Scintillation materials for medical applications. Annual progress report, January 1, 1991--December 31, 1992
Abstract
Scintillators are beginning to attract renewed attention because modern High Energy Physics accelerators are placing unprecedented demands of quantity and quality of detector materials and Positron Emission Tomography (PET), used by the medical field. Both applications required materials for scintillator detectors with properties beyond those delivered by traditional scintillators. Thallium doped halides are very efficient, but slow and chemically unstable. Two modern developments, namely the very fast BaF{sub 2}, which owed its success to the newly discovered crossover transitions, and CeF{sub 3}, which carried a promise of fast components, more practical wavelengths and attractive efficiency. Since traditional scintillators (Tl doped halides) are very efficient, and could be even more efficient at larger concentrations of Tl, if it were not for concentration quenching. However Tl transitions are spin forbidden and slow. Both ills could be remedied by replacing Tl with Ce, whose transitions are allowed and which is known to form fully concentrated compounds of high photoluminescent efficiency and no quenching. These materials, plus new Ce-doped materials, exhibiting highly promising properties for medical applications, became the target of our studies.
- Authors:
- Publication Date:
- Research Org.:
- Boston Univ., MA (United States)
- Sponsoring Org.:
- USDOE, Washington, DC (United States)
- OSTI Identifier:
- 10159424
- Report Number(s):
- DOE/ER/61033-3
ON: DE93015356
- DOE Contract Number:
- FG02-90ER61033
- Resource Type:
- Technical Report
- Resource Relation:
- Other Information: PBD: [1992]
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 62 RADIOLOGY AND NUCLEAR MEDICINE; 59 BASIC BIOLOGICAL SCIENCES; POSITRON COMPUTED TOMOGRAPHY; PHOSPHORS; CERIUM FLUORIDES; PHOSPHORESCENCE; CERIUM PHOSPHATES; LANTHANUM FLUORIDES; LANTHANUM PHOSPHATES; RARE EARTH COMPOUNDS; PROGRESS REPORT; COMPARATIVE EVALUATIONS; 550601; 550501; 550201; UNSEALED RADIONUCLIDES IN DIAGNOSTICS; TRACER TECHNIQUES
Citation Formats
Lempicki, A., and Wojtowicz, A.J. Scintillation materials for medical applications. Annual progress report, January 1, 1991--December 31, 1992. United States: N. p., 1992.
Web. doi:10.2172/10159424.
Lempicki, A., & Wojtowicz, A.J. Scintillation materials for medical applications. Annual progress report, January 1, 1991--December 31, 1992. United States. doi:10.2172/10159424.
Lempicki, A., and Wojtowicz, A.J. Thu .
"Scintillation materials for medical applications. Annual progress report, January 1, 1991--December 31, 1992". United States.
doi:10.2172/10159424. https://www.osti.gov/servlets/purl/10159424.
@article{osti_10159424,
title = {Scintillation materials for medical applications. Annual progress report, January 1, 1991--December 31, 1992},
author = {Lempicki, A. and Wojtowicz, A.J.},
abstractNote = {Scintillators are beginning to attract renewed attention because modern High Energy Physics accelerators are placing unprecedented demands of quantity and quality of detector materials and Positron Emission Tomography (PET), used by the medical field. Both applications required materials for scintillator detectors with properties beyond those delivered by traditional scintillators. Thallium doped halides are very efficient, but slow and chemically unstable. Two modern developments, namely the very fast BaF{sub 2}, which owed its success to the newly discovered crossover transitions, and CeF{sub 3}, which carried a promise of fast components, more practical wavelengths and attractive efficiency. Since traditional scintillators (Tl doped halides) are very efficient, and could be even more efficient at larger concentrations of Tl, if it were not for concentration quenching. However Tl transitions are spin forbidden and slow. Both ills could be remedied by replacing Tl with Ce, whose transitions are allowed and which is known to form fully concentrated compounds of high photoluminescent efficiency and no quenching. These materials, plus new Ce-doped materials, exhibiting highly promising properties for medical applications, became the target of our studies.},
doi = {10.2172/10159424},
journal = {},
number = ,
volume = ,
place = {United States},
year = {Thu Dec 31 00:00:00 EST 1992},
month = {Thu Dec 31 00:00:00 EST 1992}
}
-
The primary objective of the present Phase 3 effort is to perform the final testing at a 20 MNBtu/hr commercial scale of an air cooled, slogging coal combustor for application to industrial steam boilers and power plants. The focus of the test effort will be on combustor durability, automatic control of the combustor`s operation, and optimum environmental control of emissions inside the combustor. In connection with the latter, the goal is to achieve 0.4 lb/MMBtu of SO{sub 2} emissions, 0.2 lb/MMBtu of NO{sub x} emissions, and 0.02 lb particulate/MMBtu. Meeting the particulate goal will require the use of a baghousemore »
-
Methanotrophs for biological pollution control: TCE removal and nutrient removal with the expanded bed. Annual report, January 1, 1991-December 31, 1992
This project had two separate goals; the development of an innovative high biomass attached microbial film reactor for biodegrading chlorinated ethenes and the removal of macronutrients, nitrogen and phosphorus, from wastewaters. The project was initiated in 1987 to identify new approaches to treat PCE and TCE and their by-products in innovative biological systems at the Department of Agricultural and Biological Engineering at Cornell University. This project was sponsored by the Gas Research Insitute and was part of a national effort to identify new and more cost-effective technologies to purify groundwater and other wastewaters. This is the final report in thismore » -
The theory of High Energy Collision Processes. Annual technical progress report, January 1, 1991--December 31, 1991
This report briefly discusses research in proton-antiproton interactions and the standard model. (LSP) -
Novel concepts in weld metal science: Role of gradients and composite structure. Annual technical progress report, January 1, 1991--December 31, 1991
The effects of compositional and microstructural gradients on weld metal properties are being investigated. Crack propagation is solidified alloy structures is being characterized as to solidification orientation and the profile of the compositional variations. The effects of compositional gradients, are considered based on a thermodynamic analysis, referred to as the Cahn-Hillard analysis, which describes the degree to which a local surface energy is modified by the presence of a compositional gradient. The analysis predicts that both ductile and brittle fracture mechanisms are enhanced by the presence of a composition gradient. Special techniques to produce laboratory samples with microstructures which simulatemore » -
Growth of high T{sub c} superconducting fibers using a miniaturized laser-heated float zone process. Annual progress report, January 1, 1992--December 31, 1992
This report covers the research done on {open_quotes}Growth of High Tc Superconducting Fibers using a Miniaturized Laser-Heated Float Zone Process{close_quotes} during the 12 months from Jan. 1, 1992 until Dec. 31, 1992. The major part of the work focused on phase relations and kinetics in the Bi{sub 2}O{sub 3}-SrO-CaO-CuO (BSCCO) system. By analyzing the crystal and melt composition, and the growth temperature of the float-zone samples, new data was obtained on the phase relationships. These results were shown to form a subset of solid solubility ranges reported by other investigators and was typical of the data available from other fluxmore »