Pressure-induced electronic phase separation of magnetism and superconductivity in CrAs
- Paul Scherrer Inst. (PSI), Villigen (Switzerland)
- Ruhr-Univ. Bochum, Bochum (Germany); Federal Univ., Kazan (Russia)
- Paul Scherrer Inst. (PSI), Villigen (Switzerland); Univ. of Geneva, Geneva (Switzerland)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- ETH Zurich, Zurich (Switzerland)
We report that the recent discovery of pressure (p) induced superconductivity in the binary helimagnet CrAs has raised questions on how superconductivity emerges from the magnetic state and on the mechanism of the superconducting pairing. In the present work the suppression of magnetism and the occurrence of superconductivity in CrAs were studied by means of muon spin rotation. The magnetism remains bulk up to p ≃ 3.5 kbar while its volume fraction gradually decreases with increasing pressure until it vanishes at p ≃ 7 kbar. At 3.5 kbar superconductivity abruptly appears with its maximum Tc ≃ 1.2 K which decreases upon increasing the pressure. In the intermediate pressure region (3.5≲ p ≲ 7 kbar) the superconducting and the magnetic volume fractions are spatially phase separated and compete for phase volume. Our results indicate that the less conductive magnetic phase provides additional carriers (doping) to the superconducting parts of the CrAs sample thus leading to an increase of the transition temperature (Tc) and of the superfluid density (ρs). A scaling of ρs with Tc3.2 as well as the phase separation between magnetism and superconductivity point to a conventional mechanism of the Cooper-pairing in CrAs.
- Research Organization:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Sponsoring Organization:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- Grant/Contract Number:
- 57051534; AC05-00OR22725
- OSTI ID:
- 1259706
- Alternate ID(s):
- OSTI ID: 1286900
- Journal Information:
- Scientific Reports, Vol. 5; ISSN 2045-2322
- Publisher:
- Nature Publishing GroupCopyright Statement
- Country of Publication:
- United States
- Language:
- English
Web of Science
A low-background piston–cylinder-type hybrid high pressure cell for muon-spin rotation/relaxation experiments
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journal | September 2017 |
Electronic structure, phonon and superconductivity for WP 5 d -transition metal
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journal | November 2019 |
Multiple band crossings and Fermi surface topology: Role of double nonsymmorphic symmetries in MnP-type crystal structures
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journal | September 2019 |
High pressure research using muons at the Paul Scherrer Institute
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journal | March 2016 |
Why paramagnetic chiral correlations in the long wavelength limit do not contribute to muon-spin relaxation | text | January 2020 |
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