Single-shot hyperspectral coherent Raman planar imaging in the range 0–4200 cm⁻¹

Bohlin, Alexis; Kliewer, Christopher J.

doi:10.1063/1.4900477

Title: Single-shot hyperspectral coherent Raman planar imaging in the range 0–4200 cm⁻¹

Journal Article · Mon Oct 20 00:00:00 EDT 2014 · Applied Physics Letters

DOI:https://doi.org/10.1063/1.4900477· OSTI ID:1163877

Bohlin, Alexis ^[1]; Kliewer, Christopher J. ^[1]

Sandia National Laboratories, Livermore, California 94550, USA

We propose a technique for ultrabroadband planar coherent Raman spectroscopy that enables wideband chemically selective mapping of molecular partition functions in the gas-phase within a single-laser-shot. A spectral region spanning 0–4200 cm⁻¹ is excited simultaneously, in principle allowing for coherent planar imaging of most all fundamental Raman-active modes. This unique instantaneous and spatially correlated assessment enables multiplexed studies of transient dynamical systems in a two-dimensional (2D) field. Here, we demonstrate single-laser-shot high temperature diagnostics of H₂, with spatially resolved 2D measurement of transitions of both the pure-rotational H₂ S-branch and the vibrational H₂ Q-branch, analyzing the temperature contour of a reacting fuel-species as it evolves at a flame-front.

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Research Organization:: Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC04-94AL85000

OSTI ID:: 1163877

Alternate ID(s):: OSTI ID: 1214601; OSTI ID: 1416452

Journal Information:: Applied Physics Letters, Journal Name: Applied Physics Letters Vol. 105 Journal Issue: 16; ISSN 0003-6951

Publisher:: American Institute of PhysicsCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 27 works

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Title: Single-shot hyperspectral coherent Raman planar imaging in the range 0–4200 cm⁻¹

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