skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: When are surface plasmon polaritons excited in the Kretschmann-Raether configuration?

Journal Article · · Scientific Reports
DOI:https://doi.org/10.1038/srep09929· OSTI ID:1200853
 [1];  [2];  [1];  [1];  [1];  [1]
  1. Argonne National Lab. (ANL), Argonne, IL (United States)
  2. Argonne National Lab. (ANL), Argonne, IL (United States); Emory Univ., Atlanta, GA (United States)

It is widely believed that the reflection minimum in a Kretschmann-Raether experiment results from direct coupling into surface plasmon polariton modes. Our experimental results provide a surprising discrepancy between the leakage radiation patterns of surface plasmon polaritons (SPPs) launched on a layered gold/germanium film compared to the K-R minimum, clearly challenging this belief. We provide definitive evidence that the reflectance dip in K-R experiments does not correlate with excitation of an SPP mode, but rather corresponds to a particular type of perfectly absorbing (PA) mode. Results from rigorous electrodynamics simulations show that the PA mode can only exist under external driving, whereas the SPP can exist in regions free from direct interaction with the driving field. These simulations show that it is possible to indirectly excite propagating SPPs guided by the reflectance minimum in a K-R experiment, but demonstrate the efficiency can be lower by more than a factor of 3. We find that optimal coupling into the SPP can be guided by the square magnitude of the Fresnel transmission amplitude.

Research Organization:
Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-06CH11357
OSTI ID:
1200853
Journal Information:
Scientific Reports, Vol. 5, Issue 05; ISSN 2045-2322
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 46 works
Citation information provided by
Web of Science

References (42)

Random Laser Based on Waveguided Plasmonic Gain Channels journal October 2011
Plasmonic Waveguide Modes of Film-Coupled Metallic Nanocubes journal November 2013
Nonlinear plasmonics journal November 2012
Direct optical measurement of light coupling into planar waveguide by plasmonic nanoparticles journal November 2012
Enhancing surface plasmon polariton propagation lengths via coupling to asymmetric waveguide structures journal March 2008
Leakage radiation microscopy of surface plasmon polaritons journal April 2008
An Improved Virtual Mode Theory of ATR Experiments on Surface Polaritons. Application to Long-Range Surface Plasmon-Polaritons in Asymmetric Layer Structures journal September 1987
Surface-polariton-like waves guided by thin, lossy metal films journal April 1986
Surface Plasmons on Smooth and Rough Surfaces and on Gratings book January 1988
Critically coupled resonators in vertical geometry using a planar mirror and a 5 nm thick absorbing film journal January 2006
Controllable optical negative refraction and phase conjugation in graphite thin films journal May 2013
Thin-Film Optical Filters book March 2010
Surface Plasmon-Coupled Emission with Gold Films journal August 2004
Direct optical measurement of light coupling into planar waveguide by plasmonic nanoparticles text January 2012
Influence of spacer layer on enhancement of nanoplasmon-assisted random lasing journal April 2013
Surface plasmon–polariton amplifiers and lasers journal December 2011
Near-Field Second-Harmonic Generation Induced by Local Field Enhancement journal January 2003
Surface plasma waves in silver and gold journal September 1978
Nanometre optical coatings based on strong interference effects in highly absorbing media journal October 2012
Multilayer reflectors by molecular-beam epitaxy for resonance enhanced absorption in thin high-speed detectors journal March 1990
Directional surface plasmon-coupled emission: a new method for high sensitivity detection journal August 2003
Plasma Losses by Fast Electrons in Thin Films journal June 1957
Inhomogeneous Surface Plasmon Polaritons journal July 2014
Plasmonics: Fundamentals and Applications book January 2007
Ultra-thin perfect absorber employing a tunable phase change material journal November 2012
Optical Constants of the Noble Metals journal December 1972
Controlling Subnanometer Gaps in Plasmonic Dimers Using Graphene journal October 2013
Negative Refraction at Visible Frequencies journal April 2007
Near-Field Second-Harmonic Generation Induced by Local Field Enhancement text January 2003
Effect of Damping on Surface Plasmon Dispersion journal October 1973
Theory and Modeling of Plasmonic Structures journal December 2012
Ultra-confined Modes in Metal Nanoparticle Arrays for Subwavelength Light Guiding and Amplification journal February 2014
Lasing action in strongly coupled plasmonic nanocavity arrays journal June 2013
Leakage radiation microscopy of surface plasmon polaritons preprint January 2010
Unguided plasmon-mode resonance in optically excited thin film: exact modal description of Kretschmann–Raether experiment journal January 2013
Total Absorption in a Graphene Monolayer in the Optical Regime by Critical Coupling with a Photonic Crystal Guided Resonance journal March 2014
Toward parametric amplification in plasmonic systems: Second harmonic generation enhanced by surface plasmon polaritons journal January 2014
Surface plasmon interference excited by tightly focused laser beams journal January 2007
Interpretation of attenuated-total-reflection dips observed in surface plasmon resonance journal January 2007
Tunability of hybridized plasmonic waveguide mediated by surface plasmon polaritons journal January 2014
Thin-film optical filters journal August 1970
Principles of Nano-Optics book January 2012

Cited By (9)

Kretschmann-Raether configuration: Revision of the theory of resonant interaction journal October 2017
ZnO for performance enhancement of surface plasmon resonance biosensor: a review journal January 2020
Near‐field enhancements and surface plasmon polaritons with multifunctional oxide thin films journal August 2018
Corrugation-assisted metal-coated angled fiber facet for wavelength-dependent off-axis directional beaming journal January 2017
Towards the nonlinear acousto-magneto-plasmonics journal August 2016
Plasmonic layer-selective all-optical switching of magnetization with nanometer resolution journal October 2019
Dual-color near-field imaging by means of thin-film plasmonic waveguide with precise beam control of multiple wavelengths journal October 2019
Optical resonances in Kretschmann and Otto configurations journal January 2018
Influence of the dielectric substrate on the effective optical constants of silver plasmonic films journal January 2019

Figures / Tables (4)


Similar Records

When are Surface Plasmon Polaritons Excited in the Kretschmann-Raether Configuration?
Journal Article · Thu Apr 23 00:00:00 EDT 2015 · Scientific Reports · OSTI ID:1200853

Experimental analysis of waveguide-coupled surface-plasmon-polariton cone properties
Journal Article · Wed Sep 26 00:00:00 EDT 2018 · Analytica Chimica Acta · OSTI ID:1200853

Local excitation of strongly coupled exciton-surface plasmons polaritons by a single nanoantenna
Journal Article · Mon Jun 02 00:00:00 EDT 2014 · Applied Physics Letters · OSTI ID:1200853