Retained gas sampler extractor mixing and mass transfer rate study: Experimental and simulation results
Research staff at Pacific Northwest National Laboratory conducted experimental testing and computer simulations of the impeller-stirred Retained Gas Sampler (RGS) gas extractor system. This work was performed to verify experimentally the effectiveness of the extractor at mixing viscous fluids of both Newtonian and non-Newtonian rheology representative of Hanford single- and double-shell wastes, respectively. Developing the computational models and validating their results by comparing them with experimental results would enable simulations of the mixing process for a range of fluid properties and mixing speeds. Five tests were performed with a full-scale, optically transparent model extractor to provide the data needed to compare mixing times for fluid rheology, mixer rotational direction, and mixing speed variation. The computer model was developed and exercised to simulate the tests. The tests demonstrated that rotational direction of the pitched impeller blades was not as important as fluid rheology in determining mixing time. The Newtonian fluid required at least six hours to mix at the hot cell operating speed of 3 rpm, and the non-Newtonian fluid required at least 46 hours at 3 rpm to become significantly mixed. In the non-Newtonian fluid tests, stagnant regions within the fluid sometimes required days to be fully mixed. Higher-speed (30 rpm) testing showed that the laminar mixing time was correlated to mixing speed. The tests demonstrated that, using the RGS extractor and current procedures, complete mixing of the waste samples in the hot cell should not be expected. The computer simulation of Newtonian fluid mixing gave results comparable to the test while simulation of non-Newtonian fluid mixing would require further development. In light of the laboratory test results, detailed parametric analysis of the mixing process was not performed.
- Research Organization:
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
- Sponsoring Organization:
- USDOE Office of Environmental Restoration and Waste Management, Washington, DC (United States)
- DOE Contract Number:
- AC06-76RL01830
- OSTI ID:
- 671886
- Report Number(s):
- PNNL-11759; ON: DE98051303; TRN: 99:000404
- Resource Relation:
- Other Information: PBD: Nov 1997
- Country of Publication:
- United States
- Language:
- English
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