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Title: Hierarchically structured catalysts for cascade and selective steam reforming/hydrodeoxygenation reactions

Abstract

We report a hierarchically structured catalyst with steam reforming and hydrodeoxygenation functionalities being deposited in the micropores and macropores, respectively. The catalyst is highly efficient to upgrade the pyrolysis vapors of pine forest product residual, resulting in a dramatically decreased acid content and increased hydrocarbon yield without external H2 supply.

Authors:
; ; ; ; ; ;
Publication Date:
Research Org.:
Pacific Northwest National Laboratory (PNNL), Richland, WA (US), Environmental Molecular Sciences Laboratory (EMSL)
Sponsoring Org.:
USDOE
OSTI Identifier:
1229988
Report Number(s):
PNNL-SA-114345
Journal ID: ISSN 1359-7345; 47660; KP1704020
DOE Contract Number:  
AC05-76RL01830
Resource Type:
Journal Article
Journal Name:
ChemComm
Additional Journal Information:
Journal Volume: 51; Journal Issue: 93; Journal ID: ISSN 1359-7345
Publisher:
Royal Society of Chemistry
Country of Publication:
United States
Language:
English
Subject:
Catalysts; hydrodeoxygenation; micropores; macropores; Environmental Molecular Sciences Laboratory

Citation Formats

Sun, Junming, Karim, Ayman M., Li, Xiaohong S., Rainbolt, James E., Kovarik, Libor, Shin, Yongsoon, and Wang, Yong. Hierarchically structured catalysts for cascade and selective steam reforming/hydrodeoxygenation reactions. United States: N. p., 2015. Web. doi:10.1039/C5CC07244A.
Sun, Junming, Karim, Ayman M., Li, Xiaohong S., Rainbolt, James E., Kovarik, Libor, Shin, Yongsoon, & Wang, Yong. Hierarchically structured catalysts for cascade and selective steam reforming/hydrodeoxygenation reactions. United States. doi:10.1039/C5CC07244A.
Sun, Junming, Karim, Ayman M., Li, Xiaohong S., Rainbolt, James E., Kovarik, Libor, Shin, Yongsoon, and Wang, Yong. Tue . "Hierarchically structured catalysts for cascade and selective steam reforming/hydrodeoxygenation reactions". United States. doi:10.1039/C5CC07244A.
@article{osti_1229988,
title = {Hierarchically structured catalysts for cascade and selective steam reforming/hydrodeoxygenation reactions},
author = {Sun, Junming and Karim, Ayman M. and Li, Xiaohong S. and Rainbolt, James E. and Kovarik, Libor and Shin, Yongsoon and Wang, Yong},
abstractNote = {We report a hierarchically structured catalyst with steam reforming and hydrodeoxygenation functionalities being deposited in the micropores and macropores, respectively. The catalyst is highly efficient to upgrade the pyrolysis vapors of pine forest product residual, resulting in a dramatically decreased acid content and increased hydrocarbon yield without external H2 supply.},
doi = {10.1039/C5CC07244A},
journal = {ChemComm},
issn = {1359-7345},
number = 93,
volume = 51,
place = {United States},
year = {2015},
month = {9}
}