Vibrational spectroscopy of shock-compressed liquid CO
Single-pulse, multiplex, coherent anti-Stokes Raman spectroscopy (CARS) was used to observe the vibrational spectra of liquid CO shock compressed to several pressures and temperatures up to 9.9 GPa and 2010 K. The experimental spectra were compared to synthetic spectra calculated using a semiclassical model for CARS intensities and estimated vibrational frequencies, peak Raman susceptibilities and Raman line widths. A comparison of these data with result in the isoelectronic and materially very similar N{sub 2} show a significant difference in vibrational frequency shift with pressure. 21 refs., 2 figs.
- Research Organization:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Sponsoring Organization:
- USDOE; USDOE, Washington, DC (USA)
- DOE Contract Number:
- W-7405-ENG-36
- OSTI ID:
- 5728988
- Report Number(s):
- LA-UR-91-1666; CONF-9107105-9; ON: DE91013204
- Resource Relation:
- Conference: 1991 American Physical Society (APS) conference on shock compression of condensed matter, Williamsburg, VA (USA), 17-20 Jul 1991
- Country of Publication:
- United States
- Language:
- English
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Related Subjects
75 CONDENSED MATTER PHYSICS
SUPERCONDUCTIVITY AND SUPERFLUIDITY
74 ATOMIC AND MOLECULAR PHYSICS
CARBON MONOXIDE
RAMAN SPECTROSCOPY
DYE LASERS
IMPACT SHOCK
LIQUIDS
PRESSURE DEPENDENCE
RAMAN SPECTRA
TEMPERATURE DEPENDENCE
VIBRATIONAL STATES
CARBON COMPOUNDS
CARBON OXIDES
CHALCOGENIDES
ENERGY LEVELS
EXCITED STATES
FLUIDS
LASER SPECTROSCOPY
LASERS
LIQUID LASERS
OXIDES
OXYGEN COMPOUNDS
SPECTRA
SPECTROSCOPY
656002* - Condensed Matter Physics- General Techniques in Condensed Matter- (1987-)
640302 - Atomic
Molecular & Chemical Physics- Atomic & Molecular Properties & Theory
SUPERCONDUCTIVITY AND SUPERFLUIDITY
74 ATOMIC AND MOLECULAR PHYSICS
CARBON MONOXIDE
RAMAN SPECTROSCOPY
DYE LASERS
IMPACT SHOCK
LIQUIDS
PRESSURE DEPENDENCE
RAMAN SPECTRA
TEMPERATURE DEPENDENCE
VIBRATIONAL STATES
CARBON COMPOUNDS
CARBON OXIDES
CHALCOGENIDES
ENERGY LEVELS
EXCITED STATES
FLUIDS
LASER SPECTROSCOPY
LASERS
LIQUID LASERS
OXIDES
OXYGEN COMPOUNDS
SPECTRA
SPECTROSCOPY
656002* - Condensed Matter Physics- General Techniques in Condensed Matter- (1987-)
640302 - Atomic
Molecular & Chemical Physics- Atomic & Molecular Properties & Theory