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Title: Orbital-exchange and fractional quantum number excitations in an f-electron metal, Yb 2 Pt 2 Pb

Journal Article · · Science

Exotic quantum states and fractionalized magnetic excitations, such as spinons in one-dimensional chains, are generally expected to occur in 3d transition metal systems with spin 1/2. Our neutron-scattering experiments on the 4f-electron metal Yb2Pt2Pb overturn this conventional wisdom. We observe broad magnetic continuum dispersing in only one direction, which indicates that the underlying elementary excitations are spinons carrying fractional spin-1/2. These spinons are the emergent quantum dynamics of the anisotropic, orbital-dominated Yb moments. Owing to their unusual origin, only longitudinal spin fluctuations are measurable, whereas the transverse excitations such as spin waves are virtually invisible to magnetic neutron scattering. Furthermore, the proliferation of these orbital-spinons strips the electrons of their orbital identity, resulting in charge-orbital separation.

Research Organization:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
SC00112704; NSF-DMR-1310008
OSTI ID:
1441090
Alternate ID(s):
OSTI ID: 1263910
Report Number(s):
BNL-112301-2016-JA; /sci/352/6290/1206.atom
Journal Information:
Science, Journal Name: Science Vol. 352 Journal Issue: 6290; ISSN 0036-8075
Publisher:
American Association for the Advancement of Science (AAAS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 60 works
Citation information provided by
Web of Science

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Cited By (15)

Experimental observation of Bethe strings journal February 2018
Probing multi-spinon excitations outside of the two-spinon continuum in the antiferromagnetic spin chain cuprate Sr2CuO3 journal December 2018
Tomonaga–Luttinger liquid behavior and spinon confinement in YbAlO3 journal February 2019
Spinon confinement and a sharp longitudinal mode in Yb2Pt2Pb in magnetic fields journal March 2019
Low dimensional and frustrated antiferromagnetic interactions in transition metal chloride complexes with simple amine ligands journal January 2019
The cold neutron chopper spectrometer at the Spallation Neutron Source—A review of the first 8 years of operation journal September 2016
Sequential localization of a complex electron fluid journal August 2019
Theory perspective: SCES 2016 journal September 2016
Suppression of ferromagnetic order by Ag-doping: a neutron scattering investigation on Ce 2 (Pd 1− x Ag x ) 2 In ( x   =  0.20, 0.50) journal June 2018
Crystal structure and physical properties of the two stannides EuPdSn 2 and YbPdSn 2 journal November 2018
YbPd 2 In : A promising candidate for strong entropy accumulation at very low temperature journal November 2019
Low-temperature spin dynamics in the TmFeO 3 orthoferrite with a non-Kramers ion journal January 2020
Nonequilibrium spin transport in integrable spin chains: Persistent currents and emergence of magnetic domains journal July 2017
Field-induced incommensurate ordering in Heisenberg chains coupled by Ising interaction: Model for ytterbium aluminum perovskite YbAlO 3 journal June 2019
Open XXZ chain and boundary modes at zero temperature journal January 2019

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