Chemical pressure tuning of URu2Si2 via isoelectronic substitution of Ru with Fe

Das, Pinaki; Kanchanavatee, N.; Helton, J. S.; Huang, K.; Baumbach, R. E.; Bauer, E. D.; White, B. D.; Burnett, V. W.; Maple, M. B.; Lynn, J. W.; Janoschek, M.

doi:10.1103/PhysRevB.91.085122

Title: Chemical pressure tuning of ${URu}_{2} {Si}_{2}$ via isoelectronic substitution of Ru with Fe

Journal Article · Thu Feb 26 00:00:00 EST 2015 · Physical Review. B, Condensed Matter and Materials Physics

DOI:https://doi.org/10.1103/PhysRevB.91.085122· OSTI ID:1193437

Das, Pinaki ^[1]; Kanchanavatee, N. ^[2]; Helton, J. S. ^[3]; Huang, K. ^[2]; Baumbach, R. E. ^[4]; Bauer, E. D. ^[1]; White, B. D. ^[2]; Burnett, V. W. ^[2]; Maple, M. B. ^[2]; Lynn, J. W. ^[5]; Janoschek, M. ^[1]

Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Univ. of California, San Diego, La Jolla, CA (United States)
The United States Naval Academy, Annapolis, MD (United States); National Institute of Standards and Technology, Gaithersburg, MD (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Florida State Univ., Tallahassee, FL (United States)
National Institute of Standards and Technology, Gaithersburg, MD (United States)

We have used specific heat and neutron diffraction measurements on single crystals of URu_2–xFe_xSi₂ for Fe concentrations x ≤ 0.7 to establish that chemical substitution of Ru with Fe acts as “chemical pressure” P_ch as previously proposed by Kanchanavatee et al. [Phys. Rev. B 84, 245122 (2011)] based on bulk measurements on polycrystalline samples. Neutron diffraction reveals a sharp increase of the uranium magnetic moment at x = 0.1, reminiscent of the behavior at the “hidden order” to large moment antiferromagnetic (LMAFM) phase transition observed at a pressure P_x ≈ 0.5-0.7 GPa in URu₂Si₂. Using the unit cell volume determined from our measurements and an isothermal compressibility κ_T = 5.2×10⁻³ GPa⁻¹ for URu₂Si₂, we determine the chemical pressure P_ch in URu_2-xFe_xSi₂ as a function of x. The resulting temperature T-chemical pressure P_ch phase diagram for URu_2-xFe_xSi₂ is in agreement with the established temperature T-external pressure P phase diagram of URu₂Si₂.

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: FG02-04ER46105; DMR-0802478; AC52-06NA25396

OSTI ID:: 1193437

Alternate ID(s):: OSTI ID: 1179979

Report Number(s):: LA-UR-14-29641; PRBMDO

Journal Information:: Physical Review. B, Condensed Matter and Materials Physics, Vol. 91, Issue 8; ISSN 1098-0121

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 29 works

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References (50)

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Cited By (4)

NMR investigation of antiferromagnetism and coherence in ${URu}_{2} {Si}_{2 - x} P_{x}$ Shirer, K. R.; Lawson, M.; Kissikov, T. Physical Review B, Vol. 95, Issue 4 https://doi.org/10.1103/physrevb.95.041107	journal	January 2017
Single Crystal Growth of URu2Si2 by the Modified Bridgman Technique Gallagher, Andrew; Nelson, William; Chen, Kuan Crystals, Vol. 6, Issue 10 https://doi.org/10.3390/cryst6100128	journal	October 2016
Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu ₂ Si ₂ Mydosh, J. A.; Oppeneer, P. M.; Riseborough, P. S. Journal of Physics: Condensed Matter, Vol. 32, Issue 14 https://doi.org/10.1088/1361-648x/ab5eba	journal	January 2020
Pressure-induced rotational symmetry breaking in URu2Si2 Choi, J.; Ivashko, O.; Dennler, N. American Physical Society https://doi.org/10.5167/uzh-161743	text	January 2018

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