skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Subband Structure of a Two-Dimensional Electron Gas Formed at the Polar Surface of the Strong Spin-Orbit Perovskite KTaO3

Technical Report ·
DOI:https://doi.org/10.2172/1035804· OSTI ID:1035804

We demonstrate the formation of a two-dimensional electron gas (2DEG) at the (100) surface of the 5d transition-metal oxide KTaO{sub 3}. From angle-resolved photoemission, we find that quantum confinement lifts the orbital degeneracy of the bulk band structure and leads to a 2DEG composed of ladders of subband states of both light and heavy carriers. Despite the strong spin-orbit coupling, we find no experimental signatures of a Rashba spin splitting, which has important implications for the interpretation of transport measurements in both KTaO{sub 3}- and SrTiO{sub 3}-based 2DEGs. The polar nature of the KTaO{sub 3}(100) surface appears to help mediate formation of the 2DEG as compared to non-polar SrTiO{sub 3}(100).

Research Organization:
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
AC02-76SF00515
OSTI ID:
1035804
Report Number(s):
SLAC-PUB-14625; TRN: US201206%%18
Country of Publication:
United States
Language:
English

Similar Records

Overview of theoretical studies of Rashba effect in polar perovskite surfaces
Journal Article · Wed Aug 27 00:00:00 EDT 2014 · Journal of Electron Spectroscopy and Related Phenomena · OSTI ID:1035804

Spectral weight reduction of two-dimensional electron gases at oxide surfaces across the ferroelectric transition
Journal Article · Thu Oct 08 00:00:00 EDT 2020 · Scientific Reports · OSTI ID:1035804

Engineering two-dimensional superconductivity and Rashba spin–orbit coupling in LaAlO3/SrTiO3 quantum wells by selective orbital occupancy
Journal Article · Tue Jan 13 00:00:00 EST 2015 · Nature Communications · OSTI ID:1035804