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Title: Multi-stage selection catalytic reduction of NO{sub x} in lean burn engine exhaust

Conference ·
OSTI ID:325395

Recent studies suggest that the conversion of NO to NO{sub 2} is an important intermediate step in the selective catalytic reduction (SCR) of NO{sub x} to N{sub 2}. These studies have prompted the development of schemes that use an oxidation catalyst to convert NO to NO{sub 2}, followed by a reduction catalyst to convert NO{sub 2} to N{sub 2}. Multi-stage SCR offers high NO{sub x} reduction efficiency from catalysts that, separately, are not very active for reduction of NO, and alleviates the problem of selectivity between NO reduction and hydrocarbon oxidation. A plasma can also be used to oxidize NO to NO{sub 2}. This paper compares the multi-stage catalytic scheme with the plasma-assisted catalytic scheme for reduction of NO{sub x} in lean-bum engine exhausts. The advantages of plasma oxidation over catalytic oxidation are presented.

Research Organization:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Sponsoring Organization:
USDOE Office of Energy Research, Washington, DC (United States)
DOE Contract Number:
W-7405-ENG-48
OSTI ID:
325395
Report Number(s):
UCRL-JC-128071; CONF-970799-; ON: DE98052275; BR: KC0302010
Resource Relation:
Conference: 1997 diesel engine emissions reduction workshop, San Diego, CA (United States), 27-31 Jul 1997; Other Information: PBD: 26 Jan 1998
Country of Publication:
United States
Language:
English