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Title: Nuclear waste form risk assessment for US defense waste at Savannah River Plant. Annual report fiscal year 1980

Technical Report ·
DOI:https://doi.org/10.2172/5826727· OSTI ID:5826727

Waste form dissolution studies and preliminary performance analyses were carried out to contribute a part of the data needed for the selection of a waste form for the disposal of Savannah River Plant defense waste in a deep geologic repository. The first portion of this work provides descriptions of the chemical interactions between the waste form and the geologic environment. We reviewed critically the dissolution/leaching data for borosilicate glass and SYNROC. Both chemical kinetic and thermodynamic models were developed to describe the dissolution process of these candidate waste forms so as to establish a fundamental basis for interpretation of experimental data and to provide directions for future experiments. The complementary second portion of this work is an assessment of the impacts of alternate waste forms upon the consequences of disposal in various proposed geological media. Employing systems analysis methodology, we began to evaluate the performance of a generic waste form for the case of a high risk scenario for a bedded salt repository. Results of sensitivity analysis, uncertainty analyses, and sensitivity to uncertainty analysis are presented.

Research Organization:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
DOE Contract Number:
W-7405-ENG-48
OSTI ID:
5826727
Report Number(s):
UCRL-53188-80; ON: DE82005602; TRN: 82-004795
Country of Publication:
United States
Language:
English