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Title: Tailoring the electronic transitions of NdNiO3 films through (111)pc oriented interfaces

Journal Article · · APL Materials
DOI:https://doi.org/10.1063/1.4919803· OSTI ID:1229442
ORCiD logo [1];  [1];  [2]; ORCiD logo [3]; ORCiD logo [3];  [4];  [5];  [1];  [6];  [7];  [1]
  1. Univ. of Geneva (Switzerland)
  2. Paul Scherrer Inst. (PSI), Villigen (Switzerland); Brookhaven National Lab. (BNL), Upton, NY (United States)
  3. Canadian Light Source, Saskatoon, SK (Canada)
  4. Univ. of Geneva (Switzerland); Service de Physique de l’Etat Condensé (CNRS UMR 3680), Gif-sur-Yvette (France)
  5. Univ. of Geneva (Switzerland); Univ. College London (United Kingdom)
  6. Univ. of British Columbia, Vancouver, BC (Canada)
  7. Paul Scherrer Inst. (PSI), Villigen (Switzerland)

Bulk NdNiO3 and thin films grown along the pseudocubic (001)pc axis display a 1st order metal to insulator transition (MIT) together with a Néel transition at T = 200 K. Here, we show that for NdNiO3 films deposited on (111)pc NdGaO3, the MIT occurs at T = 335 K and the Néel transition at T = 230 K. By comparing transport and magnetic properties of layers grown on substrates with different symmetries and lattice parameters, we demonstrate a particularly large tuning when the epitaxy is realized on (111)pc surfaces. We attribute this effect to the specific lattice matching conditions imposed along this direction when using orthorhombic substrates.

Research Organization:
Brookhaven National Lab. (BNL), Upton, NY (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES); European Research Council (ERC); CFI; Natural Sciences and Engineering Research Council of Canada (NSERC); USNRC; CIHR; Government of Saskatchewan; WD Canada; University of Saskatchewan
Grant/Contract Number:
SC00112704
OSTI ID:
1229442
Report Number(s):
BNL-111518-2015-JA
Journal Information:
APL Materials, Vol. 3, Issue 6; ISSN 2166-532X
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 49 works
Citation information provided by
Web of Science

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Cited By (13)

Conductivity and Local Structure of LaNiO 3 Thin Films journal March 2017
Polar metals by geometric design journal April 2016
Striped nanoscale phase separation at the metal–insulator transition of heteroepitaxial nickelates journal November 2016
Structurally triggered metal-insulator transition in rare-earth nickelates journal November 2017
Complex magnetic order in nickelate slabs journal July 2018
Anisotropic suppression of octahedral breathing distortion with the fully strained BaBiO 3 /BaCeO 3 heterointerface journal January 2018
Rare-earth nickelates R NiO 3 : thin films and heterostructures journal February 2018
Distortion mode anomalies in bulk PrNiO 3 : Illustrating the potential of symmetry-adapted distortion mode analysis for the study of phase transitions journal November 2019
Controlled confinement of half-metallic two-dimensional electron gas in BaTiO 3 / Ba 2 FeReO 6 / BaTiO 3 heterostructures: A first-principles study journal October 2015
Multiple Supersonic Phase Fronts Launched at a Complex-Oxide Heterointerface journal January 2017
Complex magnetic order in nickelate slabs text January 2018
Epitaxial strain modulated electronic properties of interface controlled nickelate superlattice text January 2018
Complex magnetic order in nickelate slabs text January 2019