.021002	journal	April 2013
Theory of Superconductivity Bardeen, J.; Cooper, L. N.; Schrieffer, J. R. Physical Review, Vol. 108, Issue 5 https://doi.org/10.1103/PhysRev.108.1175	journal	December 1957
Scanning SQUID susceptometry of a paramagnetic superconductor Kirtley, J. R.; Kalisky, B.; Bert, J. A. Physical Review B, Vol. 85, Issue 22 https://doi.org/10.1103/PhysRevB.85.224518	journal	June 2012
Imaging currents in HgTe quantum wells in the quantum spin Hall regime Nowack, Katja C.; Spanton, Eric M.; Baenninger, Matthias Nature Materials, Vol. 12, Issue 9 https://doi.org/10.1038/nmat3682	journal	June 2013
Dielectric Properties of Strontium Titanate at Low Temperature Saifi, M. A.; Cross, L. E. Physical Review B, Vol. 2, Issue 3 https://doi.org/10.1103/PhysRevB.2.677	journal	August 1970
Local Electrical Imaging of Tetragonal Domains and Field-Induced Ferroelectric Twin Walls in Conducting ${SrTiO}_{3}$ Ma, H. J. Harsan; Scharinger, S.; Zeng, S. W. Physical Review Letters, Vol. 116, Issue 25 https://doi.org/10.1103/PhysRevLett.116.257601	journal	June 2016
Dramatic mobility enhancements in doped SrTiO3 thin films by defect management Kozuka, Y.; Hikita, Y.; Bell, C. Applied Physics Letters, Vol. 97, Issue 1 https://doi.org/10.1063/1.3457994	journal	July 2010
Two-dimensional normal-state quantum oscillations in a superconducting heterostructure Kozuka, Y.; Kim, M.; Bell, C. Nature, Vol. 462, Issue 7272, p. 487-490 https://doi.org/10.1038/nature08566	journal	November 2009
Superconductivity by small polarons Zinamon, Z. The Philosophical Magazine: A Journal of Theoretical Experimental and Applied Physics, Vol. 21, Issue 170 https://doi.org/10.1080/14786437008238421	journal	February 1970
Dielectric Properties of SrTi $O_{3}$ at Low Temperatures Sakudo, T.; Unoki, H. Physical Review Letters, Vol. 26, Issue 14 https://doi.org/10.1103/PhysRevLett.26.851	journal	April 1971
Multiple nodeless superconducting gaps in optimally doped ${SrTi}_{1 - x} {Nb}_{x} O_{3}$ Lin, Xiao; Gourgout, Adrien; Bridoux, German Physical Review B, Vol. 90, Issue 14 https://doi.org/10.1103/PhysRevB.90.140508	journal	October 2014
Domain Wall Damping and Elastic Softening in ${SrTiO}_{3}$ : Evidence for Polar Twin Walls Scott, J. F.; Salje, E. K. H.; Carpenter, M. A. Physical Review Letters, Vol. 109, Issue 18 https://doi.org/10.1103/PhysRevLett.109.187601	journal	October 2012
A high-mobility electron gas at the LaAlO3/SrTiO3 heterointerface Ohtomo, A.; Hwang, H. Y. Nature, Vol. 427, Issue 6973 https://doi.org/10.1038/nature02308	journal	January 2004
Microscopic mechanisms for the Fermi-liquid behavior of Nb-doped strontium titanate Klimin, S. N.; Tempere, J.; van der Marel, D. Physical Review B, Vol. 86, Issue 4 https://doi.org/10.1103/PhysRevB.86.045113	journal	July 2012
Superconducting Interfaces Between Insulating Oxides Reyren, N.; Thiel, S.; Caviglia, A. D. Science, Vol. 317, Issue 5842 https://doi.org/10.1126/science.1146006	journal	August 2007
Three-dimensional X-ray structural microscopy with submicrometre resolution Larson, B. C.; Yang, Wenge; Ice, G. E. Nature, Vol. 415, p. 887-890 https://doi.org/10.1038/415887a	journal	February 2002
SrTi $O_{3}$ : An intrinsic quantum paraelectric below 4 K Müller, K. A.; Burkard, H. Physical Review B, Vol. 19, Issue 7 https://doi.org/10.1103/PhysRevB.19.3593	journal	April 1979
Twinning-plane superconductivity Khlyustikov, I. N.; Buzdin, A. I. Advances in Physics, Vol. 36, Issue 3 https://doi.org/10.1080/00018738700101012	journal	January 1987
Landau-Ginzburg model of interphase boundaries in improper ferroelastic Perovskites of $D_{4 h}^{18}$ symmetry Cao, Wenwu; Barsch, Gerhard R. Physical Review B, Vol. 41, Issue 7 https://doi.org/10.1103/PhysRevB.41.4334	journal	March 1990
Electron Spin Resonance of Fe ³⁺ in SrTiO ₃ with Special Reference to the 110°K Phase Transition Unoki, Hiromi; Sakudo, Tunetaro Journal of the Physical Society of Japan, Vol. 23, Issue 3 https://doi.org/10.1143/JPSJ.23.546	journal	September 1967
The Race to X-ray Microbeam and Nanobeam Science Ice, G. E.; Budai, J. D.; Pang, J. W. L. Science, Vol. 334, Issue 6060 https://doi.org/10.1126/science.1202366	journal	December 2011

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Physics of SrTiO ₃ -based heterostructures and nanostructures: a review Pai, Yun-Yi; Tylan-Tyler, Anthony; Irvin, Patrick Reports on Progress in Physics, Vol. 81, Issue 3 https://doi.org/10.1088/1361-6633/aa892d	journal	February 2018
Correlation between superconductivity, band filling, and electron confinement at the ${LaAlO}_{3} / {SrTiO}_{3}$ interface Smink, A. E. M.; Stehno, M. P.; de Boer, J. C. Physical Review B, Vol. 97, Issue 24 https://doi.org/10.1103/physrevb.97.245113	journal	June 2018
Physics of SrTiO$_3$-based heterostructures and nanostructures: a review Pai, Yun-Yi; Tylan-Tyler, Anthony; Irvin, Patrick arXiv https://doi.org/10.48550/arxiv.1702.07690	text	January 2017

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