Monolayer PtSe 2 , a New Semiconducting Transition-Metal-Dichalcogenide, Epitaxially Grown by Direct Selenization of Pt

Wang, Yeliang; Li, Linfei; Yao, Wei; Song, Shiru; Sun, J. T.; Pan, Jinbo; Ren, Xiao; Li, Chen; Okunishi, Eiji; Wang, Yu-Qi; Wang, Eryin; Shao, Yan; Zhang, Y. Y.; Yang, Hai-tao; Schwier, Eike F.; Iwasawa, Hideaki; Shimada, Kenya; Taniguchi, Masaki; Cheng, Zhaohua; Zhou, Shuyun; Du, Shixuan; Pennycook, Stephen J.; Pantelides, Sokrates T.; Gao, Hong-Jun

doi:10.1021/acs.nanolett.5b00964

Title: Monolayer PtSe ₂ , a New Semiconducting Transition-Metal-Dichalcogenide, Epitaxially Grown by Direct Selenization of Pt

Journal Article · Thu May 21 00:00:00 EDT 2015 · Nano Letters

DOI:https://doi.org/10.1021/acs.nanolett.5b00964· OSTI ID:1185929

Wang, Yeliang ^[1]; Li, Linfei ^[2]; Yao, Wei ^[3]; Song, Shiru ^[2]; Sun, J. T. ^[2]; Pan, Jinbo ^[2]; Ren, Xiao ^[2]; Li, Chen ^[4]; Okunishi, Eiji ^[5]; Wang, Yu-Qi ^[2]; Wang, Eryin ^[3]; Shao, Yan ^[2]; Zhang, Y. Y. ^[6]; Yang, Hai-tao ^[2]; Schwier, Eike F. ^[7]; Iwasawa, Hideaki ^[7]; Shimada, Kenya ^[7]; Taniguchi, Masaki ^[7]; Cheng, Zhaohua ^[2]; Zhou, Shuyun ^[8] more »

Chinese Academy of Sciences (CAS), Beijing (China); Collaborative Innovation Center of Quantum Matter, Beijing (China)
Chinese Academy of Sciences (CAS), Beijing (China)
Tsinghua Univ., Beijing (China)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Jeol Ltd., Tokyo (Japan)
Chinese Academy of Sciences (CAS), Beijing (China); Vanderbilt Univ., Nashville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Hiroshima Univ., Higashi-Hiroshima (Japan)
Tsinghua Univ., Beijing (China); Collaborative Innovation Center of Quantum Matter, Beijing (China)
National Univ. of Singapore (Singapore)
Vanderbilt Univ., Nashville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Single-layer transition-metal dichalcogenides (TMDs) receive significant attention due to their intriguing physical properties for both fundamental research and potential applications in electronics, optoelectronics, spintronics, catalysis, and so on. Here, we demonstrate the epitaxial growth of high-quality single-crystal, monolayer platinum diselenide (PtSe2), a new member of the layered TMDs family, by a single step of direct selenization of a Pt(111) substrate. A combination of atomic-resolution experimental characterizations and first-principle theoretic calculations reveals the atomic structure of the monolayer PtSe2/Pt(111). Angle-resolved photoemission spectroscopy measurements confirm for the first time the semiconducting electronic structure of monolayer PtSe2 (in contrast to its semimetallic bulk counterpart). The photocatalytic activity of monolayer PtSe2 film is evaluated by a methylene-blue photodegradation experiment, demonstrating its practical application as a promising photocatalyst. Moreover, circular polarization calculations predict that monolayer PtSe2 has also potential applications in valleytronics.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Vanderbilt Univ., Nashville, TN (United States)

Sponsoring Organization:: USDOE Advanced Research Projects Agency - Energy (ARPA-E)

Grant/Contract Number:: AC05-00OR22725; FG02-09ER46554; 2013CBA01600; 2011CB932700; 61222112; 61390501; 5132504; 11334006; 1731300500015; XDB07030100; ACI-1053575

OSTI ID:: 1185929

Alternate ID(s):: OSTI ID: 1597683

Journal Information:: Nano Letters, Vol. 15, Issue 6; ISSN 1530-6984

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 506 works

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The Computational 2D Materials Database: high-throughput modeling and discovery of atomically thin crystals Haastrup, Sten; Strange, Mikkel; Pandey, Mohnish 2D Materials, Vol. 5, Issue 4 https://doi.org/10.1088/2053-1583/aacfc1	journal	September 2018
Atomically thin noble metal dichalcogenide: a broadband mid-infrared semiconductor Yu, Xuechao; Yu, Peng; Wu, Di Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-03935-0	journal	April 2018
Prospects of spintronics based on 2D materials: Spintronics Based on 2D Materials Feng, Yuan Ping; Shen, Lei; Yang, Ming Wiley Interdisciplinary Reviews: Computational Molecular Science, Vol. 7, Issue 5 https://doi.org/10.1002/wcms.1313	journal	April 2017
PtSe ₂ /graphene hetero-multilayer: gate-tunable Schottky barrier height and contact type Xia, Congxin; Du, Juan; Fang, Lizhen Nanotechnology, Vol. 29, Issue 46 https://doi.org/10.1088/1361-6528/aaddb9	journal	September 2018
Optical properties of chemical vapor deposition-grown PtSe ₂ characterized by spectroscopic ellipsometry Xie, Junfang; Zhang, Di; Yan, Xiao-Qing 2D Materials, Vol. 6, Issue 3 https://doi.org/10.1088/2053-1583/ab1490	journal	April 2019
Bilayer platinum diselenide saturable absorber for 20 μm passively Q-switched bulk lasers Yan, Bingzheng; Zhang, Baitao; Nie, Hongkun Optics Express, Vol. 26, Issue 24 https://doi.org/10.1364/oe.26.031657	journal	January 2018
Phase-Engineered PtSe ₂ -Layered Films by a Plasma-Assisted Selenization Process toward All PtSe ₂ -Based Field Effect Transistor to Highly Sensitive, Flexible, and Wide-Spectrum Photoresponse Photodetectors Su, Teng-Yu; Medina, Henry; Chen, Yu-Ze Small, Vol. 14, Issue 19 https://doi.org/10.1002/smll.201800032	journal	April 2018
Hybridization induced metallic and magnetic edge states in noble transition-metal-dichalcogenides of PtX ₂ (X = S, Se) nanoribbons Liu, Shan; Liu, Ziran Physical Chemistry Chemical Physics, Vol. 20, Issue 33 https://doi.org/10.1039/c8cp03640c	journal	January 2018
Temperature-dependent Raman spectroscopy and sensor applications of PtSe ₂ nanosheets synthesized by wet chemistry Pawar, Mahendra S.; Late, Dattatray J. Beilstein Journal of Nanotechnology, Vol. 10 https://doi.org/10.3762/bjnano.10.46	journal	January 2019
Intrinsically patterned two-dimensional materials for selective adsorption of molecules and nanoclusters Lin, X.; Lu, J. C.; Shao, Y. Nature Materials, Vol. 16, Issue 7 https://doi.org/10.1038/nmat4915	journal	June 2017
Vertically standing PtSe ₂ film: a saturable absorber for a passively mode-locked Nd:LuVO ₄ laser Tao, Lili; Huang, Xiaowen; He, Junshan Photonics Research, Vol. 6, Issue 7 https://doi.org/10.1364/prj.6.000750	journal	January 2018
Visualization of point defects in ultrathin layered 1T-PtSe ₂ Zheng, Husong; Choi, Yichul; Baniasadi, Fazel 2D Materials, Vol. 6, Issue 4 https://doi.org/10.1088/2053-1583/ab3beb	journal	September 2019
Controlled Doping of Wafer-Scale PtSe ₂ Films for Device Application Xu, Hu; Zhang, Haima; Liu, Yawen Advanced Functional Materials, Vol. 29, Issue 4 https://doi.org/10.1002/adfm.201805614	journal	December 2018
Review of mid-infrared mode-locked laser sources in the 2.0 μ m–3.5 μ m spectral region Ma, Jie; Qin, Zhipeng; Xie, Guoqiang Applied Physics Reviews, Vol. 6, Issue 2 https://doi.org/10.1063/1.5037274	journal	June 2019
Few-Layered PtS ₂ Phototransistor on h-BN with High Gain Li, Liang; Wang, Weike; Chai, Yang Advanced Functional Materials, Vol. 27, Issue 27 https://doi.org/10.1002/adfm.201701011	journal	May 2017
First-principles study on the gas sensing property of the Ge, As, and Br doped PtSe ₂ Zhang, Jing; Yang, Gui; Tian, Junlong Materials Research Express, Vol. 5, Issue 3 https://doi.org/10.1088/2053-1591/aab4e3	journal	March 2018
Van der Waals Heterostructures for High‐Performance Device Applications: Challenges and Opportunities Liang, Shi‐Jun; Cheng, Bin; Cui, Xinyi Advanced Materials https://doi.org/10.1002/adma.201903800	journal	October 2019
Fast, Self-Driven, Air-Stable, and Broadband Photodetector Based on Vertically Aligned PtSe ₂ /GaAs Heterojunction Zeng, Long-Hui; Lin, Sheng-Huang; Li, Zhong-Jun Advanced Functional Materials, Vol. 28, Issue 16 https://doi.org/10.1002/adfm.201705970	journal	February 2018
Inversion symmetry breaking induced triply degenerate points in orderly arranged PtSeTe family materials Xiao, R. C.; Cheung, C. H.; Gong, P. L. Journal of Physics: Condensed Matter, Vol. 30, Issue 24 https://doi.org/10.1088/1361-648x/aac298	journal	May 2018
High-Electron-Mobility and Air-Stable 2D Layered PtSe ₂ FETs Zhao, Yuda; Qiao, Jingsi; Yu, Zhihao Advanced Materials, Vol. 29, Issue 5 https://doi.org/10.1002/adma.201604230	journal	November 2016
Nonlinear Optical Signatures of the Transition from Semiconductor to Semimetal in PtSe ₂ Wang, Lei; Zhang, Saifeng; McEvoy, Niall Laser & Photonics Reviews, Vol. 13, Issue 8 https://doi.org/10.1002/lpor.201900052	journal	July 2019
In-situ fabrication of PtSe2/GaN heterojunction for self-powered deep ultraviolet photodetector with ultrahigh current on/off ratio and detectivity Zhuo, Ranran; Zeng, Longhui; Yuan, Huiyu Nano Research, Vol. 12, Issue 1 https://doi.org/10.1007/s12274-018-2200-z	journal	September 2018
Tunable giant Rashba-type spin splitting in PtSe ₂ /MoSe ₂ heterostructure Xiang, Longjun; Ke, Youqi; Zhang, Qingyun Applied Physics Letters, Vol. 115, Issue 20 https://doi.org/10.1063/1.5125303	journal	November 2019
Thickness dependent electronic properties of Pt dichalcogenides Villaos, Rovi Angelo B.; Crisostomo, Christian P.; Huang, Zhi-Quan npj 2D Materials and Applications, Vol. 3, Issue 1 https://doi.org/10.1038/s41699-018-0085-z	journal	January 2019
Ultrafast Carrier Dynamics and Bandgap Renormalization in Layered PtSe ₂ Wang, Gaozhong; Wang, Kangpeng; McEvoy, Niall Small, Vol. 15, Issue 34 https://doi.org/10.1002/smll.201902728	journal	July 2019
Bulk-structured PtSe ₂ for femtosecond fiber laser mode-locking Huang, Bin; Du, Lin; Yi, Qian Optics Express, Vol. 27, Issue 3 https://doi.org/10.1364/oe.27.002604	journal	January 2019
Tunable electron-phonon coupling superconductivity in platinum diselenide Cheng, Cai; Sun, Jia-Tao; Liu, Min Physical Review Materials, Vol. 1, Issue 7 https://doi.org/10.1103/physrevmaterials.1.074804	journal	December 2017
Q-switched and mode-locked Er-doped fiber laser using PtSe ₂ as a saturable absorber Zhang, Kang; Feng, Ming; Ren, Yangyang Photonics Research, Vol. 6, Issue 9 https://doi.org/10.1364/prj.6.000893	journal	January 2018
Ultrathin Layers of PdPX (X=S, Se): Two Dimensional Semiconductors for Photocatalytic Water Splitting Jing, Yu; Ma, Yandong; Wang, Yu Chemistry - A European Journal, Vol. 23, Issue 55 https://doi.org/10.1002/chem.201703683	journal	September 2017
Electrical devices from top-down structured platinum diselenide films Yim, Chanyoung; Passi, Vikram; Lemme, Max C. npj 2D Materials and Applications, Vol. 2, Issue 1 https://doi.org/10.1038/s41699-018-0051-9	journal	February 2018
Janus PtSSe and graphene heterostructure with tunable Schottky barrier Cao, Liemao; Ang, Yee Sin; Wu, Qingyun Applied Physics Letters, Vol. 115, Issue 24 https://doi.org/10.1063/1.5130756	journal	December 2019
Experimental evidence for type-II Dirac semimetal in ${PtSe}_{2}$ Zhang, Kenan; Yan, Mingzhe; Zhang, Haoxiong Physical Review B, Vol. 96, Issue 12 https://doi.org/10.1103/physrevb.96.125102	journal	September 2017
Observation of negative longitudinal magnetoresistance in the type-II Dirac semimetal ${PtSe}_{2}$ Li, Zhaoguo; Zeng, Yong; Zhang, Jicheng Physical Review B, Vol. 98, Issue 16 https://doi.org/10.1103/physrevb.98.165441	journal	October 2018
Controlled assembly of artificial 2D materials based on the transfer of oxo-functionalized graphene Hußmann, Marleen; Weintrub, Benjamin; Feicht, Patrick Freie Universität Berlin https://doi.org/10.17169/refubium-26715	text	January 2019
Controlled assembly of artificial 2D materials based on the transfer of oxo-functionalized graphene Hußmann, Marleen; Weintrub, Benjamin; Feicht, Patrick Nanoscale Advances, Vol. 2, Issue 1 https://doi.org/10.1039/c9na00594c	journal	January 2020
Lorentz-violating type-II Dirac fermions in transition metal dichalcogenide PtTe$_2$ Yan, Mingzhe; Huang, Huaqing; Zhang, Kenan arXiv https://doi.org/10.48550/arxiv.1607.03643	text	January 2016
Low-Temperature Eutectic Synthesis of PtTe2 with Weak Antilocalization and Controlled Layer Thinning Hao, Song; Zeng, Junwen; Xu, Tao arXiv https://doi.org/10.48550/arxiv.1808.02283	text	January 2018
Experimental Progress on Layered Topological Semimetals Ma, Junchao; Deng, Ke; Zheng, Lu arXiv https://doi.org/10.48550/arxiv.1902.06874	text	January 2019
PtSe2 grown directly on polymer foil for use as a robust piezoresistive sensor Boland, Conor S.; Coileáin, Cormac Ó; Wagner, Stefan arXiv https://doi.org/10.48550/arxiv.1903.11894	preprint	January 2019
Van der Waals heterostructures for high-performance device applications: challenges and opportunities Liang, Shi-Jun; Cheng, Bin; Cui, Xinyi arXiv https://doi.org/10.48550/arxiv.1912.10886	text	January 2019

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Title: Monolayer PtSe 2 , a New Semiconducting Transition-Metal-Dichalcogenide, Epitaxially Grown by Direct Selenization of Pt

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Title: Monolayer PtSe ₂ , a New Semiconducting Transition-Metal-Dichalcogenide, Epitaxially Grown by Direct Selenization of Pt