Alcohol synthesis from CO or CO.sub.2

Hu, Jianli; Dagle, Robert A; Holladay, Jamelyn D; Cao, Chunshe; Wang, Yong; White, James F; Elliott, Douglas C; Stevens, Don J

Alcohol synthesis from CO or CO.sub.2

Patent · 27 December 2010

OSTI ID:1006421

Hu, Jianli ^[1]; Dagle, Robert A ^[2]; Holladay, Jamelyn D ^[1]; Cao, Chunshe ^[3]; Wang, Yong ^[2]; White, James F ^[2]; Elliott, Douglas C ^[2]; Stevens, Don J ^[2]

Kennewick, WA
Richland, WA
Houston, TX

Methods for producing alcohols from CO or CO.sub.2 and H.sub.2 utilizing a palladium-zinc on alumina catalyst are described. Methods of synthesizing alcohols over various catalysts in microchannels are also described. Ethanol, higher alcohols, and other C.sub.2+ oxygenates can produced utilizing Rh--Mn or a Fisher-Tropsch catalyst.

Research Organization:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Sponsoring Organization:: USDOE Office of Biomass Program (EE-2E)

DOE Contract Number:: AC06-76RL01830

Assignee:: Battelle Memorial Institute (Richland, WA)

Patent Number(s):: 7,858,667

Application Number:: 11/611,160

OSTI ID:: 1006421

Country of Publication:: United States

Language:: English

References (9)

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Highly dispersed Rh/SiO2 and Rh/MnO/SiO2 catalysts 1. Synthesis, Characterization, and CO Hydrogenation Activity Dejong, K. Journal of Catalysis, Vol. 124, Issue 2 https://doi.org/10.1016/0021-9517(90)90198-S	journal	August 1990
Syngas conversion using RhVO4 and Rh2MnO4 catalysts: Regeneration and redispersion of Rh metal by calcination and reduction treatments Ishiguro, S.; Ito, S.; Kunimori, K. Catalysis Today, Vol. 45, Issue 1-4 https://doi.org/10.1016/S0920-5861(98)00215-6	journal	October 1998
Hydrogenation of carbon dioxide to methanol over palladium-promoted Cu/ZnO/A12O3 catalysts Sahibzada, M.; Chadwick, D.; Metcalfe, I. S. Catalysis Today, Vol. 29, Issue 1-4 https://doi.org/10.1016/0920-5861(95)00306-1	journal	May 1996
The Reduction of Zinc Oxide by Hydrogen. III. The Effect of Nitrogen on the Reduction Imoto, Tatsuya; Harano, Yoshio; Nishi, Yasuhide Bulletin of the Chemical Society of Japan, Vol. 37, Issue 4 https://doi.org/10.1246/bcsj.37.441	journal	April 1964
Mechanism of ethanol formation from synthesis gas over CuO/ZnO/Al2O3 Elliott, D. J.; Pennella, Filippo Journal of Catalysis, Vol. 114, Issue 1 https://doi.org/10.1016/0021-9517(88)90011-5	journal	November 1988
Conversion of Biomass Syngas to DME Using a Microchannel Reactor Hu, Jianli; Wang, Yong; Cao, Chunshe Industrial & Engineering Chemistry Research, Vol. 44, Issue 6 https://doi.org/10.1021/ie0492707	journal	March 2005
Effective synthesis of ethanol from CO2 on polyfunctional composite catalysts Inui, Tomoyuki; Yamamoto, Tetsuo Catalysis Today, Vol. 45, Issue 1-4 https://doi.org/10.1016/S0920-5861(98)00217-X	journal	October 1998
Characteristics of the Synthesis of Methanol Using Biomass-Derived Syngas Yin, Xiuli; Leung, Dennis Y. C.; Chang, Jie Energy & Fuels, Vol. 19, Issue 1 https://doi.org/10.1021/ef0498622	journal	January 2005

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