Magnetic ordering at anomalously high temperatures in Dy at extreme pressures

Lim, J.; Fabbris, G.; Haskel, D.; Schilling, J. S.

doi:10.1103/PhysRevB.91.045116

Title: Magnetic ordering at anomalously high temperatures in Dy at extreme pressures

Journal Article · Thu Jan 15 00:00:00 EST 2015 · Physical Review. B, Condensed Matter and Materials Physics

DOI:https://doi.org/10.1103/PhysRevB.91.045116· OSTI ID:1335454

Lim, J. ^[1]; Fabbris, G. ^[2]; Haskel, D. ^[3]; Schilling, J. S. ^[1]

Washington Univ., St. Louis, MO (United States)
Washington Univ., St. Louis, MO (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)

In an attempt to destabilize the magnetic state of the heavy lanthanide Dy, extreme pressures were applied in an electrical resistivity measurement to 157 GPa over the temperature range 1.3 - 295 K. The magnetic ordering temperature T_o and spin-disorder resistance R_sd of Dy, as well as the superconducting pair-breaking effect ΔT_c in Y(1 at.% Dy), are found to track each other in a highly non-monotonic fashion as a function of pressure. Above 73 GPa, the critical pressure for a 6% volume collapse in Dy, all three quantities increase sharply (dT_o=dP≃5.3 K/GPa), T_o appearing to rise above ambient temperature for P > 107 GPa. In contrast, T_o and ΔT_c for Gd and Y(0.5 at.% Gd), respectively, show no such sharp increase with pressure (dT_o=dP≃ 0.73 K/GPa). Altogether, these results suggest that extreme pressure transports Dy into an unconventional magnetic state with an anomalously high magnetic ordering temperature.

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Research Organization:: Carnegie Institution of Washington, Washington, D.C. (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: NA0002006; FC52-08NA28554; AC02-06CH11357

OSTI ID:: 1335454

Alternate ID(s):: OSTI ID: 1180135

Journal Information:: Physical Review. B, Condensed Matter and Materials Physics, Vol. 91, Issue 4; ISSN 1098-0121

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 20 works

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