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Title: Short-range atmospheric dispersion of carbon dioxide

Journal Article · · Boundary-Layer Meteorology

We present a numerical study aimed at quantifying the effects of concentration-dependent density on the spread of a seeping plume of CO{sub 2} into the atmosphere such as could arise from a leaking geologic carbon sequestration site. Results of numerical models can be used to supplement field monitoring estimates of CO{sub 2} seepage flux by modelling transport and dispersion between the source emission and concentration-measurement points. We focus on modelling CO{sub 2} seepage dispersion over relatively short distances where density effects are likely to be important. We model dense gas dispersion using the steady-state Reynolds-averaged Navier-Stokes equations with density dependence in the gravity term. Results for a two-dimensional system show that a density dependence emerges at higher fluxes than prior estimates. A universal scaling relation is derived that allows estimation of the flux from concentrations measured downwind and vice versa.

Research Organization:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
Earth Sciences Division
DOE Contract Number:
DE-AC02-05CH11231
OSTI ID:
981340
Report Number(s):
LBNL-2964E; BLMEBR; TRN: US201012%%1315
Journal Information:
Boundary-Layer Meteorology, Vol. 133, Issue 1; Related Information: Journal Publication Date: 2009; ISSN 0006-8314
Country of Publication:
United States
Language:
English