Electrical resistance of single-crystal magnetite (Fe 3 O 4 ) under quasi-hydrostatic pressures up to 100 GPa

Muramatsu, Takaki; Gasparov, Lev V.; Berger, Helmuth; Hemley, Russell J.; Struzhkin, Viktor V.

doi:10.1063/1.4945388

Title: Electrical resistance of single-crystal magnetite (Fe ₃ O ₄ ) under quasi-hydrostatic pressures up to 100 GPa

Journal Article · Thu Apr 07 00:00:00 EDT 2016 · Journal of Applied Physics

DOI:https://doi.org/10.1063/1.4945388· OSTI ID:1364599

Muramatsu, Takaki ^[1];

^[2]; Berger, Helmuth ^[3]; Hemley, Russell J. ^[4]; Struzhkin, Viktor V. ^[1]

Carnegie Inst. of Washington, Washington, DC (United States). Geophysical Lab.
Univ. of North Florida, Jacksonville, FL (United States). Dept. of Physics
Ecole Polytechnique Federale Lausanne (Switzlerland)
Carnegie Inst. of Washington, Washington, DC (United States). Geophysical Lab.; Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

We measured the pressure dependence of electrical resistance of single-crystal magnetite (Fe₃O₄) under quasi-hydrostatic conditions to 100 GPa using low-temperature, megabar diamond-anvil cell techniques in order to gain insight into the anomalous behavior of this material that has been reported over the years in different high-pressure experiments. The measurements under nearly hydrostatic pressure conditions allowed us to detect the clear Verwey transition and the high-pressure structural phase. Furthermore, the appearance of a metallic ground state after the suppression of the Verwey transition around 20 GPa and the concomitant enhancement of electrical resistance caused by the structural transformation to the high-pressure phase form reentrant semiconducting-metallic-semiconducting behavior, though the appearance of the metallic phase is highly sensitive to stress conditions and details of the measurement technique.

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Research Organization:: Carnegie Inst. of Science, Washington, DC (United States); Energy Frontier Research Centers (EFRC) (United States). Energy Frontier Research in Extreme Environments (EFree)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: NA0002006; SC-0001057; FG02-02ER45955; FG02-99ER45775; AC52-07NA27344

OSTI ID:: 1364599

Alternate ID(s):: OSTI ID: 1246184

Journal Information:: Journal of Applied Physics, Vol. 119, Issue 13; ISSN 0021-8979

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 12 works

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References (33)

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A Room‐Temperature Verwey‐type Transition in Iron Oxide, Fe ₅ O ₆ Ovsyannikov, Sergey V.; Bykov, Maxim; Medvedev, Sergey A. Angewandte Chemie, Vol. 132, Issue 14 https://doi.org/10.1002/ange.201914988	journal	January 2020
A Room‐Temperature Verwey‐type Transition in Iron Oxide, Fe ₅ O ₆ Ovsyannikov, Sergey V.; Bykov, Maxim; Medvedev, Sergey A. Angewandte Chemie International Edition, Vol. 59, Issue 14 https://doi.org/10.1002/anie.201914988	journal	January 2020

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