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Ultra-fast laser system

Patent ·
OSTI ID:1117845
;
A laser system is provided which selectively excites Raman active vibrations in molecules. In another aspect of the present invention, the system includes a laser, pulse shaper and detection device. A further aspect of the present invention employs a femtosecond laser and binary pulse shaping (BPS). Still another aspect of the present invention uses a laser beam pulse, a pulse shaper and remote sensing.
Research Organization:
Board of Trustees of Michigan State University, East Lansing, MI, USA
Sponsoring Organization:
USDOE
DOE Contract Number:
FG02-01ER15143
Assignee:
Board of Trustees of Michigan State University (East Lansing, MI)
Patent Number(s):
8,633,437
Application Number:
11/883,703
OSTI ID:
1117845
Country of Publication:
United States
Language:
English

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Vibrational ladder climbing in NO by ultrashort infrared laser pulses journal May 1997
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Acousto-optic femtosecond pulse shaping in the ultraviolet conference January 2005
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A new high-resolution femtosecond pulse shaper journal April 2001
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Holy Grails of Chemistry journal March 1995
Femtosecond dynamics of photoinduced molecular detachment from halogenated alkanes. II. Asynchronous concerted eliminationof I2 from CH2I2 journal September 1998
Discrete Intensity Jumps and Intramolecular Electronic Energy Transfer in the Spectroscopy of Single Conjugated Polymer Molecules journal August 1997
Two-dimensional nonlinear optics using Fourier-transform spectral interferometry journal January 1996
Adaptive femtosecond pulse compression journal January 1997
The dynamics of small molecules in intense laser fields journal April 2004
Laser coherent control of molecular chiral states via entanglement of the rotational and torsional degrees of freedom
  • Bychkov, Stanislav S.; Grishanin, Boris A.; Zadkov, Victor N.
  • Journal of Raman Spectroscopy, Vol. 33, Issue 11-12, p. 962-973 https://doi.org/10.1002/jrs.939
journal January 2002
Coherent control of the population transfer in complex solvated molecules at weak excitation. An experimental study
  • Prokhorenko, Valentyn I.; Nagy, Andrea M.; Miller, R. J. Dwayne
  • The Journal of Chemical Physics, Vol. 122, Issue 18, Article No. 184502 https://doi.org/10.1063/1.1886750
journal May 2005
Femtosecond spectrally dispersed three-pulse four-wave mixing: the role of sequence and chirp in controlling intramolecular dynamics journal January 2000
Frequency-resolved optical gating using cascaded second-order nonlinearities journal January 1998
Laser control of chemical reactions journal January 2002
Bond selective photochemistry in CH2BrI through electronic excitation at 210 nm journal April 1986
Photodynamic therapeutics basic principles and clinical applications journal November 1999
Chirped-pulse amplification of 85-fs pulses at 250 kHz with third-order dispersion compensation by use of holographic transmission gratings journal January 1994
Laser scanning third-harmonic-generation microscopy in biology journal January 1999
Fully quantum coherent control journal June 2001
Phase Defects in Self-Focusing of Ultrashort Pulses journal July 1999
Adaptive pulse shaping of phase and amplitude of an amplified femtosecond pulse laser by direct reference to frequency-resolved optical gating traces journal January 2002
Large interference effects of small chirp observed in two-photon absorption journal July 1992
Chirp measurement of large-bandwidth femtosecond optical pulses using two-photon absorption journal August 1991
Use of coherent control for selective two-photon fluorescence microscopy in live organisms journal January 2006
Simultaneous phase control of Li2 wave packets in two electronic states journal January 2002
Generation of 18-fs, multiterawatt pulses by regenerative pulse shaping and chirped-pulse amplification journal January 1996
Interference Effects in the Multiphoton Ionization of Sodium journal February 1995
Programmable femtosecond pulse shaping by use of a multielement liquid-crystal phase modulator journal January 1990
Nonlinear polarization description of phase‐locked pulse‐pair spectroscopy journal October 1992
Spectral phase correlation of coded femtosecond pulses by second-harmonic generation in thick nonlinear crystals journal January 2000
Using time-dependent rate equations to describe chirped pulse excitation in condensed phases journal March 1999
Phase dependence of intense-field ionization journal November 1996
Study of pulse compression from 1.5 μm distributed feedback lasers by a gires-tournois interferometer journal January 1994
Two-dimensional Fourier transform electronic spectroscopy journal October 2001
Theoretical study on quantum control of photodissociation and photodesorption dynamics by femtosecond chirped laser pulses journal April 1999
Quantum Control of Molecular Dynamics: The Strong Response Regime journal September 1995
Photon echo pulse sequences with femtosecond shaped laser pulses as a vehicle for molecule-based quantum computation journal January 2002
Controlling the Phase Evolution of Few-Cycle Light Pulses journal July 2000
Optical fibre-grating pulse compressors journal March 1988
Single-shot measurement of the intensity and phase of a femtosecond UV laser pulse with frequency-resolved optical gating journal January 1994
Femtosecond dynamics of photoinduced molecular detachment from halogenated alkanes. I. Transition state dynamics and product channel coherence journal September 1998
Coherent Laser Control of the Product Distribution Obtained in the Photoexcitation of HI journal October 1995
Time-resolved organometallic photochemistry: Femtosecond fragmentation and adaptive control of CpFe(CO)2X (X=Cl, Br, I) journal November 2002
Femtosecond real‐time probing of reactions. I. The technique journal November 1988
Dynamics of two-photon absorption by molecules and solutions journal January 2002
Single-shot measurement of carrier-envelope phase changes by spectral interferometry journal January 2001
Saturation of wave-packet interferences: Direct observation of spin precession in potassium atoms journal September 1999
Blue-shifted third-harmonic generation and correlated self-guiding during ultrafast barrier suppression ionization of subatmospheric density noble gases journal January 1996
Efficient population transfer in a three-level ladder system by frequency-swept ultrashort laser pulses journal October 1992
Population and coherence control by three-pulse four-wave mixing journal September 1999
Femtosecond pump–probe photoelectron spectroscopy on Na2: a tool to study basic coherent control schemes journal September 2000
Adsorption and surface-enhanced Raman of dyes on silver and gold sols journal August 1982
Multiphoton Intrapulse Interference. 1. Control of Multiphoton Processes in Condensed Phases journal October 2002
Femtosecond Pulse Sequences Used for Optical Manipulation of Molecular Motion journal March 1990
Laser science: Physics at the attosecond frontier journal November 2001
Coherent learning control of vibrational motion in room temperature molecular gases journal August 2001
Generation of narrowband inversion with broadband laser pulses journal March 1992
Quantum Control of Population Transfer in Green Fluorescent Protein by Using Chirped Femtosecond Pulses
  • Bardeen, Christopher J.; Yakovlev, Vladislav V.; Squier, Jeff A.
  • Journal of the American Chemical Society, Vol. 120, Issue 50, p. 13023-13027 https://doi.org/10.1021/ja9824627
journal December 1998
Rotational interference in vibrational ladder climbing in NO by chirped infrared laser pulses journal August 1999
Concerted elimination dynamics from highly excited states journal January 1997
Time and frequency-Gated FID a new approach to study the vibrational dephasing of water book January 2001
Multipulse interferometric frequency-resolved optical gating journal April 1999
Optimal Control of Molecular Motion: Design, Implementation, and Inversion journal August 2000
C OHERENT N ONLINEAR S PECTROSCOPY : From Femtosecond Dynamics to Control journal October 2001
Adaptive real-time femtosecond pulse shaping journal January 1998
Chirped multilayer coatings for broadband dispersion control in femtosecond lasers journal January 1994
Single-pulse coherently controlled nonlinear Raman spectroscopy and microscopy journal August 2002
High power ultrafast lasers journal March 1998
Population transfer via adiabatic passage in the rubidium quantum ladder system journal February 1999
Selective Bond Dissociation and Rearrangement with Optimally Tailored, Strong-Field Laser Pulses journal March 2001
Detection and control of molecular quantum dynamics
Characterization and optimization of a laser-scanning microscope in the femtosecond regime journal July 1998
Competing isomeric product channels in the 193 nm photodissociation of 2-chloropropene and in the unimolecular dissociation of the 2-propenyl radical journal January 2001
Selective preparation of enantiomers from a racemate by laser pulses: model simulation for oriented atropisomers with coupled rotations and torsions journal June 2001
Autocorrelation measurement of 6-fs pulses based on the two-photon-induced photocurrent in a GaAsP photodiode journal January 1997
Molecular dynamics: Optical control of reactions journal February 2000
Coherent Control of Femtosecond Energy Localization in Nanosystems journal January 2002
High-resolution, ultrafast laser pulse shaping and its applications book January 1997
Generation of Broadband VUV Light Using Third-Order Cascaded Processes journal June 2001
Nonlinear pulse shaping and causality journal January 1993
Precision and consistency criteria in spectral phase interferometry for direct electric-field reconstruction journal January 2002
Compression of optical solitons by conversion of nonlinear modes journal January 1995
Intense femtosecond laser field-induced Coulomb fragmentation of C2H4 journal March 2005
Generation of programmable, picosecond-resolution shaped laser pulses by fiber-grating pulse compression journal January 1987
Single-shot measurement of the amplitude and phase of ultrashort laser pulses in the violet journal January 1995
Dependence of the Laser Two-Photon Ionization Process in Solution on the Laser Pulse Width journal May 2001
Temporal coherent control induced by wave packet interferences in one and two photon atomic transitions journal June 1998
Encoding and decoding of femtosecond pulses journal January 1988
Implementation of Quantum Search Algorithm using Classical Fourier Optics journal March 2002
Quantum control of the yield of a chemical reaction journal March 1998
Acousto-optical shaping of ultraviolet femtosecond pulses journal March 2005
Molecular π pulses: Population inversion with positively chirped short pulses journal August 2000
General method for ultrashort light pulse chirp measurement journal June 1989
Generation, shaping, and characterization of intense femtosecond pulses tunable from 3 to 20 μm journal January 2000
Intrapulse Dynamical Effects in Multiphoton Processes: Theoretical Analysis journal June 1998
Vibrational ladder climbing in NO by (sub)picosecond frequency-chirped infrared laser pulses journal June 1998
Second-harmonic generation frequency-resolved optical gating in the single-cycle regime journal April 1999
Direct measurement of the two-point field correlation function journal January 1996
Selective bond fission in methyl mercaptan at 193 nm via radial derivative coupling between the 2 1A‘ and 1 1A‘ adiabatic electronic states journal March 1992
Switched Wave Packets: A Route to Nonperturbative Quantum Control journal June 2003
Femtosecond Imaging of Surface Plasmon Dynamics in a Nanostructured Silver Film journal June 2005
Determining the absolute carrier phase of a few-cycle laser pulse journal January 2000
Generation of 21-fs millijoule-energy pulses by use of Ti:sapphire journal January 1994
Femtosecond real‐time probing of reactions. V. The reaction of IHgI journal December 1989
Highly sensitive two-photon chromophores applied to three-dimensional lithographic microfabrication: design, synthesis and characterization towards two-photon absorption cross section journal January 2004
Temporal interferometric measurement of femtosecond spectral phase journal January 1996
Single-shot measurement of the intensity and phase of an arbitrary ultrashort pulse by using frequency-resolved optical gating journal January 1993
Spectral interferometry of semiconductor nanostructures journal April 1999
Propagation of Complex Laser Pulses in Optically Dense Media journal May 1999
Multidimensional Holography by Persistent Spectral Hole Burning journal April 2002
Coherent control improves biomedical imaging with ultrashort shaped pulses journal June 2006
Femtosecond pulse shaping by dynamic holograms in photorefractive multiple quantum wells journal January 1997
Real‐time femtosecond probing of ‘‘transition states’’ in chemical reactions journal August 1987
Nonresonant Control of Multimode Molecular Wave Packets at Room Temperature journal January 2002
Mechanisms for laser control of chemical reactions journal March 2002
Coherence control using the ratio of Rabi frequencies for complete coherent inversion in a four-level λ system journal January 1999
Multiphoton Intrapulse Interference 3: Probing Microscopic Chemical Environments journal January 2004
Mass-correlated pulsed extraction: Theoretical analysis and implementation with a linear matrix-assisted laser desorption/ionization time of flight mass spectrometer journal October 2000
Feedback-controlled optimization of amplified femtosecond laser pulses journal February 1999
Frequency doubling of phase-modulated, ultrashort laser pulses journal September 2001
Quantum control of I2 in the gas phase and in condensed phase solid Kr matrix journal May 1997
Ultrafast Probing and Control of Molecular Dynamics: Beyond the Pump-Probe Method book October 2001
Generation of high energy 10 fs pulses by a new pulse compression technique journal May 1996
Measurement of electric field by interferometric spectral trace observation journal January 2005
Coherent quantum control of two-photon transitions by a femtosecond laser pulse journal November 1998
Femtosecond Phase-Coherent Two-Dimensional Spectroscopy journal June 2003
Analysis and control of laser induced fragmentation processes in CpMn(CO)3 journal June 2001
Coherent ultrafast MI-FROG spectroscopy of optical field ionization in molecular H2, N2, and O2 journal July 2001
Observation of quasi-Landau wave packets journal June 1994
Elucidation of Control Mechanisms Discovered during Adaptive Manipulation of [Ru(dpb)3](PF6)2 Emission in the Solution Phase journal March 2007
Chirped pulse enhancement of multiphoton absorption in molecular iodine
  • Yakovlev, Vladislav V.; Bardeen, Christopher J.; Che, Jianwe
  • The Journal of Chemical Physics, Vol. 108, Issue 6, p. 2309-2313 https://doi.org/10.1063/1.475615
journal February 1998
Programmable dispersion compensation and pulse shaping in a 26-fs chirped-pulse amplifier journal January 1998
Open and closed loop control of complex molecules with shaped fs pulses conference January 2003
Amplitude and phase measurement of mid-infrared femtosecond pulses by using cross-correlation frequency-resolved optical gating journal January 2000
Locally designed pulse shaping for selective preparation of enantiomers from their racemate journal January 2001
Sequences for controlling laser excitation with femtosecond three-pulse four-wave mixing journal January 1999
Femtosecond optical pulse shaping and processing journal January 1995
Shaping of femtosecond pulses using phase-only filters designed by simulated annealing journal January 1993
Quantum control of coherent anti-Stokes Raman processes journal April 2002
Selective two-photon microscopy with shaped femtosecond pulses journal January 2003
Closing the Loop on Bond Selective Chemistry Using Tailored Strong Field Laser Pulses journal July 2002
High-Resolution Raman Spectra with Femtosecond Pulses: An Example of Combined Time- and Frequency-Domain Spectroscopy journal December 2006
Measurement of the Page function of an ultrashort laser pulse journal October 2001
Pulse shaping and coherent Raman spectroscopy in condensed phases journal January 1991
Development of automatically optimizing system of both spatial and temporal beam shaping for UV-laser pulse journal March 2004
Molecular “π Pulse” for Total Inversion of Electronic State Population journal February 1998
A femtosecond code-division multiple-access communication system test bed journal January 1998
Characterization of chirped-pulse amplification systems with spectral phase interferometry for direct electric-field reconstruction journal June 2000
New Photopolymers Based on Two-Photon Absorbing Chromophores and Application to Three-Dimensional Microfabrication and Optical Storage journal January 1997
Use of coherent control methods through scattering biological tissue to achieve functional imaging journal November 2004
No loss spectral phase correction and arbitrary phase shaping of regeneratively amplified femtosecond pulses using MIIPS journal January 2006
Directly measuring the spatio-temporal electric field of focusing ultrashort pulses journal January 2007
Interferometric observation of femtosecond free induction decay journal January 1994
Spatial and temporal dependence of interspark interactions in femtosecond-nanosecond dual-pulse laser-induced breakdown spectroscopy journal January 2004
Rapid measurement of ultrashort-pulse amplitude and phase from a two-photon absorption sonogram trace journal January 2001
Feedback-controlled femtosecond pulse shaping journal June 2000
Amplification of tailored white-light continuum journal June 2002
Two‐photon wave‐packet interferometry journal April 1994
High-ratio Electro-optical Data Compression for Massive Accessing Networks Using AOM-based Ultrafast Pulse Shaping journal January 2001
Quantum Control by Ultrafast Polarization Shaping journal May 2004
Time–frequency imaging of a single ultrashort light pulse from angularly resolved autocorrelation journal January 1995
Wavepacket diagnosis with chirped probe pulses journal August 1998
Absolute-phase phenomena in photoionization with few-cycle laser pulses journal November 2001
Nontrivial polarization shaping of femtosecond pulses by reference to the results of dual-channel spectral interferometry journal January 2004
Ultrabroadband femtosecond lasers journal April 1994
Direct measurement of pulse distortion near the zero-dispersion wavelength in an optical fiber by frequency-resolved optical gating journal January 1997
Generation of ultrahigh peak power pulses by chirped pulse amplification journal February 1988
Control of elementary chemical reactions by femtosecond light pulses journal June 2001
Ultrashort pulse generation by intracavity spectral shaping and phase compensation of external-cavity modelocked semiconductor lasers journal September 2000
Direct measurement of the spectral phase of femtosecond pulses journal January 1995
Application of a multilevel Redfield theory to electron transfer in condensed phases journal April 1992
Heterodyne detection of the complete electric field of femtosecond four-wave mixing signals journal January 1998
Information Storage and Retrieval Through Quantum Phase journal January 2000
Phase and intensity characterization of femtosecond pulses from a chirped-pulse amplifier by frequency-resolved optical gating journal January 1995
Adaptive compression of tunable pulses from a non-collinear-type OPA to below 16 fs by feedback-controlled pulse shaping journal June 2000
Subfemtosecond compression of periodic laser pulses journal January 1999
Nonlinear limits to the information capacity of optical fibre communications journal June 2001
Phase and amplitude control in the formation and detection of rotational wave packets in the E1Σg+ state of Li2 journal June 1998
Phase control of wavepacket dynamics using shaped femtosecond pulses journal January 1999
Evaluation of femtosecond pulse shaping with low-loss phase-only masks journal January 1998
Quantitative investigation of the multiphoton intrapulse interference phase scan method for simultaneous phase measurement and compensation of femtosecond laser pulses journal January 2006
Comment on “Time-resolved laser induced harpoon reactions’’ journal March 1997
Optimal control of one- and two-photon transitions with shaped femtosecond pulses and feedback journal September 2000
Analysis of a method of phase measurement of ultrashort pulses in the frequency domain journal May 1991
Quantum Control of NaI Photodissociation Reaction Product States by Ultrafast Tailored Light Pulses journal May 1997
Optical control of molecular dynamics: Molecular cannons, reflectrons, and wave‐packet focusers journal November 1993
Optimal control of quantum-mechanical systems: Existence, numerical approximation, and applications journal June 1988
Techniques for the characterization of sub-10-fs optical pulses a comparison journal June 2000
Programmable phase and amplitude femtosecond pulse shaping journal January 1993
Femtosecond Dynamics of Unimolecular and Unrestricted Bimolecular Reactions journal June 1998
The criterion of pulse reconstruction quality based on Wigner representation journal June 2000
Realization of a Time-Domain Fresnel Lens with Coherent Control journal October 2002
Propagation of intense, ultrashort laser pulses through metal vapor: refraction-limited behavior for single pulses journal January 1996
Femtosecond photoassociation spectroscopy: coherent bond formation journal November 1995
Amplitude and phase characterization of 45-fs pulses by frequency-resolved optical gating journal January 1998
Additive-pulse-compression mode locking of a neodymium fiber laser journal January 1991
Femtosecond photoassociation: Coherence and implications for control in bimolecular reactions journal May 1997
Mode-locking matter with light journal December 1993
Cascaded free-induction decay four-wave mixing journal May 2001
How to measure the amplitude and phase of an ultrashort light pulse with an autocorrelator and a spectrometer journal January 1994
Noise sensitivity in frequency-resolved optical-gating measurements of ultrashort pulses journal January 1995
Observation of Coherent Transients in Ultrashort Chirped Excitation of an Undamped Two-Level System journal June 2001
Innovative pulse shaping for high-performance wireless TDMA journal September 2001
Disentangling multidimensional femtosecond spectra of excitons by pulse shaping with coherent control journal May 2004
Using phase retrieval to measure the intensity and phase of ultrashort pulses: frequency-resolved optical gating journal January 1993
Narrow-Band Coherent Anti-Stokes Raman Signals from Broad-Band Pulses journal January 2002
Algorithm for complete and rapid retrieval of ultrashort pulse amplitude and phase from a sonogram journal January 1999
Programmable shaping of ultrabroad-bandwidth pulses from a Tisapphire laser journal January 1995
Quantum mechanics in terms of non-negative smoothed Wigner functions journal August 1992
Phase-matched third-harmonic generation by nonlinear phase shift in a hollow fiber journal July 1998
Probing microscopic chemical environments with high-intensity chirped pulses journal January 1999
Laser pulse control of Raman processes by chirped non-adiabatic passage journal January 2000
Control of Feshbach resonances by quantum interference journal July 2002
Interference effects in femtosecond spectroscopy journal May 2002
Visible pulse compression to 4 fs by optical parametric amplification and programmable dispersion control journal January 2002
Fluorescence‐detected wave packet interferometry. II. Role of rotations and determination of the susceptibility journal March 1992
Incorporating physical implementation concerns into closed loop quantum control experiments journal December 2000
Spectral phase transfer for indirect phase control of sub-20-fs deep UV pulses journal January 2005
Complete femtosecond linear free induction decay, Fourier algorithm for dispersion relations, and accuracy of the rotating wave approximation journal January 2001
Single-Pulse Phase-Contrast Nonlinear Raman Spectroscopy journal December 2002
Two-photon laser precision microfabrication and its applications to micro-nano devices and systems journal March 2003
Optimally shaped terahertz pulses for phase retrieval in a Rydberg-atom data register journal August 2001
Femtosecond Quantum Control journal January 2001
A theoretical study on laser control of a molecular nonadiabatic process by ultrashort chirped laser pulses journal August 1998
Observation of Plasmon Propagation, Redirection, and Fan-Out in Silver Nanowires journal August 2006
Spectral holography of shaped femtosecond pulses journal January 1992
Controlling molecular ground-state dissociation by optimizing vibrational ladder climbing journal February 2003
Frequency-time and time-space mappings for single-shot coherent four-wave mixing with chirped pulses and broad beams journal January 2001
Design and interpretation of laser pulses for the control of quantum systems journal September 2000
Adaptive Pulse Shaping of Femtosecond Laser Pulses in Amplitude and Phase through a Single-Mode Fiber by Referring to Frequency-Resolved Optical Gating Patterns journal June 2002
Control of HOD photodissociation dynamics via bond‐selective infrared multiphoton excitation and a femtosecond ultraviolet laser pulse journal December 1992
Large-ratio stretch and recompression of sub-10-fs pulses utilizing dispersion managed devices and a spatial light modulator journal June 2002
Sensing and compensation of femtosecond waveform distortion induced by all-order polarization mode dispersion at selected polarization states journal January 2007
Quantum Control of the Angular Momentum Distribution in Multiphoton Absorption Processes journal March 2004
Femtosecond pulse shaping with a stratified diffractive structure journal November 2000
Temporal Coherent Control in Two-Photon Transitions: From Optical Interferences to Quantum Interferences journal April 1997
Phase Dependence of Intense Field Ionization: A Study Using Two Colors journal September 1994
Nonadiabatic wave packet dynamics: Experiment and theory in IBr journal February 1999
Pump-dump control and the related transient absorption spectroscopies journal April 1999
Femtosecond pulse shaping with space-to-time conversion based on planar optics journal January 2007

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