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Title: Experimental and semiempirical method to determine the Pauli-limiting field in quasi-two-dimensional superconductors as applied to κ-(BEDT-TTF)2Cu(NCS)2: strong evidence of a FFLO state

Abstract

We present upper critical field data for {kappa}-(BEDT-TTF){sub 2}Cu(NCS){sub 2} with the magnetic field close to parallel and parallel to the conducting layers. We show that we can eliminate the effect of vortex dynamics in these layered materials if the layers are oriented within 0.3-inch of parallel to the applied magnetic field. Eliminating vortex effects leaves one remaining feature in the data that corresponds to the Pauli paramagnetic limit (H{sub p}). We propose a semiempirical method to calculate the H{sub p} in quasi-2D superconductors. This method takes into account the energy gap of each of the quasi-2D superconductors, which is calculated from specific-heat data, and the influence of many-body effects. The calculated Pauli paramagnetic limits are then compared to critical field data for the title compound and other organic conductors. Many of the examined quasi-2D superconductors, including the above organic superconductors and CeCoIn{sub 5}, exhibit upper critical fields that exceed their calculated H{sub p} suggesting unconventional superconductivity. We show that the high-field low-temperature state in {kappa}-(BEDT-TTF){sub 2}Cu(NCS){sub 2} is consistent with the Fulde-Ferrell-Larkin-Ovchinnikov state.

Authors:
; ; ; ; ; ; ; ; ; ; ;  [1];  [2];  [2];  [2]
  1. (Materials Science Division)
  2. (
Publication Date:
Research Org.:
Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1050177
Report Number(s):
ANL/MSD/JA-72068
Journal ID: ISSN 1098-0121; TRN: US201218%%530
DOE Contract Number:
DE-AC02-06CH11357
Resource Type:
Journal Article
Resource Relation:
Journal Name: Physical Review. B, Condensed Matter and Materials Physics; Journal Volume: 85; Journal Issue: 21
Country of Publication:
United States
Language:
ENGLISH
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; CRITICAL FIELD; ENERGY GAP; MAGNETIC FIELDS; ORGANIC SUPERCONDUCTORS; SPECIFIC HEAT; SUPERCONDUCTIVITY; SUPERCONDUCTORS

Citation Formats

Agosta, C. C., Jin, J., Coniglio, W. A., Smith, B. E., Cho, K., Mihut, I., Martin, C., Tozer, S. W., Murphy, T. P., Palm, E. C., Schlueter, J. A., Kurmoo, M., Clark Univ.), Nat. High Field Magnet Lab.), and The Royal Inst.). Experimental and semiempirical method to determine the Pauli-limiting field in quasi-two-dimensional superconductors as applied to κ-(BEDT-TTF)2Cu(NCS)2: strong evidence of a FFLO state. United States: N. p., 2012. Web. doi:10.1103/PhysRevB.85.214514.
Agosta, C. C., Jin, J., Coniglio, W. A., Smith, B. E., Cho, K., Mihut, I., Martin, C., Tozer, S. W., Murphy, T. P., Palm, E. C., Schlueter, J. A., Kurmoo, M., Clark Univ.), Nat. High Field Magnet Lab.), & The Royal Inst.). Experimental and semiempirical method to determine the Pauli-limiting field in quasi-two-dimensional superconductors as applied to κ-(BEDT-TTF)2Cu(NCS)2: strong evidence of a FFLO state. United States. doi:10.1103/PhysRevB.85.214514.
Agosta, C. C., Jin, J., Coniglio, W. A., Smith, B. E., Cho, K., Mihut, I., Martin, C., Tozer, S. W., Murphy, T. P., Palm, E. C., Schlueter, J. A., Kurmoo, M., Clark Univ.), Nat. High Field Magnet Lab.), and The Royal Inst.). Sun . "Experimental and semiempirical method to determine the Pauli-limiting field in quasi-two-dimensional superconductors as applied to κ-(BEDT-TTF)2Cu(NCS)2: strong evidence of a FFLO state". United States. doi:10.1103/PhysRevB.85.214514.
@article{osti_1050177,
title = {Experimental and semiempirical method to determine the Pauli-limiting field in quasi-two-dimensional superconductors as applied to κ-(BEDT-TTF)2Cu(NCS)2: strong evidence of a FFLO state},
author = {Agosta, C. C. and Jin, J. and Coniglio, W. A. and Smith, B. E. and Cho, K. and Mihut, I. and Martin, C. and Tozer, S. W. and Murphy, T. P. and Palm, E. C. and Schlueter, J. A. and Kurmoo, M. and Clark Univ.) and Nat. High Field Magnet Lab.) and The Royal Inst.)},
abstractNote = {We present upper critical field data for {kappa}-(BEDT-TTF){sub 2}Cu(NCS){sub 2} with the magnetic field close to parallel and parallel to the conducting layers. We show that we can eliminate the effect of vortex dynamics in these layered materials if the layers are oriented within 0.3-inch of parallel to the applied magnetic field. Eliminating vortex effects leaves one remaining feature in the data that corresponds to the Pauli paramagnetic limit (H{sub p}). We propose a semiempirical method to calculate the H{sub p} in quasi-2D superconductors. This method takes into account the energy gap of each of the quasi-2D superconductors, which is calculated from specific-heat data, and the influence of many-body effects. The calculated Pauli paramagnetic limits are then compared to critical field data for the title compound and other organic conductors. Many of the examined quasi-2D superconductors, including the above organic superconductors and CeCoIn{sub 5}, exhibit upper critical fields that exceed their calculated H{sub p} suggesting unconventional superconductivity. We show that the high-field low-temperature state in {kappa}-(BEDT-TTF){sub 2}Cu(NCS){sub 2} is consistent with the Fulde-Ferrell-Larkin-Ovchinnikov state.},
doi = {10.1103/PhysRevB.85.214514},
journal = {Physical Review. B, Condensed Matter and Materials Physics},
number = 21,
volume = 85,
place = {United States},
year = {Sun Jan 01 00:00:00 EST 2012},
month = {Sun Jan 01 00:00:00 EST 2012}
}