Effects of Mg doping on the remarkably enhanced electrochemical performance of Na3V2(PO4)3 cathode materials for sodium ion batteries
Abstract
Na3V2-xMgx(PO4)3/C composites with different Mg2+ doping contents (x=0, 0.01, 0.03, 0.05, 0.07 and 0.1) were prepared by a facile sol-gel method. The doping effects on the crystal structure were investigated by XRD, XPS and EXAFS. The results show that low dose doping Mg2+ does not alter the structure of the material, and magnesium is successfully substituted for vanadium site. The Mg doped Na3V2-xMgx(PO4)3/C composites exhibit significant improvements on the electrochemistry performances in terms of the rate capability and cycle performance, especially for the Na3V1.95Mg0.05(PO4)3/C. For example, when the current density increased from 1 C to 30 C, the specific capacity only decreased from 112.5 mAh g-1 to 94.2 mAh g-1 showing very good rate capability. Moreover, even cycling at a high rate of 20 C, an excellent capacity retention of 81% is maintained from the initial value of 106.4 mAh g-1 to 86.2 mAh g-1 at the 50th cycle. Enhanced rate capability and cycle performance can be attributed to the optimized particle size, structural stability and enhanced ionic and electronic conductivity induced by Mg doping.
- Authors:
-
- Beijing Inst. of Technology, Beijing (China). Key Lab. of Environmental Science and Engineering, School of Chemical Engineering and Environment
- Brookhaven National Lab. (BNL), Upton, NY (United States). Chemistry Dept.
- Publication Date:
- Research Org.:
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE)
- OSTI Identifier:
- 1177849
- Report Number(s):
- BNL-107707-2015-JA; BNL-107707-2015-JAAM
Journal ID: ISSN 2050-7488; JMCAET; R&D Project: MA453MAEA; VT0301010
- Grant/Contract Number:
- AC02-98CH10886; 2015CB251100; NCET-12-0047; NCET-13-0033
- Resource Type:
- Journal Article: Accepted Manuscript
- Journal Name:
- Journal of Materials Chemistry. A
- Additional Journal Information:
- Journal Volume: 3; Journal Issue: 18; Journal ID: ISSN 2050-7488
- Publisher:
- Royal Society of Chemistry
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE
Citation Formats
Li, Hui, Yu, Xiqian, Bai, Ying, Wu, Feng, Wu, Chuan, Liu, Liang-Yu, and Yang, Xiao-Qing. Effects of Mg doping on the remarkably enhanced electrochemical performance of Na3V2(PO4)3 cathode materials for sodium ion batteries. United States: N. p., 2015.
Web. doi:10.1039/C5TA00277J.
Li, Hui, Yu, Xiqian, Bai, Ying, Wu, Feng, Wu, Chuan, Liu, Liang-Yu, & Yang, Xiao-Qing. Effects of Mg doping on the remarkably enhanced electrochemical performance of Na3V2(PO4)3 cathode materials for sodium ion batteries. United States. https://doi.org/10.1039/C5TA00277J
Li, Hui, Yu, Xiqian, Bai, Ying, Wu, Feng, Wu, Chuan, Liu, Liang-Yu, and Yang, Xiao-Qing. 2015.
"Effects of Mg doping on the remarkably enhanced electrochemical performance of Na3V2(PO4)3 cathode materials for sodium ion batteries". United States. https://doi.org/10.1039/C5TA00277J. https://www.osti.gov/servlets/purl/1177849.
@article{osti_1177849,
title = {Effects of Mg doping on the remarkably enhanced electrochemical performance of Na3V2(PO4)3 cathode materials for sodium ion batteries},
author = {Li, Hui and Yu, Xiqian and Bai, Ying and Wu, Feng and Wu, Chuan and Liu, Liang-Yu and Yang, Xiao-Qing},
abstractNote = {Na3V2-xMgx(PO4)3/C composites with different Mg2+ doping contents (x=0, 0.01, 0.03, 0.05, 0.07 and 0.1) were prepared by a facile sol-gel method. The doping effects on the crystal structure were investigated by XRD, XPS and EXAFS. The results show that low dose doping Mg2+ does not alter the structure of the material, and magnesium is successfully substituted for vanadium site. The Mg doped Na3V2-xMgx(PO4)3/C composites exhibit significant improvements on the electrochemistry performances in terms of the rate capability and cycle performance, especially for the Na3V1.95Mg0.05(PO4)3/C. For example, when the current density increased from 1 C to 30 C, the specific capacity only decreased from 112.5 mAh g-1 to 94.2 mAh g-1 showing very good rate capability. Moreover, even cycling at a high rate of 20 C, an excellent capacity retention of 81% is maintained from the initial value of 106.4 mAh g-1 to 86.2 mAh g-1 at the 50th cycle. Enhanced rate capability and cycle performance can be attributed to the optimized particle size, structural stability and enhanced ionic and electronic conductivity induced by Mg doping.},
doi = {10.1039/C5TA00277J},
url = {https://www.osti.gov/biblio/1177849},
journal = {Journal of Materials Chemistry. A},
issn = {2050-7488},
number = 18,
volume = 3,
place = {United States},
year = {Thu Jan 01 00:00:00 EST 2015},
month = {Thu Jan 01 00:00:00 EST 2015}
}
Web of Science
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Strategies to Build High‐Rate Cathode Materials for Na‐Ion Batteries
journal, June 2019
- Lv, Wei‐Jun; Huang, Zhigao; Yin, Ya‐Xia
- ChemNanoMat, Vol. 5, Issue 10
Simultaneously tuning cationic and anionic redox in a P2-Na 0.67 Mn 0.75 Ni 0.25 O 2 cathode material through synergic Cu/Mg co-doping
journal, January 2019
- Kong, Weijin; Gao, Rui; Li, Qingyuan
- Journal of Materials Chemistry A, Vol. 7, Issue 15
A Promising Carbon/g‐C 3 N 4 Composite Negative Electrode for a Long‐Life Sodium‐Ion Battery
journal, September 2019
- Weng, Guo‐Ming; Xie, Yu; Wang, Hang
- Angewandte Chemie International Edition, Vol. 58, Issue 39
Synthesis and electrochemical performance of Na 3− x Li x V 2 (PO 4 ) 3 /C as cathode materials for Li‐ion batteries
journal, July 2019
- Jia, Maomao; Zhang, Yanhui; Tian, Hualing
- International Journal of Energy Research, Vol. 43, Issue 11
Boron Substituted Na 3 V 2 (P 1−x B x O 4 ) 3 Cathode Materials with Enhanced Performance for Sodium-Ion Batteries
journal, January 2017
- Hu, Pu; Wang, Xiaofang; Wang, Tianshi
- Advanced Science, Vol. 4, Issue 2