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Title: Models of the elastic x-ray scattering feature for warm dense aluminum

Journal Article · · Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics
 [1];  [1]
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

The elastic feature of x-ray scattering from warm dense aluminum has recently been measured by Fletcher et al. [Nature Photonics 9, 274 (2015)] with much higher accuracy than had hitherto been possible. This measurement is a direct test of the ionic structure predicted by models of warm dense matter. We use the method of pseudoatom molecular dynamics to predict this elastic feature for warm dense aluminum with temperatures of 1–100 eV and densities of 2.7–8.1g/cm3. We compare these predictions to experiments, finding good agreement with Fletcher et al. and corroborating the discrepancy found in analyses of an earlier experiment of Ma et al. [Phys. Rev. Lett. 110, 065001 (2013)]. Lastly, we also evaluate the validity of the Thomas-Fermi model of the electrons and of the hypernetted chain approximation in computing the elastic feature and find them both wanting in the regime currently probed by experiments.

Research Organization:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
AC52-06NA25396
OSTI ID:
1247299
Alternate ID(s):
OSTI ID: 1213946
Report Number(s):
LA-UR-15-23901; PLEEE8
Journal Information:
Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics, Vol. 92, Issue 3; ISSN 1539-3755
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 21 works
Citation information provided by
Web of Science

References (34)

X-Ray Thomson-Scattering Measurements of Density and Temperature in Shock-Compressed Beryllium journal March 2009
Equation of State Measurements of Warm Dense Carbon Using Laser-Driven Shock and Release Technique journal April 2014
Inelastic X-Ray Scattering from Shocked Liquid Deuterium journal December 2012
Observations of Continuum Depression in Warm Dense Matter with X-Ray Thomson Scattering journal April 2014
Electronic structure measurements of dense plasmas journal May 2004
Observations of Plasmons in Warm Dense Matter journal February 2007
Probing warm dense lithium by inelastic X-ray scattering journal October 2008
Measurements of Ionic Structure in Shock Compressed Lithium Hydride from Ultrafast X-Ray Thomson Scattering journal December 2009
Ultrabright X-ray laser scattering for dynamic warm dense matter physics journal March 2015
X-Ray Scattering Measurements of Strong Ion-Ion Correlations in Shock-Compressed Aluminum journal February 2013
Predictions of x-ray scattering spectra for warm dense matter journal February 2014
Ab Initio Simulations for the Ion-Ion Structure Factor of Warm Dense Aluminum journal April 2014
Evidence for out-of-equilibrium states in warm dense matter probed by x-ray Thomson scattering journal January 2015
Pseudoatom molecular dynamics journal January 2015
An equation of state for fully ionized hydrogen journal January 1990
One-component plasma structure factor in tabular form journal November 1983
Comments on the variational modified-hypernetted-chain theory for simple fluids journal February 1986
Description of strongly coupled Yukawa fluids using the variational modified hypernetted chain approach journal June 2004
Integral equation model for warm and hot dense mixtures journal September 2014
A simple method for determining the ionic structure of warm dense matter journal March 2014
Electronic and ionic structures of warm and hot dense matter journal January 2013
Accurate Homogeneous Electron Gas Exchange-Correlation Free Energy for Local Spin-Density Calculations journal February 2014
Equation of state and sound velocity of a helium plasma by Thomas-Fermi-Dirac molecular dynamics journal September 2006
Ion-ion dynamic structure factor of warm dense mixtures journal June 2015
Coupling strength in Coulomb and Yukawa one-component plasmas journal November 2014
Interaction of photons with plasmas and liquid metals - photoabsorption and scattering journal December 1999
X-ray Thomson scattering in high energy density plasmas journal December 2009
Screening of ionic cores in partially ionized plasmas within linear response journal June 2010
Ion structure in warm dense matter: Benchmarking solutions of hypernetted-chain equations by first-principle simulations journal January 2009
Behavior of the coupling parameter under isochoric heating in a high- Z plasma journal June 2013
Thomas-Fermi Z -scaling laws and coupling stabilization for plasmas journal December 2013
Out-of-equilibrium conditions in x-ray Thomson scattering experiments journal June 2015
Variational modified hypernetted-chain approximation for multicomponent liquids: Formalism and application to simple-liquid binary mixtures journal March 1992
The pair distribution functions of the liquid alkali metals journal January 1991

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