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Title: Inverse modeling of pan-Arctic methane emissions at high spatial resolution: what can we learn from assimilating satellite retrievals and using different process-based wetland and lake biogeochemical models?

Journal Article · · Atmospheric Chemistry and Physics (Online)

Abstract. Understanding methane emissions from the Arctic, a fast-warming carbon reservoir, is important for projecting future changes in the global methane cycle. Here we optimized methane emissions from north of 60°N (pan-Arctic) regions using a nested-grid high-resolution inverse model that assimilates both high-precision surface measurements and column-average SCanning Imaging Absorption spectroMeter for Atmospheric CHartogrphY (SCIAMACHY) satellite retrievals of methane mole fraction. For the first time, methane emissions from lakes were integrated into an atmospheric transport and inversion estimate, together with prior wetland emissions estimated with six biogeochemical models. In our estimates, in 2005, global methane emissions were in the range of 496.4–511.5Tgyr–1, and pan-Arctic methane emissions were in the range of 11.9–28.5Tgyr–1. Methane emissions from pan-Arctic wetlands and lakes were 5.5–14.2 and 2.4–14.2Tgyr–1, respectively. Methane emissions from Siberian wetlands and lakes are the largest and also have the largest uncertainty. Our results indicate that the uncertainty introduced by different wetland models could be much larger than the uncertainty of each inversion. We also show that assimilating satellite retrievals can reduce the uncertainty of the nested-grid inversions. The significance of lake emissions cannot be identified across the pan-Arctic by high-resolution inversions, but it is possible to identify high lake emissions from some specific regions. In contrast to global inversions, high-resolution nested-grid inversions perform better in estimating near-surface methane concentrations.

Research Organization:
Purdue Univ., West Lafayette, IN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Biological and Environmental Research (BER)
Grant/Contract Number:
FG02-08ER64599; AC02-05CH11231
OSTI ID:
1328713
Alternate ID(s):
OSTI ID: 1465820
Journal Information:
Atmospheric Chemistry and Physics (Online), Journal Name: Atmospheric Chemistry and Physics (Online) Vol. 16 Journal Issue: 19; ISSN 1680-7324
Publisher:
Copernicus Publications, EGUCopyright Statement
Country of Publication:
Germany
Language:
English
Citation Metrics:
Cited by: 21 works
Citation information provided by
Web of Science

References (91)

Anthropogenic emissions of methane in the United States journal November 2013
Methane emissions in East Asia for 2000-2011 estimated using an atmospheric Bayesian inversion: METHANE EMISSIONS IN EAST ASIA journal May 2015
Seasonal climatology of CO 2 across North America from aircraft measurements in the NOAA/ESRL Global Greenhouse Gas Reference Network : VERTICAL CLIMATOLOGY OF CO journal May 2015
Interannual growth rate variations of atmospheric CO 2 and its δ 13 C, H 2 , CH 4 , and CO between 1992 and 1999 linked to biomass burning : MULTISPECIES INTERANNUAL VARIABILITY journal September 2002
A multi-year methane inversion using SCIAMACHY, accounting for systematic errors using TCCON measurements journal January 2014
CarbonTracker-CH 4 : an assimilation system for estimating emissions of atmospheric methane journal January 2014
Reduced methane growth rate explained by decreased Northern Hemisphere microbial sources journal August 2011
Climate change and the permafrost carbon feedback journal April 2015
Long-term decline of global atmospheric ethane concentrations and implications for methane journal August 2012
Renewed growth of atmospheric methane journal January 2008
Magnitude and seasonality of wetland methane emissions from the Hudson Bay Lowlands (Canada) journal January 2011
Inverse Modeling of Atmospheric Carbon Dioxide Fluxes journal October 2001
Modeling methane emissions from arctic lakes: Model development and site‐level study journal April 2015
On the consistency between global and regional methane emissions inferred from SCIAMACHY, TANSO-FTS, IASI and surface measurements journal January 2014
Impact of meteorology and emissions on methane trends, 1990–2004 journal January 2006
Improved Attribution of Climate Forcing to Emissions journal October 2009
Reactive greenhouse gas scenarios: Systematic exploration of uncertainties and the role of atmospheric chemistry: ATMOSPHERIC CHEMISTRY AND GREENHOUSE GASES journal May 2012
Inverse modelling of CH 4 emissions for 2010–2011 using different satellite retrieval products from GOSAT and SCIAMACHY journal January 2015
Estimating regional methane surface fluxes: the relative importance of surface and GOSAT mole fraction measurements journal January 2013
Atmospheric observations of Arctic Ocean methane emissions up to 82° north journal April 2012
Natural and anthropogenic methane fluxes in Eurasia: a mesoscale quantification by generalized atmospheric inversion journal January 2015
CH 4 retrievals from space-based solar backscatter measurements: Performance evaluation against simulated aerosol and cirrus loaded scenes : EVALUATION OF CH journal December 2010
Extensive release of methane from Arctic seabed west of Svalbard during summer 2014 does not influence the atmosphere: CH journal May 2016
Methane observations from the Greenhouse Gases Observing SATellite: Comparison to ground-based TCCON data and model calculations: GOSAT CH journal August 2011
Estimating global and North American methane emissions with high spatial resolution using GOSAT satellite data journal January 2015
A scalable model for methane consumption in arctic mineral soils journal May 2016
Estimating wetland methane emissions from the northern high latitudes from 1990 to 2009 using artificial neural networks: METHANE EMISSIONS FROM NORTHERN WETLANDS journal June 2013
An assessment of the carbon balance of Arctic tundra: comparisons among observations, process models, and atmospheric inversions journal January 2012
Freshwater Methane Emissions Offset the Continental Carbon Sink journal January 2011
NET EMISSIONS OF CH 4 AND CO 2 IN ALASKA: IMPLICATIONS FOR THE REGION'S GREENHOUSE GAS BUDGET journal January 2007
Inverse Methods for Atmospheric Sounding: Theory and Practice book July 2000
HEMCO v1.0: a versatile, ESMF-compliant component for calculating emissions in atmospheric models journal January 2014
Large-Scale Controls of Methanogenesis Inferred from Methane and Gravity Spaceborne Data journal January 2010
Methane release from wetlands and watercourses in Europe journal March 2009
Tropical methane emissions: A revised view from SCIAMACHY onboard ENVISAT journal January 2008
Methane emissions from pan‐Arctic lakes during the 21st century: An analysis with process‐based models of lake evolution and biogeochemistry journal December 2015
Global fire emissions and the contribution of deforestation, savanna, forest, agricultural, and peat fires (1997–2009) journal January 2010
Development of the adjoint of GEOS-Chem journal January 2007
Three-dimensional model synthesis of the global methane cycle journal January 1991
The Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS) mission: design, execution, and first results journal January 2010
Methane bubbling from Siberian thaw lakes as a positive feedback to climate warming journal September 2006
Conversion of NOAA atmospheric dry air CH 4 mole fractions to a gravimetrically prepared standard scale journal January 2005
Modeling methane emissions from the Alaskan Yukon River basin, 1986-2005, by coupling a large-scale hydrological model and a process-based methane model: CH journal April 2012
Inverse Problems in Atmospheric Constituent Transport book January 2002
Comparison of adjoint and analytical Bayesian inversion methods for constraining Asian sources of carbon monoxide using satellite (MOPITT) measurements of CO columns journal January 2009
Methane bubbling from northern lakes: present and future contributions to the global methane budget
  • Walter, Katey M.; Smith, Laurence C.; Stuart Chapin, F.
  • Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 365, Issue 1856 https://doi.org/10.1098/rsta.2007.2036
journal May 2007
Satellite chartography of atmospheric methane from SCIAMACHY on board ENVISAT: Analysis of the years 2003 and 2004 journal January 2006
Global column-averaged methane mixing ratios from 2003 to 2009 as derived from SCIAMACHY: Trends and variability journal January 2011
Satellite chartography of atmospheric methane from SCIAMACHY on board ENVISAT: 2. Evaluation based on inverse model simulations journal January 2007
Comparison of CH 4 inversions based on 15 months of GOSAT and SCIAMACHY observations : INVERSE MODELING OF SATELLITE RETRIEVED journal October 2013
Towards robust regional estimates of CO2 sources and sinks using atmospheric transport models journal February 2002
Development and validation of a global database of lakes, reservoirs and wetlands journal August 2004
Multidimensional Flux-Form Semi-Lagrangian Transport Schemes journal September 1996
Arctic methane sources: Isotopic evidence for atmospheric inputs: ARCTIC METHANE SOURCES journal November 2011
Atmospheric constraints on the methane emissions from the East Siberian Shelf journal January 2016
Methane fluxes between terrestrial ecosystems and the atmosphere at northern high latitudes during the past century: A retrospective analysis with a process-based biogeochemistry model: METHANE EMISSIONS FROM NORTHERN HIGH LATITUDES journal August 2004
Recent decreases in fossil-fuel emissions of ethane and methane derived from firn air journal August 2011
Inverse modelling of national and European CH<sub>4</sub> emissions using the atmospheric zoom model TM5 journal January 2005
Observational constraints on recent increases in the atmospheric CH 4 burden journal January 2009
Three decades of global methane sources and sinks journal September 2013
Global-scale transport of carbon dioxide in the troposphere journal January 2008
No inter-hemispheric δ13CH4 trend observed journal June 2012
CO 2 and CH 4 exchanges between land ecosystems and the atmosphere in northern high latitudes over the 21st century journal January 2006
Atmospheric methane levels off: Temporary pause or a new steady-state? journal January 2003
Aircraft and tower measurements of CO 2 concentration in the planetary boundary layer and the lower free troposphere over southern taiga in West Siberia: Long-term records from 2002 to 2011 : VERTICAL CO journal August 2013
Contribution of anthropogenic and natural sources to atmospheric methane variability journal September 2006
Continuing decline in the growth rate of the atmospheric methane burden journal June 1998
Improved analysis-error covariance matrix for high-dimensional variational inversions: application to source estimation using a 3D atmospheric transport model: Improved Analysis-Error Covariance Estimates journal January 2015
Methane fluxes from the sea to the atmosphere across the Siberian shelf seas: CH journal June 2016
Permafrost carbon-climate feedbacks accelerate global warming journal August 2011
Inferring regional sources and sinks of atmospheric CO 2 from GOSAT XCO 2 data journal January 2014
Inverse modeling of global and regional CH 4 emissions using SCIAMACHY satellite retrievals journal January 2009
Seasonal and interannual variability in wetland methane emissions simulated by CLM4Me' and CAM-chem and comparisons to observations of concentrations journal January 2015
Natural and transboundary pollution influences on sulfate-nitrate-ammonium aerosols in the United States: Implications for policy journal January 2004
Methane on the Rise--Again journal January 2014
Mapping of North American methane emissions with high spatial resolution by inversion of SCIAMACHY satellite data: NORTH AMERICA METHANE EMISSION INVERSION journal June 2014
Global modeling of tropospheric chemistry with assimilated meteorology: Model description and evaluation journal October 2001
Present state of global wetland extent and wetland methane modelling: conclusions from a model inter-comparison project (WETCHIMP) journal January 2013
Comparative inverse analysis of satellite (MOPITT) and aircraft (TRACE-P) observations to estimate Asian sources of carbon monoxide: COMPARATIVE INVERSE ANALYSIS journal December 2004
Quantifying the impact of model errors on top-down estimates of carbon monoxide emissions using satellite observations journal January 2011
Atmospheric CH 4 in the first decade of the 21st century: Inverse modeling analysis using SCIAMACHY satellite retrievals and NOAA surface measurements : CH journal July 2013
Methane Emissions from a Small Wind Shielded Lake Determined by Eddy Covariance, Flux Chambers, Anchored Funnels, and Boundary Model Calculations: A Comparison journal April 2012
Present state of global wetland extent and wetland methane modelling: methodology of a model inter-comparison project (WETCHIMP) journal January 2013
Atmospheric Methane:  Trends and Cycles of Sources and Sinks journal April 2007
Optimized regional and interannual variability of lightning in a global chemical transport model constrained by LIS/OTD satellite data: IAV OF LIGHTNING CONSTRAINED BY LIS/OTD journal October 2012
Construction of non-diagonal background error covariance matrices for global chemical data assimilation journal January 2011
A 3-D model analysis of the slowdown and interannual variability in the methane growth rate from 1988 to 1997: METHANE INTERANNUAL VARIABILITY journal August 2004
Observational constraints on the distribution, seasonality, and environmental predictors of North American boreal methane emissions journal February 2014
Soil organic carbon pools in the northern circumpolar permafrost region: SOIL ORGANIC CARBON POOLS journal June 2009
Four-dimensional variational data assimilation for inverse modelling of atmospheric methane emissions: method and comparison with synthesis inversion journal January 2008
Arctic lakes are continuous methane sources to the atmosphere under warming conditions journal May 2015

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