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Title: Experimentally determining the exchange parameters of quasi-two dimensional Heisenbert magnets

Journal Article · · New Journal of Physics
OSTI ID:960573

Though long-range magnetic order cannot occur at temperatures T > 0 in a perfect two-dimensional (2D) Heisenberg magnet, real quasi-2D materials will invariably possess nonzero inter-plane coupling J{sub {perpendicular}} driving the system to order at elevated temperatures. This process can be studied using quantum Monte Carlo calculations. However, it is difficult to test the results of these calculations experimentally since for highly anisotropic materials in which the in-plane coupling is comparable with attainable magnetic fields J{sub {perpendicular}} is necessarily very small and inaccessible directly. In addition, because of the large anisotropy, the Neel temperatures are low and difficult to determine from thermodynamic measurements. Here, we present an elegant method of assessing the calculations via two independent experimental probes: pulsed-field magnetization in fields of up to 85 T, and muon-spin rotation.

Research Organization:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
AC52-06NA25396
OSTI ID:
960573
Report Number(s):
LA-UR-08-05324; LA-UR-08-5324; TRN: US1002072
Journal Information:
New Journal of Physics, Journal Name: New Journal of Physics
Country of Publication:
United States
Language:
English