Entangled valence electron-hole dynamics revealed by stimulated attosecond x-ray Raman scattering
Journal Article
·
· Journal of Physical Chemistry Letters, 3(17):2326-2331
We show that broadband x-ray pulses can create wavepackets of valence electrons and holes localized in the vicinity of a selected atom (nitrogen, oxygen or sulfur in cysteine) by resonant stimulated Raman scattering. The subsequent dynamics reveals highly correlated motions of entangled electrons and hole quasiparticles. This information goes beyond the time-dependent total charge density derived from x-ray diffraction.
- Research Organization:
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States). Environmental Molecular Sciences Lab. (EMSL)
- Sponsoring Organization:
- USDOE
- DOE Contract Number:
- AC05-76RL01830
- OSTI ID:
- 1054439
- Report Number(s):
- PNNL-SA-88270; 46003; 46900; KP1704020
- Journal Information:
- Journal of Physical Chemistry Letters, 3(17):2326-2331, Journal Name: Journal of Physical Chemistry Letters, 3(17):2326-2331
- Country of Publication:
- United States
- Language:
- English
Similar Records
Simulation and visualization of attosecond stimulated x-ray Raman spectroscopy signals in trans-N-methylacetamide at the nitrogen and oxygen K-edges
Manipulating quantum entanglement of quasiparticles in many-electron systems by attosecond x-ray pulses
Dissecting X-Ray Raman Resonances Using Four-Wave Mixing
Journal Article
·
Mon Mar 28 00:00:00 EDT 2011
· Journal of Chemical Physics
·
OSTI ID:1054439
Manipulating quantum entanglement of quasiparticles in many-electron systems by attosecond x-ray pulses
Journal Article
·
Tue Jun 15 00:00:00 EDT 2010
· Physical Review. A
·
OSTI ID:1054439
Dissecting X-Ray Raman Resonances Using Four-Wave Mixing
Conference
·
Tue Jan 01 00:00:00 EST 2013
· EPJ Web of Conferences
·
OSTI ID:1054439
+7 more