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Title: Two-dimensional fourier transform spectrometer

Abstract

The present invention relates to a system and methods for acquiring two-dimensional Fourier transform (2D FT) spectra. Overlap of a collinear pulse pair and probe induce a molecular response which is collected by spectral dispersion of the signal modulated probe beam. Simultaneous collection of the molecular response, pulse timing and characteristics permit real time phasing and rapid acquisition of spectra. Full spectra are acquired as a function of pulse pair timings and numerically transformed to achieve the full frequency-frequency spectrum. This method demonstrates the ability to acquire information on molecular dynamics, couplings and structure in a simple apparatus. Multi-dimensional methods can be used for diagnostic and analytical measurements in the biological, biomedical, and chemical fields.

Inventors:
;
Publication Date:
Research Org.:
Massachusetts Institute of Technology, Cambridge, MA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1330327
Patent Number(s):
9,476,768
Application Number:
13/955,158
Assignee:
Massachusetts Institute of Technology (Cambridge, MA) CHO
DOE Contract Number:  
FG02-99ER14988
Resource Type:
Patent
Resource Relation:
Patent File Date: 2013 Jul 31
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS

Citation Formats

DeFlores, Lauren, and Tokmakoff, Andrei. Two-dimensional fourier transform spectrometer. United States: N. p., 2016. Web.
DeFlores, Lauren, & Tokmakoff, Andrei. Two-dimensional fourier transform spectrometer. United States.
DeFlores, Lauren, and Tokmakoff, Andrei. Tue . "Two-dimensional fourier transform spectrometer". United States. doi:. https://www.osti.gov/servlets/purl/1330327.
@article{osti_1330327,
title = {Two-dimensional fourier transform spectrometer},
author = {DeFlores, Lauren and Tokmakoff, Andrei},
abstractNote = {The present invention relates to a system and methods for acquiring two-dimensional Fourier transform (2D FT) spectra. Overlap of a collinear pulse pair and probe induce a molecular response which is collected by spectral dispersion of the signal modulated probe beam. Simultaneous collection of the molecular response, pulse timing and characteristics permit real time phasing and rapid acquisition of spectra. Full spectra are acquired as a function of pulse pair timings and numerically transformed to achieve the full frequency-frequency spectrum. This method demonstrates the ability to acquire information on molecular dynamics, couplings and structure in a simple apparatus. Multi-dimensional methods can be used for diagnostic and analytical measurements in the biological, biomedical, and chemical fields.},
doi = {},
journal = {},
number = ,
volume = ,
place = {United States},
year = {Tue Oct 25 00:00:00 EDT 2016},
month = {Tue Oct 25 00:00:00 EDT 2016}
}

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Works referenced in this record:

Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide
journal, May 2007

  • Shim, S.-H.; Strasfeld, D. B.; Ling, Y. L.
  • Proceedings of the National Academy of Sciences, Vol. 104, Issue 36, p. 14197-14202
  • DOI: 10.1073/pnas.0700804104