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Title: Fabrication and Characterization of Suspended Carbon Nanotube Devices in Liquid

Abstract

Suspended carbon nanotube devices are a promising platform for future bio-electronic applications. Suspended carbon nanotube transistors have been previously fabricated in air; however all previous attempts to bring them into liquid failed. We analyze forces acting on the suspended nanotube devices during immersion into liquids and during device operation and show that surface tension forces acting on the suspended nanotubes during transfer into the liquid phase are responsible for the nanotube damage. We have developed a new strategy that circumvents these limitations by coating suspended nanotubes with a rigid inorganic shell in the gas phase. The coating reinforces the nanotubes and allows them to survive transfer through the interface. Subsequent removal of the coating in the solution phase restores pristine suspended nanotubes. We demonstrate that devices fabricated using this technique preserve their original electrical characteristics.

Authors:
; ; ; ;
Publication Date:
Research Org.:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
936945
Report Number(s):
UCRL-JRNL-225782
TRN: US200821%%146
DOE Contract Number:  
W-7405-ENG-48
Resource Type:
Journal Article
Journal Name:
International Journal of Nanotechnology, vol. 5, no. 4/5, April 1, 2008, pp. 488-496
Additional Journal Information:
Journal Volume: 5; Journal Issue: 4/5
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; AIR; CARBON; COATINGS; FABRICATION; NANOTUBES; REMOVAL; SURFACE TENSION; TRANSISTORS

Citation Formats

Artyukhin, A, Stadermann, M, Stroeve, P, Bakajin, O, and Noy, A. Fabrication and Characterization of Suspended Carbon Nanotube Devices in Liquid. United States: N. p., 2006. Web.
Artyukhin, A, Stadermann, M, Stroeve, P, Bakajin, O, & Noy, A. Fabrication and Characterization of Suspended Carbon Nanotube Devices in Liquid. United States.
Artyukhin, A, Stadermann, M, Stroeve, P, Bakajin, O, and Noy, A. 2006. "Fabrication and Characterization of Suspended Carbon Nanotube Devices in Liquid". United States. https://www.osti.gov/servlets/purl/936945.
@article{osti_936945,
title = {Fabrication and Characterization of Suspended Carbon Nanotube Devices in Liquid},
author = {Artyukhin, A and Stadermann, M and Stroeve, P and Bakajin, O and Noy, A},
abstractNote = {Suspended carbon nanotube devices are a promising platform for future bio-electronic applications. Suspended carbon nanotube transistors have been previously fabricated in air; however all previous attempts to bring them into liquid failed. We analyze forces acting on the suspended nanotube devices during immersion into liquids and during device operation and show that surface tension forces acting on the suspended nanotubes during transfer into the liquid phase are responsible for the nanotube damage. We have developed a new strategy that circumvents these limitations by coating suspended nanotubes with a rigid inorganic shell in the gas phase. The coating reinforces the nanotubes and allows them to survive transfer through the interface. Subsequent removal of the coating in the solution phase restores pristine suspended nanotubes. We demonstrate that devices fabricated using this technique preserve their original electrical characteristics.},
doi = {},
url = {https://www.osti.gov/biblio/936945}, journal = {International Journal of Nanotechnology, vol. 5, no. 4/5, April 1, 2008, pp. 488-496},
number = 4/5,
volume = 5,
place = {United States},
year = {Mon Oct 30 00:00:00 EST 2006},
month = {Mon Oct 30 00:00:00 EST 2006}
}