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Title: An Alternative Mechanism for Accelerated Carbon Sequestration in Concrete

Abstract

The increased rate of carbon dioxide sequestration (carbonation) is desired in many primary and secondary life applications of concrete in order to make the life cycle of concrete structures more carbon neutral. Most carbonation rate studies have focused on concrete exposed to air under various conditions. An alternative mechanism for accelerated carbon sequestration in concrete was investigated in this research based on the pH change of waters in contact with pervious concrete which have been submerged in carbonate laden waters. The results indicate that the concrete exposed to high levels of carbonate species in water may carbonate faster than when exposed to ambient air, and that the rate is higher with higher concentrations. Validation of increased carbon dioxide sequestration was also performed via thermogravimetric analysis (TGA). It is theorized that the proposed alternative mechanism reduces a limiting rate effect of carbon dioxide dissolution in water in the micro pores of the concrete.

Authors:
;
Publication Date:
Research Org.:
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1136593
Report Number(s):
PNNL-SA-93506
DOE Contract Number:
AC05-76RL01830
Resource Type:
Journal Article
Resource Relation:
Journal Name: Sustainable Cities and Society, 12:25-30
Country of Publication:
United States
Language:
English
Subject:
Cement; Carbonation; pH

Citation Formats

Haselbach, Liv M., and Thomle, Jonathan N.. An Alternative Mechanism for Accelerated Carbon Sequestration in Concrete. United States: N. p., 2014. Web. doi:10.1016/j.scs.2014.01.001.
Haselbach, Liv M., & Thomle, Jonathan N.. An Alternative Mechanism for Accelerated Carbon Sequestration in Concrete. United States. doi:10.1016/j.scs.2014.01.001.
Haselbach, Liv M., and Thomle, Jonathan N.. 2014. "An Alternative Mechanism for Accelerated Carbon Sequestration in Concrete". United States. doi:10.1016/j.scs.2014.01.001.
@article{osti_1136593,
title = {An Alternative Mechanism for Accelerated Carbon Sequestration in Concrete},
author = {Haselbach, Liv M. and Thomle, Jonathan N.},
abstractNote = {The increased rate of carbon dioxide sequestration (carbonation) is desired in many primary and secondary life applications of concrete in order to make the life cycle of concrete structures more carbon neutral. Most carbonation rate studies have focused on concrete exposed to air under various conditions. An alternative mechanism for accelerated carbon sequestration in concrete was investigated in this research based on the pH change of waters in contact with pervious concrete which have been submerged in carbonate laden waters. The results indicate that the concrete exposed to high levels of carbonate species in water may carbonate faster than when exposed to ambient air, and that the rate is higher with higher concentrations. Validation of increased carbon dioxide sequestration was also performed via thermogravimetric analysis (TGA). It is theorized that the proposed alternative mechanism reduces a limiting rate effect of carbon dioxide dissolution in water in the micro pores of the concrete.},
doi = {10.1016/j.scs.2014.01.001},
journal = {Sustainable Cities and Society, 12:25-30},
number = ,
volume = ,
place = {United States},
year = 2014,
month = 7
}