Competing antiferromagnetism in a quasi-2D itinerant ferromagnet: Fe3GeTe2

Yi, Jieyu; Zhuang, Houlong; Zou, Qiang; Wu, Zhiming; Cao, Guixin; Tang, Siwei; Calder, S. A.; Kent, P. R. C.; Mandrus, David; Gai, Zheng

doi:10.1088/2053-1583/4/1/011005

Title: Competing antiferromagnetism in a quasi-2D itinerant ferromagnet: Fe₃GeTe₂

Journal Article · Tue Nov 15 00:00:00 EST 2016 · 2D Materials

DOI:https://doi.org/10.1088/2053-1583/4/1/011005· OSTI ID:1332067

Yi, Jieyu ^[1]; Zhuang, Houlong ^[2]; Zou, Qiang ^[2]; Wu, Zhiming ^[2]; Cao, Guixin ^[2]; Tang, Siwei ^[1]; Calder, S. A. ^[2];

^[2]; Mandrus, David ^[1];

^[2]

Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Fe₃GeTe₂ is known as an air-stable layered metal with itinerant ferromagnetism with a transition temperature of about 220 K. From extensive dc and ac magnetic measurements, we have determined that the ferromagnetic layers of Fe₃GeTe₂ order antiferromagnetically along the c-axis blow 152 K. The antiferromagnetic state was further substantiated by theoretical calculation to be the ground state. A magnetic structure model was proposed to describe the antiferromagnetic ground state as well as competition between antiferromagnetic and ferromagnetic states. Furthermore, Fe₃GeTe₂ shares many common features with pnictide superconductors and may be a promising system in which to search for unconventional superconductivity.

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Research Organization:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1332067

Alternate ID(s):: OSTI ID: 1332019

Journal Information:: 2D Materials, Vol. 4, Issue 1; ISSN 2053-1583

Publisher:: IOP PublishingCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 88 works

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Lattice Dynamics, Phonon Chirality, and Spin–Phonon Coupling in 2D Itinerant Ferromagnet Fe ₃ GeTe ₂ Du, Luojun; Tang, Jian; Zhao, Yanchong Advanced Functional Materials, Vol. 29, Issue 48 https://doi.org/10.1002/adfm.201904734	journal	September 2019
Fe _{5− x} Ge ₂ Te ₂ —a New Exfoliable Itinerant Ferromagnet with High Curie Temperature and Large Perpendicular Magnetic Anisotropy Jothi, Palani R.; Scheifers, Jan P.; Zhang, Yuemei physica status solidi (RRL) – Rapid Research Letters, Vol. 14, Issue 3 https://doi.org/10.1002/pssr.201900666	journal	December 2019
The van der Waals Ferromagnets Fe _5- _δ GeTe ₂ and Fe _5- _δ _-x Ni _x GeTe ₂ - Crystal Structure, Stacking Faults, and Magnetic Properties : The van der Waals Ferromagnets Fe Stahl, Juliane; Shlaen, Evgeniya; Johrendt, Dirk Zeitschrift für anorganische und allgemeine Chemie, Vol. 644, Issue 24 https://doi.org/10.1002/zaac.201800456	journal	November 2018
Hard magnetic properties in nanoflake van der Waals Fe3GeTe2 Tan, Cheng; Lee, Jinhwan; Jung, Soon-Gil Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-04018-w	journal	April 2018
Two-dimensional itinerant ferromagnetism in atomically thin Fe3GeTe2 Fei, Zaiyao; Huang, Bevin; Malinowski, Paul Nature Materials, Vol. 17, Issue 9 https://doi.org/10.1038/s41563-018-0149-7	journal	August 2018
Critical behavior of the van der Waals bonded high T C ferromagnet Fe3GeTe2 Liu, Bingjie; Zou, Youming; Zhou, Shiming Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-06671-5	journal	July 2017
Anisotropic magnetocaloric effect in Fe3−xGeTe2 Liu, Yu; Li, Jun; Tao, Jing Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-019-49654-4	journal	September 2019
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Emergence of Kondo lattice behavior in a van der Waals itinerant ferromagnet, Fe ₃ GeTe ₂ Zhang, Yun; Lu, Haiyan; Zhu, Xiegang Science Advances, Vol. 4, Issue 1 https://doi.org/10.1126/sciadv.aao6791	journal	January 2018
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Two-Dimensional Itinerant Ising Ferromagnetism in Atomically thin Fe3GeTe2 Fei, Zaiyao; Huang, Bevin; Malinowski, Paul arXiv https://doi.org/10.48550/arxiv.1803.02559	text	January 2018
Hard magnetic properties in nanoflake van der Waals Fe3GeTe2 Tan, Cheng; Lee, Jinhwan; Jung, Soon-Gil arXiv https://doi.org/10.48550/arxiv.1803.02934	text	January 2018
Long Range Intrinsic Ferromagnetism in Two Dimensional Materials and Dissipationless Future Technologies Shabbir, Babar; Nadeem, Muhammad; Dai, Zhigao arXiv https://doi.org/10.48550/arxiv.1810.09053	text	January 2018
Anisotropic magnetocaloric effect in Fe$_{3-x}$GeTe$_2$ Liu, Yu; Li, Jun; Tao, Jing arXiv https://doi.org/10.48550/arxiv.1904.03873	text	January 2019
Thickness-dependent magnetic order in CrI$_3$ single crystals Liu, Yu; Wu, Lijun; Tong, Xiao arXiv https://doi.org/10.48550/arxiv.1908.09969	text	January 2019

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Title: Competing antiferromagnetism in a quasi-2D itinerant ferromagnet: Fe3GeTe2

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Title: Competing antiferromagnetism in a quasi-2D itinerant ferromagnet: Fe₃GeTe₂