Carrier-free Radioisotopes from Cyclotron Targets I. Preparation and Isolation of Sn113 and In114 from Cadmium
The cyclotron is the only practical source of many carrier-free radioisotopes. The preparation and radiochemical isolation of a number of these activities, produced in the 60-inch cyclotron of Crocker Laboratory, will be presented in this paper and in subsequent papers of this series. In most cases the carrier-free radioisotopes were prepared for use in biological systems and the final preparations were in the form of isotonic saline solutions at a range of pH from 5 to 8. The present paper reports the radiochemical isolation of carrier-free Sn{sup 113} and In{sup 114} produced by bombarding cadmium with 38 Mev alpha-particles. At this energy, Sn{sup 113} and In{sup 114} are produced in a thick target by the nuclear reactions; Cd{sup 110}({alpha},n)Sn{sup 113}, Cd{sup 111}({alpha},2n)Sn{sup 113}, Cd{sup 112}({alpha},3n)Sn{sup 113}, Cd{sup 111}({alpha},p)In{sup 114}, Cd{sup 112}({alpha},pn) In{sup 114}. The shorter-lived tin and indium activities together with the possible radioisotopes of silver produced by (n,p) reactions, were allowed to decay out prior to the chemical separations.
- Research Organization:
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Sponsoring Organization:
- Physics Division
- DOE Contract Number:
- DE-AC02-05CH11231
- OSTI ID:
- 942299
- Report Number(s):
- UCRL-403; TRN: US200902%%245
- Country of Publication:
- United States
- Language:
- English
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