Modeling of water radiolysis at spallation neutron sources
In spallation neutron sources neutrons are produced when a beam of high-energy particles (e.g., 1 GeV protons) collides with a (water-cooled) heavy metal target such as tungsten. The resulting spallation reactions produce a complex radiation environment (which differs from typical conditions at fission and fusion reactors) leading to the radiolysis of water molecules. Most water radiolysis products are short-lived but extremely reactive. When formed in the vicinity of the target surface they can react with metal atoms, thereby contributing to target corrosion. The authors describe the results of calculations and experiments performed at los alamos to determine the impact on target corrosion of water radiolysis in the spallation radiation environment. The computational methodology relies on the use of the Los Alamos radiation transport code, LAHET, to determine the radiation environment, and the AEA code, FACSIMILE, to model reaction-diffusion processes.
- Research Organization:
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Sponsoring Organization:
- USDOE Office of Energy Research, Washington, DC (United States)
- DOE Contract Number:
- W-7405-ENG-36
- OSTI ID:
- 677142
- Report Number(s):
- LA-UR-98-1023; CONF-970201-; ON: DE99000681; TRN: 99:001265
- Resource Relation:
- Conference: 126. annual meeting of the Minerals, Metals and Materials Society, Orlando, FL (United States), 9-13 Feb 1997; Other Information: PBD: [1998]
- Country of Publication:
- United States
- Language:
- English
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