Electric polarization observed in single crystals of multiferroic Lu2MnCoO6

Chikara, Shalinee; Singleton, John; Bowlan, John M.; Yarotski, Dmitry Anatolievitch; Lee, N.; Choi, H. Y.; Choi, Y. J.; Zapf, Vivien S.

doi:10.1103/PhysRevB.93.180405

Title: Electric polarization observed in single crystals of multiferroic ${Lu}_{2} {MnCoO}_{6}$

Journal Article · Tue May 17 00:00:00 EDT 2016 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.93.180405· OSTI ID:1338804

Chikara, Shalinee ^[1]; Singleton, John ^[1]; Bowlan, John M. ^[1]; Yarotski, Dmitry Anatolievitch ^[1]; Lee, N. ^[2]; Choi, H. Y. ^[2]; Choi, Y. J. ^[2]; Zapf, Vivien S. ^[1]

Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Yonsei Univ., Seoul (South Korea)

We report electric polarization and magnetization measurements in single crystals of double perovskite Lu₂MnCoO₆ using pulsed magnetic fields and optical second harmonic generation in dc magnetic fields. We observe well-resolved magnetic field-induced changes in the electric polarization in single crystals and thereby resolve the question about whether multiferroic behavior is intrinsic to these materials or is an extrinsic feature of polycrystals. We find electric polarization along the crystalline b axis, that is suppressed by applying a magnetic fields along the c axis, and advance a model for the origin of magnetoelectric coupling. We furthermore map the phase diagram using both capacitance and electric polarization to identify regions of ordering and regions of magnetoelectric hysteresis. This compound is a rare example of coupled hysteretic behavior in the magnetic and electric properties. Furthermore, the ferromagneticlike magnetic hysteresis loop that couples to hysteretic electric polarization can be attributed not to ordinary ferromagnetic domains, but to the rich physics of magnetic frustration of Ising-like spins in the axial next-nearest-neighbor interaction model.

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Research Organization:: Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC52-06NA25396

OSTI ID:: 1338804

Alternate ID(s):: OSTI ID: 1253432

Report Number(s):: LA-UR-16-21949; PRBMDO

Journal Information:: Physical Review B, Vol. 93, Issue 18; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 24 works

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References (24)

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Magnetoelectric behavior via a spin state transition Chikara, Shalinee; Gu, Jie; Zhang, X. -G. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-11967-3	journal	September 2019
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Magnetocaloric effect and influence of Fe/Cr disorder on the magnetization reversal and dielectric relaxation in R Fe _0.5 Cr _0.5 O ₃ systems Yin, L. H.; Yang, J.; Tong, P. Applied Physics Letters, Vol. 110, Issue 19 https://doi.org/10.1063/1.4983363	journal	May 2017

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